113 research outputs found
Role of Linker Functionality in Polymers Exhibiting Main-Chain Thermally Activated Delayed Fluorescence
Excellent performance has been reported for organic lightâemitting diodes (OLEDs) based on small molecule emitters that exhibit thermally activated delayed fluorescence. However, the necessary vacuum processing makes the fabrication of largeâarea devices based on these emitters cumbersome and expensive. Here, the authors present high performance OLEDs, based on novel, TADF polymers that can be readily processed from a solution. These polymers are based on the acridineâbenzophenone donorâacceptor motif as mainâchain TADF chromophores, linked by various conjugated and nonâconjugated spacer moieties. The authorsâ extensive spectroscopic and electronic analysis shows that in particular in case of alkyl spacers, the properties and performance of the monomeric TADF chromophores are virtually left unaffected by the polymerization. They present efficient solutionâprocessed OLEDs based on these TADF polymers, diluted in oligostyrene as a host. The devices based on the alkyl spacerâbased TADF polymers exhibit external quantum efficiencies (EQEs) â12%, without any outcouplingâenhancing measures. What's more, the EQE of these devices does not drop substantially upon diluting the polymer down to only ten weight percent of active material. In contrast, the EQE of devices based on the monomeric chromophore show significant losses upon dilution due to loss of charge percolation
The search for transient astrophysical neutrino emission with IceCube-DeepCore
We present the results of a search for astrophysical sources of brief transient neutrino emission using IceCube and DeepCore data acquired between 2012 May 15 and 2013 April 30. While the search methods employed in this analysis are similar to those used in previous IceCube point source searches, the data set being examined consists of a sample of predominantly sub-TeV muon-neutrinos from the Northern Sky (-5 degrees < delta < 90 degrees) obtained through a novel event selection method. This search represents a first attempt by IceCube to identify astrophysical neutrino sources in this relatively unexplored energy range. The reconstructed direction and time of arrival of neutrino events are used to search for any significant self-correlation in the data set. The data revealed no significant source of transient neutrino emission. This result has been used to construct limits at timescales ranging from roughly 1 s to 10 days for generic soft-spectra transients. We also present limits on a specific model of neutrino emission from soft jets in core-collapse supernovae
All-sky search for time-integrated neutrino emission from astrophysical sources with 7 years of IceCube data
Since the recent detection of an astrophysical flux of high energy neutrinos,
the question of its origin has not yet fully been answered. Much of what is
known about this flux comes from a small event sample of high neutrino purity,
good energy resolution, but large angular uncertainties. In searches for
point-like sources, on the other hand, the best performance is given by using
large statistics and good angular reconstructions. Track-like muon events
produced in neutrino interactions satisfy these requirements. We present here
the results of searches for point-like sources with neutrinos using data
acquired by the IceCube detector over seven years from 2008--2015. The
discovery potential of the analysis in the northern sky is now significantly
below , on average
lower than the sensitivity of the previously published analysis of four
years exposure. No significant clustering of neutrinos above background
expectation was observed, and implications for prominent neutrino source
candidates are discussed.Comment: 19 pages, 17 figures, 3 tables; ; submitted to The Astrophysical
Journa
Characterization of the Atmospheric Muon Flux in IceCube
Muons produced in atmospheric cosmic ray showers account for the by far
dominant part of the event yield in large-volume underground particle
detectors. The IceCube detector, with an instrumented volume of about a cubic
kilometer, has the potential to conduct unique investigations on atmospheric
muons by exploiting the large collection area and the possibility to track
particles over a long distance. Through detailed reconstruction of energy
deposition along the tracks, the characteristics of muon bundles can be
quantified, and individual particles of exceptionally high energy identified.
The data can then be used to constrain the cosmic ray primary flux and the
contribution to atmospheric lepton fluxes from prompt decays of short-lived
hadrons.
In this paper, techniques for the extraction of physical measurements from
atmospheric muon events are described and first results are presented. The
multiplicity spectrum of TeV muons in cosmic ray air showers for primaries in
the energy range from the knee to the ankle is derived and found to be
consistent with recent results from surface detectors. The single muon energy
spectrum is determined up to PeV energies and shows a clear indication for the
emergence of a distinct spectral component from prompt decays of short-lived
hadrons. The magnitude of the prompt flux, which should include a substantial
contribution from light vector meson di-muon decays, is consistent with current
theoretical predictions.Comment: 36 pages, 39 figure
Neutrinos and Cosmic Rays Observed by IceCube
The core mission of the IceCube Neutrino observatory is to study the origin
and propagation of cosmic rays. IceCube, with its surface component IceTop,
observes multiple signatures to accomplish this mission. Most important are the
astrophysical neutrinos that are produced in interactions of cosmic rays, close
to their sources and in interstellar space. IceCube is the first instrument
that measures the properties of this astrophysical neutrino flux, and
constrains its origin. In addition, the spectrum, composition and anisotropy of
the local cosmic-ray flux are obtained from measurements of atmospheric muons
and showers. Here we provide an overview of recent findings from the analysis
of IceCube data, and their implications on our understanding of cosmic rays.Comment: Review article, to appear in Advances in Space Research, special
issue "Origins of Cosmic Rays
The IceCube Neutrino Observatory - Contributions to ICRC 2015 Part II: Atmospheric and Astrophysical Diffuse Neutrino Searches of All Flavors
Papers on atmospheric and astrophysical diffuse neutrino searches of all
flavors submitted to the 34th International Cosmic Ray Conference (ICRC 2015,
The Hague) by the IceCube Collaboration.Comment: 66 pages, 36 figures, Papers submitted to the 34th International
Cosmic Ray Conference, The Hague 2015, v2 has a corrected author lis
Searches for sterile neutrinos with the IceCube detector
The IceCube neutrino telescope at the South Pole has measured the atmospheric muon neutrino spectrum as a function of zenith angle and energy in the approximate 320 GeV to 20 TeV range, to search for the oscillation signatures of light sterile neutrinos. No evidence for anomalous nu(mu) or (nu) over bar (mu) disappearance is observed in either of two independently developed analyses, each using one year of atmospheric neutrino data. New exclusion limits are placed on the parameter space of the 3 + 1 model, in which muon antineutrinos experience a strong Mikheyev-Smirnov-Wolfenstein-resonant oscillation. The exclusion limits extend to sin(2)2 theta(24) <= 0.02 at Delta m(2) similar to 0.3 eV(2) at the 90% confidence level. The allowed region from global analysis of appearance experiments, including LSND and MiniBooNE, is excluded at approximately the 99% confidence level for the global best-fit value of vertical bar U-e4 vertical bar(2)
Observation and Characterization of a Cosmic Muon Neutrino Flux from the Northern Hemisphere using six years of IceCube data
The IceCube Collaboration has previously discovered a high-energy
astrophysical neutrino flux using neutrino events with interaction vertices
contained within the instrumented volume of the IceCube detector. We present a
complementary measurement using charged current muon neutrino events where the
interaction vertex can be outside this volume. As a consequence of the large
muon range the effective area is significantly larger but the field of view is
restricted to the Northern Hemisphere. IceCube data from 2009 through 2015 have
been analyzed using a likelihood approach based on the reconstructed muon
energy and zenith angle. At the highest neutrino energies between 191 TeV and
8.3 PeV a significant astrophysical contribution is observed, excluding a
purely atmospheric origin of these events at significance. The
data are well described by an isotropic, unbroken power law flux with a
normalization at 100 TeV neutrino energy of
and a hard spectral index of . The observed spectrum is
harder in comparison to previous IceCube analyses with lower energy thresholds
which may indicate a break in the astrophysical neutrino spectrum of unknown
origin. The highest energy event observed has a reconstructed muon energy of
which implies a probability of less than 0.005% for
this event to be of atmospheric origin. Analyzing the arrival directions of all
events with reconstructed muon energies above 200 TeV no correlation with known
-ray sources was found. Using the high statistics of atmospheric
neutrinos we report the currently best constraints on a prompt atmospheric muon
neutrino flux originating from charmed meson decays which is below in
units of the flux normalization of the model in Enberg et al. (2008).Comment: 20 pages, 21 figure
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