751 research outputs found
Power-law carrier dynamics in semiconductor nanocrystals at nanosecond time scales
We report the observation of power law dynamics on nanosecond to microsecond
time scales in the fluorescence decay from semiconductor nanocrystals, and draw
a comparison between this behavior and power-law fluorescence blinking from
single nanocrystals. The link is supported by comparison of blinking and
lifetime data measured simultaneously from the same nanocrystal. Our results
reveal that the power law coefficient changes little over the nine decades in
time from 10 ns to 10 s, in contrast with the predictions of some diffusion
based models of power law behavior.Comment: 3 pages, 2 figures, compressed for submission to Applied Physics
Letter
The broadening of Fe II lines by neutral hydrogen collisions
Data for the broadening of 24188 Fe II lines by collisions with neutral
hydrogen atoms have been computed using the theory of Anstee & O'Mara as
extended to singly ionised species and higher orbital angular momentum states
by Barklem & O'Mara. Data have been computed for all Fe II lines between
observed energy levels in the line lists of Kurucz with log gf > -5 for which
the theory is applicable. The variable energy debt parameter Ep used in
computing the second order perturbation theory potential is chosen to be
consistent with the long range dispersion interaction constant C6 computed
using the f-values from Kurucz.Comment: Accepted for A&A. 5 pages, 5 figures, 2 electronic tables. Tables
will be available via CDS; presently also at
http://www.astro.uu.se/~barklem/papers/fe2_data.tar.g
The Ratio of Ortho- to Para-H2 in Photodissociation Regions
We discuss the ratio of ortho- to para-H2 in photodissociation regions
(PDRs). We draw attention to an apparent confusion in the literature between
the ortho-to-para ratio of molecules in FUV-pumped vibrationally excited
states, and the H2 ortho-to-para abundance ratio. These ratios are not the same
because the process of FUV-pumping of fluorescent H2 emission in PDRs occurs
via optically thick absorption lines. Thus, gas with an equilibrium ratio of
ortho- to para-H2 equal to 3 will yield FUV-pumped vibrationally excited
ortho-to-para ratios smaller than 3, because the ortho-H2 pumping rates are
preferentially reduced by optical depth effects. Indeed, if the ortho and para
pumping lines are on the ``square root'' part of the curve-of-growth, then the
expected ratio of ortho and para vibrational line strengths is the square root
of 3, ~ 1.7, close to the typically observed value. Thus, contrary to what has
sometimes been stated in the literature, most previous measurements of the
ratio of ortho- to para-H2 in vibrationally excited states are entirely
consistent with a total ortho-to-para ratio of 3, the equilibrium value for
temperatures greater than 200 K. We present an analysis and several detailed
models which illustrate the relationship between the total ratios of ortho- to
para-H2 and the vibrationally excited ortho-to-para ratios in PDRs. Recent
Infrared Space Observatory (ISO) measurements of pure rotational and
vibrational H2 emissions from the PDR in the star-forming region S140 provide
strong observational support for our conclusions.Comment: 23 pages (including 5 figures), LaTeX, uses aaspp4.sty, accepted for
publication in Ap
Rate coefficients for rovibrational transitions in H_2 due to collisions with He
We present quantum mechanical and quasiclassical trajectory calculations of
cross sections for rovibrational transitions in ortho- and para-H_2 induced by
collisions with He atoms. Cross sections were obtained for kinetic energies
between 10^-4 and 3 eV, and the corresponding rate coefficients were calculated
for the temperature range 100<T<4000 K. Comparisons are made with previous
calculations.Comment: 21 pages, 2 figures, AAS, eps
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Design and Additive Fabrication of Foot and Ankle-Foot Orthoses
Foot and ankle-foot orthoses are prescribed in order to promote mobility through supporting
and/or realigning the lower leg and alleviating pain in the foot in different parts of the gait
cycle. This paper will outline new approaches to the design and manufacture of personalised
foot and ankle-foot orthoses (FO and AFO) using additive fabrication technology. The
research is addressing the need for specific software design tools for orthosis design which
enable their properties to be locally tailored within a mass customisation framework.
Structure/material testing to support that activity is also being undertaken and will be
described.Mechanical Engineerin
Ultracold collision properties of metastable alkaline-earth atoms
Ultra-cold collisions of spin-polarized 24Mg,40Ca, and 88Sr in the metastable
3P2 excited state are investigated. We calculate the long-range interaction
potentials and estimate the scattering length and the collisional loss rate as
a function of magnetic field. The estimates are based on molecular potentials
between 3P2 alkaline-earth atoms obtained from ab initio atomic and molecular
structure calculations. The scattering lengths show resonance behavior due to
the appearance of a molecular bound state in a purely long-range interaction
potential and are positive for magnetic fields below 50 mT. A loss-rate model
shows that losses should be smallest near zero magnetic field and for fields
slightly larger than the resonance field, where the scattering length is also
positive.Comment: 4 pages, 4 figure
Separation and identification of dominant mechanisms in double photoionization
Double photoionization by a single photon is often discussed in terms of two
contributing mechanisms, {\it knock-out} (two-step-one) and {\it shake-off}
with the latter being a pure quantum effect. It is shown that a quasi-classical
description of knock-out and a simple quantum calculation of shake-off provides
a clear separation of the mechanisms and facilitates their calculation
considerably. The relevance of each mechanism at different photon energies is
quantified for helium. Photoionization ratios, integral and singly differential
cross sections obtained by us are in excellent agreement with benchmark
experimental data and recent theoretical results.Comment: 4 pages, 5 figure
Absorption and photoluminescence spectroscopy on a single self-assembled charge-tunable quantum dot
We have performed detailed photoluminescence (PL) and absorption spectroscopy
on the same single self-assembled quantum dot in a charge-tunable device. The
transition from neutral to charged exciton in the PL occurs at a more negative
voltage than the corresponding transition in absorption. We have developed a
model of the Coulomb blockade to account for this observation. At large
negative bias, the absorption broadens as a result of electron and hole
tunneling. We observe resonant features in this regime whenever the quantum dot
hole level is resonant with two-dimensional hole states located at the capping
layer-blocking barrier interface in our structure.Comment: 6 pages, 6 figure
A Search for EUV Emission from Comets with the Cosmic Hot Interstellar Plasma Spectrometer (CHIPS)
We have obtained EUV spectra between 90 and 255 \AA of the cometsC/2002 T7
(LINEAR), C/2001 Q4 (NEAT), and C/2004 Q2 (Machholz) near their perihelion
passages in 2004 with the Cosmic Hot Interstellar Plasma Spectrometer (CHIPS).
We obtained contemporaneous data on Comet NEAT Q4 with the X-ray
Observatory ACIS instrument, marking the first simultaneous EUV and X-ray
spectral observations of a comet. The total CHIPS/EUV observing times were 337
ks for Q4, 234 ks for T7, and 483 ks for Machholz and for both CHIPS and
we calculate we have captured all the comet flux in the instrument
field of view. We set upper limits on solar wind charge exchange emission lines
of O, C, N, Ne and Fe occurring in the spectral bandpass of CHIPS. The spectrum
of Q4 obtained with can be reproduced by modeling emission lines of
C, N O, Mg, Fe, Si, S, and Ne solar wind ions. The measured X-ray emission line
intensities are consistent with our predictions from a solar wind charge
exchange model. The model predictions for the EUV emission line intensities are
determined from the intensity ratios of the cascading X-ray and EUV photons
arising in the charge exchange processes. They are compatible with the measured
limits on the intensities of the EUV lines. For comet Q4, we measured a total
X-ray flux of 3.7 ergs cm s, and derive from
model predictions a total EUV flux of 1.5 erg cm
s. The CHIPS observations occurred predominantly while the satellite was
on the dayside of Earth. For much of the observing time, CHIPS performed
observations at smaller solar angles than it was designed for and EUV emission
from the Sun scattered into the instrument limited the sensitivity of the EUV
measurements.Comment: 28 pages total, 4 tables, 7 figures. Accepted by The Astrophysical
Journa
Near-Infrared Spectroscopy of Molecular Filaments in the Reflection Nebula NGC 7023
We present near-infrared spectroscopy of fluorescent molecular hydrogen (H_2)
emission from molecular filaments in the reflection nebula NGC 7023. We derive
the relative column densities of H_2 rotational-vibrational states from the
measured line emission and compare these results with several model
photodissociation regions covering a range of densities, incident UV-fields,
and excitation mechanisms. Our best-fit models for one filament suggest, but do
not require, either a combination of different densities, suggesting clumps of
10^6 cm^{-3} in a 10^4 - 10^5 cm^{-3} filament, or a combination of fluorescent
excitation and thermally-excited gas, perhaps due to a shock from a bipolar
outflow. We derive densities and UV fields for these molecular filaments that
are in agreement with previous determinations.Comment: ApJ accepted, 26 pages including 5 embedded figures, uses AASTEX.
Also available at http://www-astronomy.mps.ohio-state.edu/~martini/pubs.htm
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