845 research outputs found
Spatiotemporal imaging of valence electron motion
Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural phenomena such as light-induced phase transitions and chemical reactions. Whereas static electron densities in single molecules can be imaged in real space using scanning tunnelling and atomic force microscopy, probing real-time electron motion inside molecules requires ultrafast laser pulses. Here, we demonstrate an all-optical approach to imaging an ultrafast valence electron wave packet in real time with a time-resolution of a few femtoseconds. We employ a pump-probe-deflect scheme that allows us to prepare an ultrafast wave packet via strong-field ionization and directly image the resulting charge oscillations in the residual ion. This approach extends and overcomes limitations in laser-induced orbital imaging and may enable the real-time imaging of electron dynamics following photoionization such as charge migration and charge transfer processes
Three-particle States in Nonrelativistic Four-fermion Model
On a nonrelativistic contact four-fermion model we have shown that the simple
Lambda-cut-off prescription together with definite fine-tuning of the Lambda
dependency of "bare"quantities lead to self-adjoint semi-bounded Hamiltonian in
one-, two- and three-particle sectors. The fixed self-adjoint extension and
exact solutions in two-particle sector completely define three-particle
problem. The renormalized Faddeev equations for the bound states with Fredholm
properties are obtained and analyzed.Comment: 9 pages, LaTex, no figure
Measurement of air fluorescence light yield induced by an electromagnetic shower
For most of the Ultra High Energy Cosmic Ray (UHECR) experiments and projects (HiRes, AUGER, TA, JEM-EUSO, TUS,...), the detection technique of Extensive Air Showers (EAS) is based, at least, on the measurement of the air fluorescence induced signal. The knowledge of the Fluorescence Light Yield (FLY) is of paramount importance for the UHECR energy reconstruction. The MACFLY experiment was designed to perform such FLY measurements. In this paper we will present the results of dry air FLY induced by 50 GeV electromagnetic showers as a function of shower age and as a function of the pressure. The experiment was performed at CERN using an SPS electron test beam line. It is shown that the FLY is proportional to deposited energy in air (E_d) and that the ratio FLY/E_d and its pressure dependence remain constant independently of shower age and more generally independently of the excitation source used (single electron track or air shower).For most of the Ultra High Energy Cosmic Ray (UHECR) experiments and projects (HiRes, AUGER, TA, JEM-EUSO, TUS,...), the detection technique of Extensive Air Showers (EAS) is based, at least, on the measurement of the air fluorescence induced signal. The knowledge of the Fluorescence Light Yield (FLY) is of paramount importance for the UHECR energy reconstruction. The MACFLY experiment was designed to perform such FLY measurements. In this paper we will present the results of dry air FLY induced by 50 GeV electromagnetic showers as a function of shower age and as a function of the pressure. The experiment was performed at CERN using an SPS electron test beam line. It is shown that the FLY is proportional to deposited energy in air (E_d) and that the ratio FLY/E_d and its pressure dependence remain constant independently of shower age and more generally independently of the excitation source used (single electron track or air shower)
Probing multiphoton light-induced molecular potentials
The strong coupling between intense laser fields and valence electrons in molecules causes distortions of the potential energy hypersurfaces which determine the motion of the nuclei and influence possible reaction pathways. The coupling strength varies with the angle between the light electric field and valence orbital, and thereby adds another dimension to the effective molecular potential energy surface, leading to the emergence of light-induced conical intersections. Here, we demonstrate that multiphoton couplings can give rise to complex light-induced potential energy surfaces that govern molecular behavior. In the laser-induced dissociation of H2+, the simplest of molecules, we measure a strongly modulated angular distribution of protons which has escaped prior observation. Using two-color Floquet theory, we show that the modulations result from ultrafast dynamics on light-induced molecular potentials. These potentials are shaped by the amplitude, duration and phase of the dressing fields, allowing for manipulating the dissociation dynamics of small molecules
Synthesis, Single Crystal Growth, and Properties of Cobalt Deficient Double Perovskite EuBaCo2-xO6-delta (x=0-0.1)
The cobalt deficient double perovskites EuBaCo2−xO6−δ with x=0–0.1 were obtained both as powders and as single crystal. Formation of cobalt vacancies in their crystal lattice was shown to be accompanied by the formation of oxygen ones. Chemical lattice strain caused by this cooperative disordering of cobalt and oxygen sublattices was found to be isotropic contrary to that caused by the formation of oxygen vacancies only. Cobalt deficiency was also shown to lead to lowering overall conductivity and Seebeck coefficient of EuBaCo2−xO6−δ double perovskites as a result of simultaneous decrease of charge carriers’ concentration and their mobility as well as number of sites available for electrons and holes transfer. Strong anisotropy of the overall conductivity of the single crystal double perovskites EuBaCo2−xO6−δ was found and explained on the basis of preferential location of oxygen vacancies in the rare-earth-oxygen- (REO-) planes
Synthesis, Single Crystal Growth, and Properties of Cobalt Deficient Double Perovskite EuBaCo 2− x
The cobalt deficient double perovskites EuBaCo2−xO6−δ with x=0–0.1 were obtained both as powders and as single crystal. Formation of cobalt vacancies in their crystal lattice was shown to be accompanied by the formation of oxygen ones. Chemical lattice strain caused by this cooperative disordering of cobalt and oxygen sublattices was found to be isotropic contrary to that caused by the formation of oxygen vacancies only. Cobalt deficiency was also shown to lead to lowering overall conductivity and Seebeck coefficient of EuBaCo2−xO6−δ double perovskites as a result of simultaneous decrease of charge carriers’ concentration and their mobility as well as number of sites available for electrons and holes transfer. Strong anisotropy of the overall conductivity of the single crystal double perovskites EuBaCo2−xO6−δ was found and explained on the basis of preferential location of oxygen vacancies in the rare-earth-oxygen- (REO-) planes
Dark Matter Search Perspectives with GAMMA-400
GAMMA-400 is a future high-energy gamma-ray telescope, designed to measure
the fluxes of gamma-rays and cosmic-ray electrons + positrons, which can be
produced by annihilation or decay of dark matter particles, and to survey the
celestial sphere in order to study point and extended sources of gamma-rays,
measure energy spectra of Galactic and extragalactic diffuse gamma-ray
emission, gamma-ray bursts, and gamma-ray emission from the Sun. GAMMA-400
covers the energy range from 100 MeV to ~3000 GeV. Its angular resolution is
~0.01 deg(Eg > 100 GeV), and the energy resolution ~1% (Eg > 10 GeV). GAMMA-400
is planned to be launched on the Russian space platform Navigator in 2019. The
GAMMA-400 perspectives in the search for dark matter in various scenarios are
presented in this paperComment: 4 pages, 4 figures, submitted to the Proceedings of the International
Cosmic-Ray Conference 2013, Brazil, Rio de Janeir
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