Final results of an experiment to search for 2beta processes in zinc and tungsten with the help of radiopure ZnWO4 crystal scintillators

A search for the double beta decay of zinc and tungsten isotopes has been performed with the help of radiopure ZnWO4 crystal scintillators (0.1-0.7 kg) at the Gran Sasso National Laboratories of the INFN. The total exposure of the low background measurements is 0.529 kg yr. New improved half-life limits on the double beta decay modes of 64Zn, 70Zn, 180W, and 186W have been established at the level of 10^{18}-10^{21} yr. In particular, limits on double electron capture and electron capture with positron emission in 64Zn have been set: T_{1/2}(2\nu 2K) > 1.1 10^{19} yr, T_{1/2} (0\nu 2\epsilon) > 3.2 10^{20} yr, T_{1/2} (2\nu \epsilon \beta^+) > 9.4 10^{20} yr, and T_{1/2} (0\nu \epsilon \beta^+) > 8.5 10^{20} yr, all at 90% C.L. Resonant neutrinoless double electron capture in 180W has been restricted on the level of T_{1/2} (0\nu 2\epsilon) > 1.3 10^{18} yr. A new half-life limit on alpha transition of 183W to the metastable excited level 1/2^- 375 keV of 179Hf has been established: T_{1/2} > 6.7 10^{20} yr.Comment: This is an author-created, un-copyedited version of an article published in J. Phys. G: Nucl. Part. Phys. IOP Publishing Ltd is not responsible for any errors or omissions in this version of the manuscript or any version derived from it. The definitive publisher authenticated version is available online at doi: 10.1088/0954-3899/38/11/11510

Search for long-lived superheavy eka-tungsten with radiopure ZnWO4_4 crystal scintillator

The data collected with a radioactively pure ZnWO$_4$ crystal scintillator (699 g) in low background measurements during 2130 h at the underground (3600 m w.e.) Laboratori Nazionali del Gran Sasso (INFN, Italy) were used to set a limit on possible concentration of superheavy eka-W (seaborgium Sg, Z = 106) in the crystal. Assuming that one of the daughters in a chain of decays of the initial Sg nucleus decays with emission of high energy $\alpha$ particle ($Q_\alpha > 8$ MeV) and analyzing the high energy part of the measured $\alpha$ spectrum, the limit N(Sg)/N(W) < 5.5 $\times$ 10$^{-14}$ atoms/atom at 90% C.L. was obtained (for Sg half-life of 10$^9$ yr). In addition, a limit on the concentration of eka-Bi was set by analysing the data collected with a large BGO scintillation bolometer in an experiment performed by another group [L. Cardani et al., JINST 7 (2012) P10022]: N(eka-Bi)/N(Bi) < 1.1 $\times$ 10$^{-13}$ atoms/atom with 90% C.L. Both the limits are comparable with those obtained in recent experiments which instead look for spontaneous fission of superheavy elements or use the accelerator mass spectrometry.Comment: 9 pages, 2 figures; in press on Physica Script

Investigation of rare nuclear decays with BaF2_2 crystal scintillator contaminated by radium

The radioactive contamination of a BaF$_2$ scintillation crystal with mass of 1.714 kg was measured over 101 hours in the low-background DAMA/R&D set-up deep underground (3600 m w.e.) at the Gran Sasso National Laboratories of INFN (LNGS, Italy). The half-life of $^{212}$Po (present in the crystal scintillator due to contamination by radium) was measured as $T_{1/2}(^{212}$Po) = 298.8$\pm$0.8(stat.)$\pm$1.4(syst.) ns by analysis of the events' pulse profiles. The $^{222}$Rn nuclide is known as 100% decaying via emission of $\alpha$ particle with $T_{1/2}$ = 3.82 d; however, its $\beta$ decay is also energetically allowed with $Q_\beta = 24\pm21$ keV. Search for decay chains of events with specific pulse shapes characteristic for $\alpha$ or for $\beta/\gamma$ signals and with known energies and time differences allowed us to set, for the first time, the limit on the branching ratio of $^{222}$Rn relatively to $\beta$ decay as $B_\beta < 0.13$% at 90% C.L. (equivalent to limit on partial half-life $T_{1/2}^\beta > 8.0$ y). Half-life limits of $^{212}$Pb, $^{222}$Rn and $^{226}$Ra relatively to $2\beta$ decays are also improved in comparison with the earlier results.Comment: 10 pages, 9 figures, 2 table

Rejection of randomly coinciding events in Li2_2100^{100}MoO4_4 scintillating bolometers using light detectors based on the Neganov-Luke effect

Random coincidences of nuclear events can be one of the main background sources in low-temperature calorimetric experiments looking for neutrinoless double-beta decay, especially in those searches based on scintillating bolometers embedding the promising double-beta candidate $^{100}$Mo, because of the relatively short half-life of the two-neutrino double-beta decay of this nucleus. We show in this work that randomly coinciding events of the two-neutrino double decay of $^{100}$Mo in enriched Li$_2$$^{100}$MoO$_4$ detectors can be effectively discriminated by pulse-shape analysis in the light channel if the scintillating bolometer is provided with a Neganov-Luke light detector, which can improve the signal-to-noise ratio by a large factor, assumed here at the level of $\sim 750$ on the basis of preliminary experimental results obtained with these devices. The achieved pile-up rejection efficiency results in a very low contribution, of the order of $\sim 6\times10^{-5}$ counts/(keV$\cdot$kg$\cdot$y), to the background counting rate in the region of interest for a large volume ($\sim 90$ cm$^3$) Li$_2$$^{100}$MoO$_4$ detector. This background level is very encouraging in view of a possible use of the Li$_2$$^{100}$MoO$_4$ solution for a bolometric tonne-scale next-generation experiment as that proposed in the CUPID project

Search for double beta decay of 136^{136}Ce and 138^{138}Ce with HPGe gamma detector

Search for double $\beta$ decay of $^{136}$Ce and $^{138}$Ce was realized with 732 g of deeply purified cerium oxide sample measured over 1900 h with the help of an ultra-low background HPGe $\gamma$ detector with a volume of 465 cm$^3$ at the STELLA facility of the Gran Sasso National Laboratories of the INFN (Italy). New improved half-life limits on double beta processes in the cerium isotopes were set at the level of $\lim T_{1/2}\sim 10^{17}-10^{18}$~yr; many of them are even two orders of magnitude larger than the best previous results.Comment: 21 pages, 6 figures, 3 tables; version accepted for publication on Nucl. Phys.

First test of an enriched 116^{116}CdWO4_4 scintillating bolometer for neutrinoless double-beta-decay searches

For the first time, a cadmium tungstate crystal scintillator enriched in $^{116}$Cd has been succesfully tested as a scintillating bolometer. The measurement was performed above ground at a temperature of 18 mK. The crystal mass was 34.5 g and the enrichment level ~82 %. Despite a substantial pile-up effect due to above-ground operation, the detector demonstrated a high energy resolution (2-7 keV FWHM in 0.2-2.6 MeV $\gamma$ energy range), a powerful particle identification capability and a high level of internal radiopurity. These results prove that cadmium tungstate is an extremely promising detector material for a next-generation neutrinoless double-beta decay bolometric experiment, like that proposed in the CUPID project (CUORE Upgrade with Particle IDentification)

Search for 2\beta\ decays of 96Ru and 104Ru by ultra-low background HPGe gamma spectrometry at LNGS: final results

An experiment to search for double beta decay processes in 96Ru and 104Ru, which are accompanied by gamma rays, has been realized in the underground Gran Sasso National Laboratories of the I.N.F.N. (Italy). Ruthenium samples with masses of about (0.5-0.7) kg were measured with the help of ultra-low background high purity Ge gamma ray spectrometry. After 2162 h of data taking the samples were deeply purified to reduce the internal contamination of 40K. The last part of the data has been accumulated over 5479 h. New improved half life limits on 2\beta+/\epsilon \beta+/2\epsilon\ processes in 96Ru have been established on the level of 10^{20} yr, in particular for decays to the ground state of 96Mo: T1/2(2\nu 2\beta+) > 1.4 10^{20} yr, T1/2(2\nu \epsilon\beta+) > 8.0 10^{19} yr and T1/2(0\nu 2K) > 1.0 10^{21} yr (all limits are at 90% C.L.). The resonant neutrinoless double electron captures to the 2700.2 keV and 2712.7 keV excited states of 96Mo are restricted as: T1/2(0\nu KL) > 2.0 10^{20} yr and T1/2(0\nu 2L) > 3.6 10^{20} yr, respectively. Various two neutrino and neutrinoless 2\beta\ half lives of 96Ru have been estimated in the framework of the QRPA approach. In addition, the T1/2 limit for 0\nu 2\beta- transitions of 104Ru to the first excited state of 104Pd has been set as > 6.5 10^{20} yr.Comment: 14 pages, 5 figures, 2 tables; version accepted for publication on Phys. Rev.

Radioactive contamination of ZnWO4 crystal scintillators

The radioactive contamination of ZnWO4 crystal scintillators has been measured deep underground at the Gran Sasso National Laboratory (LNGS) of the INFN in Italy with a total exposure 3197 kg x h. Monte Carlo simulation, time-amplitude and pulse-shape analyses of the data have been applied to estimate the radioactive contamination of the ZnWO4 samples. One of the ZnWO4 crystals has also been tested by ultra-low background gamma spectrometry. The radioactive contaminations of the ZnWO4 samples do not exceed 0.002 -- 0.8 mBq/kg (depending on the radionuclide), the total alpha activity is in the range: 0.2 - 2 mBq/kg. Particular radioactivity, beta active 65Zn and alpha active 180W, has been detected. The effect of the re-crystallization on the radiopurity of the ZnWO4 crystal has been studied. The radioactive contamination of samples of the ceramic details of the set-ups used in the crystals growth has been checked by low background gamma spectrometry. A project scheme on further improvement of the radiopurity level of the ZnWO4 crystal scintillators is briefly addressed.Comment: 15 pages, 8 figures, 6 tables, submitted for publicatio