Hour-glass magnetic spectrum in a stripe-less insulating transition metal oxide

An hour-glass shaped magnetic excitation spectrum appears to be an universal characteristic of the high-temperature superconducting cuprates. Fluctuating charge stripes or alternative band structure approaches are able to explain the origin of these spectra. Recently, an hour- glass spectrum has been observed in an insulating cobaltate, thus, favouring the charge stripe scenario. Here we show that neither charge stripes nor band structure effects are responsible for the hour-glass dispersion in a cobaltate within the checkerboard charge ordered regime of La2-xSrxCoO4. The search for charge stripe ordering reflections yields no evidence for charge stripes in La1.6Sr0.4CoO4 which is supported by our phonon studies. With the observation of an hour-glass-shaped excitation spectrum in this stripe-less insulating cobaltate, we provide experimental evidence that the hour-glass spectrum is neither necessarily connected to charge stripes nor to band structure effects, but instead, probably intimately coupled to frustration and arising chiral or non-collinear magnetic correlations

Impact of high solar zenith angles on dynamical and chemical processes in a coupled chemistry-climate model

International audienceActinic fluxes at high solar zenith angles (SZAs) are important for atmospheric chemistry, especially under twilight conditions in polar winter and spring. The results of a sensitivity experiment employing the fully coupled 3D chemistry-climate model ECHAM4.L39(DLR)/CHEM have been analysed to quantify the impact of SZAs greater than 87.5° on dynamical and chemical processes in the lower stratosphere, in particular their influence on the ozone layer. Although the actinic fluxes at SZAs larger than 87.5° are small, ozone concentrations are significantly affected because daytime photolytic ozone destruction is switched on earlier, especially the conversion of Cl2 and Cl2O2 into ClO at the end of polar night in the lower stratosphere. Comparing climatological mean ozone column values of a simulation considering SZAs up to 93° with those of the sensitivity run with SZAs confined to 87.5° total ozone is reduced by about 20% in the polar Southern Hemisphere, i.e., the ozone hole is "deeper'' if twilight conditions are considered in the model because there is 2?3 weeks more time for ozone destruction. This causes an additional cooling of the polar lower stratosphere (50 hPa) up to ?4 K with obvious consequences for chemical processes. In the Northern Hemisphere the impact of high SZAs cannot be determined on the basis of climatological mean values due to the pronounced dynamic variability of the stratosphere in winter and spring

Incommensurate antiferromagnetic fluctuations in single-crystalline LiFeAs studied by inelastic neutron scattering

We present an inelastic neutron scattering study on single-crystalline LiFeAs devoted to the characterization of the incommensurate antiferromagnetic fluctuations at $\mathbf{Q}=(0.5\pm\delta, 0.5\mp\delta, q_l)$. Time-of-flight measurements show the presence of these magnetic fluctuations up to an energy transfer of 60 meV, while polarized neutrons in combination with longitudinal polarization analysis on a triple-axis spectrometer prove the pure magnetic origin of this signal. The normalization of the magnetic scattering to an absolute scale yields that magnetic fluctuations in LiFeAs are by a factor eight weaker than the resonance signal in nearly optimally Co-doped BaFe$_2$As$_2$, although a factor two is recovered due to the split peaks owing to the incommensurability. The longitudinal polarization analysis indicates weak spin space anisotropy with slightly stronger out-of-plane component between 6 and 12 meV. Furthermore, our data suggest a fine structure of the magnetic signal most likely arising from superposing nesting vectors.Comment: 9 pages, 8 figure

Magnetic Blue Phase in the Chiral Itinerant Magnet MnSi

Chiral nematic liquid crystals sometimes form blue phases characterized by spirals twisting in different directions. By combining model calculations with neutron-scattering experiments, we show that the magnetic analogue of blue phases does form in the chiral itinerant magnet MnSi in a large part of the phase diagram. The properties of this blue phase explain a number of previously reported puzzling features of MnSi such as partial magnetic order and a two-component specific-heat and thermal-expansion anomaly at the magnetic transition