40,644 research outputs found

    Competing Ground States in Triple-layered Sr4Ru3O10: Verging on Itinerant Ferromagnetism with Critical Fluctuations

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    Sr4Ru3O10 is characterized by a sharp metamagnetic transition and ferromagnetic behavior occurring within the basal plane and along the c-axis, respectively. Resistivity at magnetic field, B, exhibits low-frequency quantum oscillations when B||c-axis and large magnetoresistivity accompanied by critical fluctuations driven by the metamagnetism when B^c-axis. The complex behavior evidenced in resistivity, magnetization and specific heat presented is not characteristic of any obvious ground states, and points to an exotic state that shows a delicate balance between fluctuations and order.Comment: 18 pages, 4 figure

    Suppression of magnetism in Ba5AlIr2O11: interplay of Hund's coupling, molecular orbitals and spin-orbit interaction

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    The electronic and magnetic properties of Ba5_5AlIr2_2O11_{11} containing Ir-Ir dimers are investigated using the GGA and GGA+SOC calculations. We found that strong suppression of the magnetic moment in this compound recently found in [J. Terzic {\it et al.}, Phys. Rev. B {\bf 91}, 235147 (2015)] is not due to charge-ordering, but is related to the joint effect of the spin-orbit interaction and strong covalency, resulting in the formation of metal-metal bonds. They conspire and act against the intra-atomic Hund's rule exchange interaction to reduce total magnetic moment of the dimer. We argue that the same mechanism could be relevant for other 4d4d and 5d5d dimerized transition metal compounds

    Fluence dependent femtosecond quasi-particle and Eu^{2+} -spin relaxation dynamics in EuFe_{2}(As,P)_{2}

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    We investigated temperature and fluence dependent dynamics of the time resolved optical reflectivity in undoped spin-density-wave (SDW) and doped superconducting (SC) EuFe2_{2}(As,P)2_{2} with emphasis on the ordered Eu2+^{2+}-spin temperature region. The data indicate that the SDW order coexists at low temperature with the SC and Eu2+^{2+}-ferromagnetic order. Increasing the excitation fluence leads to a thermal suppression of the Eu2+^{2+}-spin order due to the crystal-lattice heating while the SDW order is suppressed nonthermally at a higher fluence

    First-principles study of multiferroic RbFe(MoO4_4)2_2

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    We have investigated the magnetic structure and ferroelectricity in RbFe(MoO4_4)2_2 via first-principles calculations. Phenomenological analyses have shown that ferroelectricity may arise due to both the triangular chirality of the magnetic structure, and through coupling between the magnetic helicity and the ferroaxial structural distortion. Indeed, it was recently proposed that the structural distortion plays a key role in stabilising the chiral magnetic structure itself. We have determined the relative contribution of the two mechanisms via \emph{ab-initio} calculations. Whilst the structural axiality does induce the magnetic helix by modulating the symmetric exchange interactions, the electric polarization is largely due to the in-plane spin triangular chirality, with both electronic and ionic contributions being of relativistic origin. At the microscopic level, we interpret the polarization as a secondary steric consequence of the inverse Dzyaloshinskii-Moriya mechanism and accordingly explain why the ferroaxial component of the electric polarization must be small
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