300 research outputs found
Mott transition in Cr-doped V2O3 studied by ultrafast reflectivity: electron correlation effects on the transient response
The ultrafast response of the prototype Mott-Hubbard system (V1-xCrx)2O3 was
systematically studied with fs pump-probe reflectivity, allowing us to clearly
identify the effects of the metal-insulator transition on the transient
response. The isostructural nature of the phase transition in this material
made it possible to follow across the phase diagram the behaviour of the
detected coherent acoustic wave, whose average value and lifetime depend on the
thermodynamic phase and on the correlated electron density of states. It is
also shown how coherent lattice oscillations can play an important role in some
changes affecting the ultrafast electronic peak relaxation at the phase
transition, changes which should not be mistakenly attributed to genuine
electronic effects. These results clearly show that a thorough understanding of
the ultrafast response of the material over several tenths of ps is necessary
to correctly interpret its sub-ps excitation and relaxation regime, and appear
to be of general interest also for other strongly correlated materials.Comment: 6 pages, 3 figures. Europhysics Letters (in press
Observation of longitudinal and transverse self-injections in laser-plasma accelerators
Laser-plasma accelerators can produce high quality electron beams, up to
giga-electronvolts in energy, from a centimeter scale device. The properties of
the electron beams and the accelerator stability are largely determined by the
injection stage of electrons into the accelerator. The simplest mechanism of
injection is self-injection, in which the wakefield is strong enough to trap
cold plasma electrons into the laser wake. The main drawback of this method is
its lack of shot-to-shot stability. Here we present experimental and numerical
results that demonstrate the existence of two different self-injection
mechanisms. Transverse self-injection is shown to lead to low stability and
poor quality electron beams, because of a strong dependence on the intensity
profile of the laser pulse. In contrast, longitudinal injection, which is
unambiguously observed for the first time, is shown to lead to much more stable
acceleration and higher quality electron beams.Comment: 7 pages, 7 figure
Superadiabatic transitions in quantum molecular dynamics
We study the dynamics of a molecule’s nuclear wave function near an avoided crossing of two electronic energy levels for one nuclear degree of freedom. We derive the general form of the Schrödinger equation in the nth superadiabatic representation for all n є N. Using these results, we obtain closed formulas for the time development of the component of the wave function in an initially unoccupied energy subspace when a wave packet travels through the transition region. In the optimal superadiabatic representation, which we define, this component builds up monotonically. Finally, we give an explicit formula for the transition wave function away from the avoided crossing, which is in excellent agreement with high-precision numerical calculations
Facultative Hyperparasitism: Extreme Survival Behaviour of the Primary Solitary Ectoparasitoid, Dinarmus basalis
This study investigated the egg-laying behaviour of ectoparsitoid, Dinarmus basalis Rondani (Hymenoptera: Pteromalidae), females when faced with a prolonged deprivation of suitable hosts leading to extreme ‘oviposition pressure’. The egg-laying behaviour of virgin D. basalis females was tested with Callosobruchus maculatus (F.) (Coleoptera: Bruchidae) hosts previously parasitized by the conspecific females in which the developing larvae had reached the last larval instar (L5) or pupae. The hyperparasitism did not prevent the occurrence of superparasitism, but only one D. basalis egg from a hyperparasitized D. basalis L5 larvae reached the adult stage due to the solitary behaviour of the D. basalis larvae. Under these experimental conditions, 60.78% of the D. basalis adults emerging from larvae were miniaturized due to the depletion of host resources
Laser based synchrotron radiation
Beams of x rays in the kiloelectronvolt energy range have been produced from laser-matter interaction. Here, energetic electrons are accelerated by a laser wakefield, and experience betatron oscillations in an ion channel formed in the wake of the intense femtosecond laser pulse. Experiments using a 50 TW laser (30 fs duration) are described, as well as comparisons with numerical simulations. These results pave the way of a new generation of radiation in the x-ray spectral range, with a high collimation and an ultrafast pulse duration, produced by the use of compact laser system.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/87767/2/023101_1.pd
Mapping the X-Ray Emission Region in a Laser-Plasma Accelerator
The x-ray emission in laser-plasma accelerators can be a powerful tool to
understand the physics of relativistic laser-plasma interaction. It is shown
here that the mapping of betatron x-ray radiation can be obtained from the
x-ray beam profile when an aperture mask is positioned just beyond the end of
the emission region. The influence of the plasma density on the position and
the longitudinal profile of the x-ray emission is investigated and compared to
particle-in-cell simulations. The measurement of the x-ray emission position
and length provides insight on the dynamics of the interaction, including the
electron self-injection region, possible multiple injection, and the role of
the electron beam driven wakefield.Comment: 5 pages, 4 figure
Electron localization and possible phase separation in the absence of a charge density wave in single-phase 1T-VS
We report on a systematic study of the structural, magnetic and transport
properties of high-purity 1T-VS powder samples prepared under high
pressure. The results differ notably from those previously obtained by
de-intercalating Li from LiVS. First, no Charge Density Wave (CDW) is found
by transmission electron microscopy down to 94 K. Though, \textit{ab initio}
phonon calculations unveil a latent CDW instability driven by an acoustic
phonon softening at the wave vector (0.21,0.21,0)
previously reported in de-intercalated samples. A further indication of latent
lattice instability is given by an anomalous expansion of the V-S bond distance
at low temperature. Second, infrared optical absorption and electrical
resistivity measurements give evidence of non metallic properties, consistent
with the observation of no CDW phase. On the other hand, magnetic
susceptibility and NMR data suggest the coexistence of localized moments with
metallic carriers, in agreement with \textit{ab initio} band structure
calculations. This discrepancy is reconciled by a picture of electron
localization induced by disorder or electronic correlations leading to a phase
separation of metallic and non-metallic domains in the nm scale. We conclude
that 1T-VS is at the verge of a CDW transition and suggest that residual
electronic doping in Li de-intercalated samples stabilizes a uniform CDW phase
with metallic properties.Comment: 22 pages, 10 Figures. Full resolution pictures available at
http://journals.aps.org/prb/abstract/10.1103/PhysRevB.89.23512
Enhanced He-alpha emission from "smoked" Ti targets irradiated with 400nm, 45 fs laser pulses
We present a study of He-like 1s(2)-1s2p line emission from solid and low-density Ti targets under similar or equal to 45 fs laser pulse irradiation with a frequency doubled Ti: Sapphire laser. By varying the beam spot, the intensity on target was varied from 10(15) W/cm(2) to 10(19) W/cm(2). At best focus, low density "smoked" Ti targets yield similar to 20 times more He-alpha than the foil targets when irradiated at an angle of 45 degrees with s-polarized pulses. The duration of He-alpha emission from smoked targets, measured with a fast streak camera, was similar to that from Ti foils
Phase Separation in LiFePO Induced by Correlation Effects
We report on a significant failure of LDA and GGA to reproduce the phase
stability and thermodynamics of mixed-valence LiFePO compounds.
Experimentally, LiFePO compositions () are known to be
unstable and phase separate into Li FePO and FePO. However,
first-principles calculations with LDA/GGA yield energetically favorable
intermediate compounds an d hence no phase separation. This qualitative failure
of LDA/GGA seems to have its origin in the LDA/GGA self-interaction which de
localizes charge over the mixed-valence Fe ions, and is corrected by explicitly
considering correlation effects in this material. This is demonstrated with
LDA+U calculations which correctly predict phase separation in LiFePO
for eV. T he origin of the destabilization of intermediate
compounds is identified as electron localization and charge ordering at
different iron sites. Introduction of correlation also yields more accurate
electrochemical reaction energies between FePO/LiFePO and
Li/Li electrodes.Comment: 12 pages, 5 figures, Phys. Rev. B 201101R, 200
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