Magnetic properties of the double perovskites LaPbMSbO6 (M = Mn, Co and Ni)

New double perovskites LaPbMSbO6, where M2+ = Mn2+, Co2+, and Ni2+, were synthesized as polycrystals by an aqueous synthetic route at temperatures below 1000 oC. All samples are monoclinic, space group P21/n, as obtained from Rietveld analysis of X-ray powder diffraction patterns. The distribution of M2+ and Sb5+ among the two octahedral sites have 3% of disorder for M2+ = Ni2+, whereas for M2+ = Mn2+ and Co2+ less disorder is found. The three samples have an antiferromagnetic transition, due to the antiferromagnetic coupling between M2+ through super-superexchange paths M2+ - O2- - Sb5+ - O2- - M2+. Transition temperatures are low: 8, 10 and 17 K for Mn2+, Co2+, and Ni2+ respectively, as a consequence of the relatively long distances between the magnetic ions M2+. Besides, for LaPbMnSbO6 a small transition at 45 K was found, with ferrimagnetic characteristics, possibly as a consequence of a small disorder between Mn2+ and Sb5+. This disorder would give additional and shorter interaction paths: superexchange Mn2+ - O2- - Mn2+.Comment: 4 pages, 4 figures included. Manuscript submitted to IEEE Transactions on Magnetics, proceedings of the LAW3M 2013 conferenc

Tailoring the ground state of the ferrimagnet La2Ni(Ni1/3Sb2/3)O6

We report on the magnetic and structural properties of La2Ni(Ni1/3Sb2/3)O6 in polycrystal, single crystal and thin film samples. We found that this material is a ferrimagnet (Tc ~ 100 K) which possesses a very distinctive and uncommon feature in its virgin curve of the hysteresis loops. We observe that bellow 20 K it lies outside the hysteresis cycle, and this feature was found to be an indication of a microscopically irreversible process possibly involving the interplay of competing antiferromagnetic interactions that hinder the initial movement of domain walls. This initial magnetic state is overcome by applying a temperature dependent characteristic field. Above this field, an isothermal magnetic demagnetization of the samples yield a ground state different from the initial thermally demagnetized one.Comment: 21 pages, 8 figures, submitted to JMM

NLTE spectroscopic analysis of the 3^3He anomaly in subluminous B-type stars

Several B-type main-sequence stars show chemical peculiarities. A particularly striking class are the $^3$He stars, which exhibit a remarkable enrichment of $^3$He with respect to $^4$He. This isotopic anomaly has also been found in blue horizontal branch (BHB) and subdwarf B (sdB) stars, which are helium-core burning stars of the extreme horizontal branch. Using a hybrid local/non-local thermodynamic equilibrium (LTE/NLTE) approach for B-type stars, we analyzed high-quality spectra of two known $^3$He BHBs and nine known $^3$He sdBs to determine their isotopic helium abundances and $^4$He/$^3$He abundance ratios. We redetermined their atmospheric parameters and analyzed selected neutral helium lines, including $\lambda$4922 $\mathring{A}$ and $\lambda$6678 $\mathring{A}$, which are very sensitive to $^4$He/$^3$He. Most of the $^3$He sdBs cluster in a narrow temperature strip between 26000 K and 30000 K and are helium deficient in accordance with previous LTE analyses. BD+48$^\circ$ 2721 is reclassified as a BHB star because of its low temperature ($T_{\mathrm{eff}}=$ 20700 K). Whereas $^4$He is almost absent ($^4$He/$^3$He$<$ 0.25) in most of the known $^3$He stars, other sample stars show abundance ratios up to $^4$He/$^3$He$=$2.51. A search for $^3$He stars in the ESO SPY survey led to the discovery of two new $^3$He sdB stars (HE 0929-0424 and HE 1047-0436). The observed helium line profiles of all BHBs and of three sdBs are not matched by chemically homogeneous atmospheres, but hint at vertical helium stratification. This phenomenon has been seen in other peculiar B-type stars, but is found for the first time for sdBs. We estimate helium to increase from the outer to the inner atmosphere by factors ranging from 1.4 (SB 290) up to 8.0 (BD+48$^\circ$ 2721).Comment: 19 pages, 79 figures submitted to Astronomy&Astrophysic

Normal state magnetotransport properties of β\beta-FeSe superconductors

We present $\beta$-FeSe magnetotransport data, and describe them theoretically. Using a simplified microscopic model with two correlated effective orbitals, we determined the normal state electrical conductivity and Hall coefficient, using Kubo formalism. With model parameters relevant for Fe-chalcogenides, we describe the observed effect of the structural transition on the ab-plane electrical resistivity, as well as on the magnetoresistance. Temperature-dependent Hall coefficient data were measured at 16 Tesla, and their theoretical description improves upon inclusion of moderate electron correlations. We confirm the effect of the structural transition on the electronic structure, finding deformation-induced band splittings comparable to those reported in angle-resolved photoemission.Comment: 6 pages, 5 figure

C II abundances in early-type stars: solution to a notorious non-LTE problem

We address a long-standing discrepancy between non-LTE analyses of the prominent C II 4267 and 6578/82 A multiplets in early-type stars. A comprehensive non-LTE model atom of C II is constructed based on critically selected atomic data. This model atom is used for an abundance study of six apparently slow-rotating main-sequence and giant early B-type stars. High-resolution and high-S/N spectra allow us to derive highly consistent abundances not only from the classical features but also from up to 18 further C II lines in the visual - including two so far unreported emission features equally well reproduced in non-LTE. These results require the stellar atmospheric parameters to be determined with care. A homogeneous (slightly) sub-solar present-day carbon abundance from young stars in the solar vicinity (in associations and in the field) of log C/H +12= 8.29+/-0.03 is indicated.Comment: 8 pages, 5 figure

Creating and Probing Electron Whispering Gallery Modes in Graphene

Designing high-finesse resonant cavities for electronic waves faces challenges due to short electron coherence lengths in solids. Previous approaches, e.g. the seminal nanometer-sized quantum corrals, depend on careful positioning of adatoms at clean surfaces. Here we demonstrate an entirely different approach, inspired by the peculiar acoustic phenomena in whispering galleries. Taking advantage of graphene's unique properties, namely gate-tunable light-like carriers, we create Whispering Gallery Mode (WGM) resonators defined by circular pn-junctions, induced by a scanning tunneling probe. We can tune the resonator size and the carrier concentration under the probe in a back-gated graphene device over a wide range, independently and in situ. The confined modes, revealed through characteristic resonances in the tunneling spectrum, originate from Klein scattering at pn junction boundaries. The WGM-type confinement and resonances are a new addition to the quantum electron-optics toolbox, paving the way to real-world electronic lenses and resonators

Inhomogeneous ferrimagnetic-like behavior in Gd2/3Ca1/3MnO3 single crystals

We present a study of the magnetic properties of Gd2/3Ca1/3MnO3 single crystals at low temperatures. We show that this material behave as an inhomogeneous ferrimagnet. In addition to small saturation magnetization at 5 K, we have found history dependent effects in the magnetization and the presence of exchange bias. These features are compatible with microscopic phase separation in the clean Gd2/3Ca1/3MnO3 system studied.Comment: 7 pages, 6 figures, submitted Journal of Magnetism and Magnetic Material

Magnetic field geometry and chemical abundance distribution of the He-strong star CPD -57 3509

The magnetic field of CPD -57 3509 was recently detected in the framework of the BOB (B fields in OB stars) collaboration. We acquired low-resolution spectropolarimetric observations of CPD -57 3509 with FORS2 and high-resolution UVES observations randomly distributed over a few months to search for periodicity, to study the magnetic field geometry, and to determine the surface distribution of silicon and helium. We also obtained supplementary photometric observations at a timeline similar to the spectroscopic and spectropolarimetric observations. A period of 6.36d was detected in the measurements of the mean longitudinal magnetic field. A sinusoidal fit to our measurements allowed us to constrain the magnetic field geometry and estimate the dipole strength in the range of 3.9-4.5kG. Our application of the Doppler imaging technique revealed the presence of He I spots located around the magnetic poles, with a strong concentration at the positive pole and a weaker one around the negative pole. In contrast, high concentration Si III spots are located close to the magnetic equator. Further, our analysis of the spectral variability of CPD -57 3509 on short time scales indicates distinct changes in shape and position of line profiles possibly caused by the presence of beta Cep-like pulsations. A small periodic variability in line with the changes of the magnetic field strength is clearly seen in the photometric data.Comment: 11 pages, 5 tables, 7 figures, accepted for publication in MNRA

Role of twin boundaries on the vortex dynamics in YBa2_2Cu3_3O7_7

By means of a novel technique of rotating the applied current we have directly measured the influence of twin boundaries on the vortex motion in a YBa$_2$Cu$_3$O$_7$ single crystal. The results indicate that the effect of twin planes on the vortex dynamics starts to develop below a certain temperature, being responsible for an anisotropic viscosity in the vortex liquid state and a guided motion in the solid state.Comment: 4 pages, 4 figure