3,162 research outputs found
Hidden quantum phase transition in MnFeGe: evidence brought by small-angle neutron scattering
The magnetic system of the MnFeGe solid solution is ordered in
a spiral spin structure in the whole concentration range of .
The close inspection of the small-angle neutron scattering data reveals the
quantum phase transition from the long-range ordered (LRO) to short range
ordered (SRO) helical structure upon increase of Fe-concentration at . The SRO of the helical structure is identified as a
Lorentzian contribution, while LRO is associated with the Gaussian contribution
into the scattering profile function. The scenario of the quantum phase
transition with as a driving parameter is similar to the thermal phase
transition in pure MnGe. The quantum nature of the SRO is proved by the
temperature independent correlation length of the helical structure at low and
intermediate temperature ranges with remarkable decrease above certain
temperature . We suggest the -dependent modification of the effective
Ruderman-Kittel-Kasuya-Yosida exchange interaction within the Heisenberg model
of magnetism to explain the quantum critical regime in MnFeGe.Comment: 6 pages, 4 figure
Structure and dynamics of the 4p -\u3e ns,md autoionizing resonances between the P-3 and S-1 thresholds in atomic bromine
The relative partial photoionization cross sections sigma(i) and photoelectron angular distribution parameters beta(1) are measured for all possible final ionic states of Br+ between the P-3(2) and S-1(0) thresholds. The decay patterns of the autoionizing 4p(4 3)P(1,0) nl, 4p(4 1)D(2) nl, and 4p(4 1)S(0) nl Rydberg series arising from the 4p ins,md excitations are observed at the fine-structure level in all available channels. For each Rydberg series, the energies, quantum defects, and photoelectron angular distribution parameters are determined, as well as the widths and shape parameters of the low-lying members. Relative total cross sections are derived from the partial cross sections and from ion-yield measurements over the lowest members of the P-3(1,0) and D-1(2) series. All major spectroscopic and dynamic properties of these series are reported for this open-shell atom. Conclusions are drawn from the comprehensive data sets in comparison with other halogen atoms and the neighboring closed-shell rare gas atoms. Our results, encompassing the entire autoionization regime, are compared with other experimental data and theoretical calculations, where available
Multipole nonlinearity of metamaterials
We report on the linear and nonlinear optical response of metamaterials
evoked by first and second order multipoles. The analytical ground on which our
approach bases permits for new insights into the functionality of
metamaterials. For the sake of clarity we focus here on a key geometry, namely
the split-ring resonator, although the introduced formalism can be applied to
arbitrary structures. We derive the equations that describe linear and
nonlinear light propagation where special emphasis is put on second harmonic
generation. This contribution basically aims at stretching versatile and
existing concepts to describe light propagation in nonlinear media towards the
realm of metamaterials.Comment: 7 pages, 3 figure
Mössbauer and magnetic study of Co x Fe3−x O4 nanoparticles
Magnetic nanoparticles of cobalt ferrites Co x Fe3−x O4 (x = 1 or 2) have been obtained either by mechanical milling or thermal treatment of pre-prepared layered double hydroxide carbonate x-LDH–CO3. Mechanical milling of the 1-LDH–CO3 leads to the large-scale preparation of nearly spherical nanoparticles of CoFe2O4, the size of which (5 to 20 nm) is controlled by the treatment time. Core-shell structure with surface spin-canting has been considered for the nanoparticles formed to explain the observed hysteresis loop shift (from ZFC–FC) in the magnetic properties. Annealing treatment of the 2-LDH–CO3 below 673 K results in the formation of nearly spherical pure Co2FeO4 nanoparticles. At 673 K and above, the LDH decomposition leads to the formation of a mixture of both spinels phases Co2FeO4 and CoFe2O4, the amount of the latter increases with annealing temperature. Unusually high magnetic hardness characterized by a 22 kOe coercive field at 1.8 K has been observed, which reflects the high intrinsic anisotropy for Co2FeO4
Natural Widths In Open-Shell Atoms: The K Absorption Spectrum Of Atomic Oxygen
Total-ion-yield measurements and Hartree-Fock calculations are presented for the 1s-- \u3enp, n=2 to 5 photoexcitations in atomic oxygen. Energies and relative intensities of the [1s]2s(2)2p(4)(P-4)np and [1s]2s(2)2p(4)(P-2)np series members are determined, and the apparent linewidths are measured. It is shown that natural widths in an open-shell atom can be deduced from an absorption spectrum only with the aid of theoretical input. The linewidth for the six individual components contained in the 1s--\u3e2p transition is determined to be 140(9) meV
Partial Photoionization Cross Sections And Photoelectron Angular Distributions For Double Excitations Up To The N=5 Threshold In Helium
Partial photoionization cross sections sigma(n) and photoelectron angular distributions beta(n) were measured for all possible final ionic states He+(n) in the region of the double excitations N(K,T)(A) up to the N=5 threshold. At a photon energy bandpass of 12 meV below the thresholds N=3,4, and 5, this level of differentiation offers the most critical assessment of the dynamics of the two-electron excitations to date. The experimental data are very well described by the most advanced theoretical calculations. Weaker double-excitation series with K=N-4 are clearly visible in the beta(n) data, and even previously unobserved extremely weak series members with A=-1 can be discerned, showing the high sensitivity of the angular resolved measurements. The shapes of the resonance-induced variations of sigma(n) or beta(n) in the double excitations below a given threshold N change radically depending on the final ionic state n but display striking similarities when comparing the satellite states with n=N-1 and n=N-2 below each threshold N. These systematic patterns may indicate a general rule for the underlying two-electron dynamics
Response of neutron detectors to high-energy mixed radiation fields
Radiation protection around CERN's high-energy accelerators represents a major challenge due to the presence of complex, mixed radiation fields. Behind thick shielding neutrons dominate and their energy ranges from fractions of eV to about 1 GeV. In this work the response of various portable detectors sensitive to neutrons was studied at CERN's High-Energy Reference Field Facility (CERF). The measurements were carried out with conventional rem counters, which usually cover neutron energies up to 20 MeV, the Thermo WENDI-2, which is specified to measure neutrons up to several GeV, and a tissue-equivalent proportional counter. The experimentally determined neutron dose equivalent results were compared with Monte Carlo (MC) simulations. Based on these studies field calibration factors can be determined, which result in a more reliable estimate of H*(10) in an unknown, but presumably similar high-energy field around an accelerator than a calibration factor determined in a radiation field of a reference neutron sourc
Intermanifold similarities in partial photoionization cross sections of helium
Using the eigenchannel R-matrix method we calculate partial photoionization
cross sections from the ground state of the helium atom for incident photon
energies up to the N=9 manifold. The wide energy range covered by our
calculations permits a thorough investigation of general patterns in the cross
sections which were first discussed by Menzel and co-workers [Phys. Rev. A {\bf
54}, 2080 (1996)]. The existence of these patterns can easily be understood in
terms of propensity rules for autoionization. As the photon energy is increased
the regular patterns are locally interrupted by perturber states until they
fade out indicating the progressive break-down of the propensity rules and the
underlying approximate quantum numbers. We demonstrate that the destructive
influence of isolated perturbers can be compensated with an energy-dependent
quantum defect.Comment: 10 pages, 10 figures, replacement with some typos correcte
Metastable precursors during the oxidation of the Ru(0001) surface
Using density-functional theory, we predict that the oxidation of the
Ru(0001) surface proceeds via the accumulation of sub-surface oxygen in
two-dimensional islands between the first and second substrate layer. This
leads locally to a decoupling of an O-Ru-O trilayer from the underlying metal.
Continued oxidation results in the formation and stacking of more of these
trilayers, which unfold into the RuO_2(110) rutile structure once a critical
film thickness is exceeded. Along this oxidation pathway, we identify various
metastable configurations. These are found to be rather close in energy,
indicating a likely lively dynamics between them at elevated temperatures,
which will affect the surface chemical and mechanical properties of the
material.Comment: 11 pages including 9 figures. Submitted to Phys. Rev. B. Related
publications can be found at http://www.fhi-berlin.mpg.de/th/paper.htm
Diagonalization of replicated transfer matrices for disordered Ising spin systems
We present an alternative procedure for solving the eigenvalue problem of
replicated transfer matrices describing disordered spin systems with (random)
1D nearest neighbor bonds and/or random fields, possibly in combination with
(random) long range bonds. Our method is based on transforming the original
eigenvalue problem for a matrix (where ) into an
eigenvalue problem for integral operators. We first develop our formalism for
the Ising chain with random bonds and fields, where we recover known results.
We then apply our methods to models of spins which interact simultaneously via
a one-dimensional ring and via more complex long-range connectivity structures,
e.g. dimensional neural networks and `small world' magnets.
Numerical simulations confirm our predictions satisfactorily.Comment: 24 pages, LaTex, IOP macro
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