189 research outputs found
Energy boost in laser wakefield accelerators using sharp density transitions
The energy gain in laser wakefield accelerators is limited by dephasing
between the driving laser pulse and the highly relativistic electrons in its
wake. Since this phase depends on both the driver and the cavity length, the
effects of dephasing can be mitigated with appropriate tailoring of the plasma
density along propagation. Preceding studies have discussed the prospects of
continuous phase-locking in the linear wakefield regime. However, most
experiments are performed in the highly non-linear regime and rely on
self-guiding of the laser pulse. Due to the complexity of the driver evolution
in this regime it is much more difficult to achieve phase locking. As an
alternative we study the scenario of rapid rephasing in sharp density
transitions, as was recently demonstrated experimentally. Starting from a
phenomenological model we deduce expressions for the electron energy gain in
such density profiles. The results are in accordance with particle-in-cell
simulations and we present gain estimations for single and multiple stages of
rephasing
3D printing of gas jet nozzles for laser-plasma accelerators
Recent results on laser wakefield acceleration in tailored plasma channels
have underlined the importance of controlling the density profile of the gas
target. In particular it was reported that appropriate density tailoring can
result in improved injection, acceleration and collimation of laser-accelerated
electron beams. To achieve such profiles innovative target designs are
required. For this purpose we have reviewed the usage of additive layer
manufacturing, commonly known as 3D printing, in order to produce gas jet
nozzles. Notably we have compared the performance of two industry standard
techniques, namely selective laser sintering (SLS) and stereolithography (SLA).
Furthermore we have used the common fused deposition modeling (FDM) to
reproduce basic gas jet designs and used SLA and SLS for more sophisticated
nozzle designs. The nozzles are characterized interferometrically and used for
electron acceleration experiments with the Salle Jaune terawatt laser at
Laboratoire d'Optique Appliqu\'ee
All-optical Compton scattering at shallow interaction angles
All-optical Compton sources combine laser-wakefield accelerators and intense scattering pulses to generate ultrashort bursts of backscattered radiation. The scattering pulse plays the role of a small-period undulator (∼1μm) in which relativistic electrons oscillate and emit X-ray radiation. To date, most of the working laser-plasma accelerators operate preferably at energies of a few hundreds of megaelectronvolts and the Compton sources developed so far produce radiation in the range from hundreds of kiloelectronvolts to a few megaelectronvolts. However, for such applications as medical imaging and tomography the relevant energy range is 10–100 keV. In this article, we discuss different scattering geometries for the generation of X-rays in this range. Through numerical simulations, we study the influence of electron beam parameters on the backscattered photons. We find that the spectral bandwidth remains constant for beams of the same emittance regardless of the scattering geometry. A shallow interaction angle of 30∘ or less seems particularly promising for imaging applications given parameters of existing laser-plasma accelerators. Finally, we discuss the influence of the radiation properties for potential applications in medical imaging and non-destructive testing
Quick X-ray microtomography using a laser-driven betatron source
Laser-driven X-ray sources are an emerging alternative to conventional X-ray
tubes and synchrotron sources. We present results on microtomographic X-ray
imaging of a cancellous human bone sample using synchrotron-like betatron
radiation. The source is driven by a 100-TW-class titanium-sapphire laser
system and delivers over X-ray photons per second. Compared to earlier
studies, the acquisition time for an entire tomographic dataset has been
reduced by more than an order of magnitude. Additionally, the reconstruction
quality benefits from the use of statistical iterative reconstruction
techniques. Depending on the desired resolution, tomographies are thereby
acquired within minutes, which is an important milestone towards real-life
applications of laser-plasma X-ray sources
A bremsstrahlung gamma-ray source based on stable ionization injection of electrons into a laser wakefield accelerator
Laser wakefield acceleration permits the generation of ultra-short,
high-brightness relativistic electron beams on a millimeter scale. While those
features are of interest for many applications, the source remains constraint
by the poor stability of the electron injection process. Here we present
results on injection and acceleration of electrons in pure nitrogen and argon.
We observe stable, continuous ionization-induced injection of electrons into
the wakefield for laser powers exceeding a threshold of 7 TW. The beam charge
scales approximately linear with the laser energy and is limited by beam
loading. For 40 TW laser pulses we measure a maximum charge of almost 1 nC per
shot, originating mostly from electrons of less than 10 MeV energy. The
relatively low energy, the high charge and its stability make this source
well-suited for applications such as non-destructive testing. Hence, we
demonstrate the production of energetic radiation via bremsstrahlung conversion
at 1 Hz repetition rate. In accordance with Geant4 Monte-Carlo simulations, we
measure a gamma-ray source size of less than 100 microns for a 0.5 mm tantalum
converter placed at 2 mm from the accelerator exit. Furthermore we present
radiographs of image quality indicators
Pareto Optimization of a Laser Wakefield Accelerator
Optimization of accelerator performance parameters is limited by numerous
trade-offs and finding the appropriate balance between optimization goals for
an unknown system is challenging to achieve. Here we show that multi-objective
Bayesian optimization can map the solution space of a laser wakefield
accelerator in a very sample-efficient way. Using a Gaussian mixture model, we
isolate contributions related to an electron bunch at a certain energy and we
observe that there exists a wide range of Pareto-optimal solutions that trade
beam energy versus charge at similar laser-to-beam efficiency. However, many
applications such as light sources require particle beams at a certain target
energy. Once such a constraint is introduced we observe a direct trade-off
between energy spread and accelerator efficiency. We furthermore demonstrate
how specific solutions can be exploited using \emph{a posteriori} scalarization
of the objectives, thereby efficiently splitting the exploration and
exploitation phases
Study of electron acceleration and X-ray radiation as a function of plasma density in capillary-guided laser wakefield accelerators
Laser wakefield electron acceleration in the blow-out regime and the associated betatron X-rayradiation were investigated experimentally as a function of the plasma density in a configuration where the laser is guided. Dielectric capillary tubes were employed to assist the laser keeping self-focused over a long distance by collecting the laser energy around its central focal spot. With a 40 fs, 16 TW pulsed laser, electron bunches with tens of pC charge were measured to be accelerated to an energy up to 300 MeV, accompanied by X-ray emission with a peak brightness of the order of 10 21 ph/s/mm 2 / mrad 2 /0.1%BW. Electron trapping and acceleration were studied using the emitted X-ray beamdistribution to map the acceleration process; the number of betatron oscillations performed by theelectrons was inferred from the correlation between measured X-ray fluence and beam charge. A studyof the stability of electron and X-ray generation suggests that the fluctuation of X-ray emission can be reduced by stabilizing the beam charge. The experimental results are in good agreement with 3D particle-in-cell (PIC) simulation.Fil: Ju, L.. Universite de Paris Xi; Francia;Fil: Svensson, K.. Lund University; SueciaFil: Ferrari, Hugo Emilio. Comisión Nacional de EnergÃa Atómica. Gerencia del Area de Investigación y Aplicaciones No Nucleares. Gerencia de FÃsica (centro Atómico Bariloche); Argentina. Consejo Nacional de Investigaciones CientÃficas y Técnicas; ArgentinaFil: Döpp, A.. Universite de Paris Xi; Francia;Fil: Cassou, K.. Universite de Paris Xi; Francia;Fil: Genoud, G.. Lund University; Suecia;Fil: Wojda, F.. Lund University; Suecia;Fil: Burza, M.. Lund University; Suecia;Fil: Persson, A.. Lund University; Suecia;Fil: Lundh, O.. Lund University; Suecia;Fil: Wahlström, C. G.. Lund University; Suecia;Fil: Cros, B.. Universite de Paris Xi; Francia
Light-Induced Mechanistic Divergence in Gold(I) Catalysis:Revisiting the Reactivity of Diazonium Salts
In a systematic study of the Au-catalyzed reaction of o-alkynylphenols with aryldiazonium salts, we find that essentially the same reaction conditions lead to a change in mechanism when a light source is applied. If the reaction is carried out at room temperature using a AuI catalyst, the diazonium salt undergoes electrophilic deauration of a vinyl AuI intermediate and provides access to substituted azobenzofurans. If the reaction mixture is irradiated with blue LED light, C−C bond formation due to N2-extrusion from the diazonium salt is realized selectively, using the same starting materials without the need for an additional photo(redox) catalyst under aerobic conditions. We report a series of experiments demonstrating that the same vinyl AuI intermediate is capable of producing the observed products under photolytic and thermal conditions. The finding that a vinyl AuI complex can directly, without the need for an additional photo(redox) catalyst, result in C−C bond formation under photolytic conditions is contrary to the proposed mechanistic pathways suggested in the literature till date and highlights that the role of oxidation state changes in photoredox catalysis involving Au is thus far only poorly understood and may hold surprises for the future. Computational results indicate that photochemical activation can occur directly from a donor–acceptor complex formed between the vinyl AuI intermediate and the diazonium salt
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