Collective states in highly symmetric atomic configurations, and single-photon traps

Abbreviated Abstract: We study correlated states in a circular and linear-chain configuration of identical two-level atoms containing the energy of a single quasi-resonant photon in the form of a collective excitation, where the collective behaviour is mediated by exchange of transverse photons between the atoms. For a circular configuration of atoms the effective Hamiltonian on the radiationless subspace of the system can be diagonalized analytically. In this case, the radiationless energy eigenstates carry a $\mathbb{Z}_N$ quantum number $p=0,1, ..., N$ which is analogous to the angular momentum quantum number $l= 0, 1, ...$, carried by particles propagating in a central potential, such as a hydrogen-like system. Just as the hydrogen s-states are the only electronic wave functions which can occupy the central region of the Coulomb potential, the quasi-particle corresponding to a collective excitation of the circular atomic sample can occupy the central atom only for vanishing $\mathbb{Z}_N$ quantum number $p$. For large numbers of atoms in a maximally subradiant state, a critical interatomic distance of $\lambda/2$ emerges both in the linear-chain and the circular configuration of atoms. The spontaneous decay rate of the linear configuration exhibits a jump-like "critical" behaviour for next-neighbour distances close to a half-wavelength. Furthermore, both the linear-chain and the circular configuration exhibit exponential photon trapping once the next-neighbour distance becomes less than a half-wavelength, with the suppression of spontaneous decay being particularly pronounced in the circular system. In this way, circular configurations containing sufficiently many atoms may be natural candidates for {\it single-photon traps}.Comment: Invited contribution to "Xth International Conference on Quantum Optics ICQO 2004" in Minsk, Belarus. To be published in Optics and Spectroscop

Three fluid hydrodynamics of spin-1 Bose-Einstein condensates

We study excitations of the spin-1 Bose gas at finite temperatures and in the presence of a not so strong magnetic field, or equivalently, when the gas sample is partially polarized. Motivated by the success of two-fluid hydrodynamics of scalar superfluids we develop a three-fluid hydrodynamic description to treat the low frequency and long wavelength excitations of the spin-1 Bose gas. We derive the coupled linear hydrodynamic equations of the three sounds and evaluate them numerically in a self-consistent mean field approximation valid for the dilute gas at the intermediate and critical temperature regions. In this latter region we identify the critical mode

Femtosecond pulses and dynamics of molecular photoexcitation: RbCs example

We investigate the dynamics of molecular photoexcitation by unchirped femtosecond laser pulses using RbCs as a model system. This study is motivated by a goal of optimizing a two-color scheme of transferring vibrationally-excited ultracold molecules to their absolute ground state. In this scheme the molecules are initially produced by photoassociation or magnetoassociation in bound vibrational levels close to the first dissociation threshold. We analyze here the first step of the two-color path as a function of pulse intensity from the low-field to the high-field regime. We use two different approaches, a global one, the 'Wavepacket' method, and a restricted one, the 'Level by Level' method where the number of vibrational levels is limited to a small subset. The comparison between the results of the two approaches allows one to gain qualitative insights into the complex dynamics of the high-field regime. In particular, we emphasize the non-trivial and important role of far-from-resonance levels which are adiabatically excited through 'vertical' transitions with a large Franck-Condon factor. We also point out spectacular excitation blockade due to the presence of a quasi-degenerate level in the lower electronic state. We conclude that selective transfer with femtosecond pulses is possible in the low-field regime only. Finally, we extend our single-pulse analysis and examine population transfer induced by coherent trains of low-intensity femtosecond pulses.Comment: 25 pages, 12 figure

Control of dipolar relaxation in external fields

We study dipolar relaxation in both ultra-cold thermal and Bose-condensed chromium atom gases. We show three different ways to control dipolar relaxation, making use of either a static magnetic field, an oscillatory magnetic field, or an optical lattice to reduce the dimensionality of the gas from 3D to 2D. Although dipolar relaxation generally increases as a function of a static magnetic field intensity, we find a range of non-zero magnetic field intensities where dipolar relaxation is strongly reduced. We use this resonant reduction to accurately determine the S=6 scattering length of chromium atoms: $a_6 = 103 \pm 4 a_0$. We compare this new measurement to another new determination of $a_6$, which we perform by analysing the precise spectroscopy of a Feshbach resonance in d-wave collisions, yielding $a_6 = 102.5 \pm 0.4 a_0$. These two measurements provide by far the most precise determination of $a_6$ to date. We then show that, although dipolar interactions are long-range interactions, dipolar relaxation only involves the incoming partial wave $l=0$ for large enough magnetic field intensities, which has interesting consequences on the stability of dipolar Fermi gases. We then study ultra-cold chromium gases in a 1D optical lattice resulting in a collection of independent 2D gases. We show that dipolar relaxation is modified when the atoms collide in reduced dimensionality at low magnetic field intensities, and that the corresponding dipolar relaxation rate parameter is reduced by a factor up to 7 compared to the 3D case. Finally, we study dipolar relaxation in presence of radio-frequency (rf) oscillating magnetic fields, and we show that both the output channel energy and the transition amplitude can be controlled by means of rf frequency and Rabi frequency.Comment: 25 pages, 17 figure

Dual-probe decoherence microscopy: Probing pockets of coherence in a decohering environment

We study the use of a pair of qubits as a decoherence probe of a non-trivial environment. This dual-probe configuration is modelled by three two-level-systems which are coupled in a chain in which the middle system represents an environmental two-level-system (TLS). This TLS resides within the environment of the qubits and therefore its coupling to perturbing fluctuations (i.e. its decoherence) is assumed much stronger than the decoherence acting on the probe qubits. We study the evolution of such a tripartite system including the appearance of a decoherence-free state (dark state) and non-Markovian behaviour. We find that all parameters of this TLS can be obtained from measurements of one of the probe qubits. Furthermore we show the advantages of two qubits in probing environments and the new dynamics imposed by a TLS which couples to two qubits at once.Comment: 29 pages, 10 figure

Preparation of decoherence-free, subradiant states in a cavity

The cause of decoherence in a quantum system can be traced back to the interaction with the environment. As it has been pointed out first by Dicke, in a system of N two-level atoms where each of the atoms is individually dipole coupled to the environment, there are collective, subradiant states, that have no dipole coupling to photon modes, and therefore they are expected to decay slower. This property also implies that these type of states, which form an N-1 dimensional subspace of the atomic subsytem, also decohere slower. We propose a scheme which will create such states. First the two-level atoms are placed in a strongly detuned cavity and one of the atoms, called the control atom is excited. The time evolution of the coupled atom-cavity system leads to an appropriately entangled state of the atoms. By applying subsequent laser pulses at a well defined time instant, it is possible to drive the atomic state into the subradiant, i. e., decoherence free subspace. Up to a certain average number of the photons, the result is independent of the state of the cavity. The analysis of the conditions shows that this scheme is feasible with present day techniques achieved in atom cavity interaction experiments.Comment: 5 page

Mean field ground state of a spin-1 condensate in a magnetic field

We revisit the topic of the mean field ground state of a spin-1 atomic condensate inside a uniform magnetic field ($B$) under the constraints that both the total number of atoms ($N$) and the magnetization ($\cal M$) are conserved. In the presence of an internal state (spin component) independent trap, we also investigate the dependence of the so-called single spatial mode approximation (SMA) on the magnitude of the magnetic field and ${\cal M}$. Our result indicate that the quadratic Zeeman effect is an important factor in balancing the mean field energy from elastic atom-atom collisions that are known to conserve both $N$ and $\cal M$.Comment: 13 pages, 9 figures, to be published in New J. Phys. (http://www.njp.org/

Application of B-splines to determining eigen-spectrum of Feshbach molecules

The B-spline basis set method is applied to determining the rovibrational eigen-spectrum of diatomic molecules. A particular attention is paid to a challenging numerical task of an accurate and efficient description of the vibrational levels near the dissociation limit (halo-state and Feshbach molecules). Advantages of using B-splines are highlighted by comparing the performance of the method with that of the commonly-used discrete variable representation (DVR) approach. Several model cases, including the Morse potential and realistic potentials with 1/R^3 and 1/R^6 long-range dependence of the internuclear separation are studied. We find that the B-spline method is superior to the DVR approach and it is robust enough to properly describe the Feshbach molecules. The developed numerical method is applied to studying the universal relation of the energy of the last bound state to the scattering length. We numerically illustrate the validity of the quantum-defect-theoretic formulation of such a relation for a 1/R^6 potential.Comment: submitted to can j phys: Walter Johnson symposu

Complete eigenstates of identical qubits arranged in regular polygons

We calculate the energy eigenvalues and eigenstates corresponding to coherent single and multiple excitations of an array of N identical qubits or two-level atoms (TLA's) arranged on the vertices of a regular polygon. We assume only that the coupling occurs via an exchange interaction which depends on the separation between the qubits. We include the interactions between all pairs of qubits, and our results are valid for arbitrary distances relative to the radiation wavelength. To illustrate the usefulness of these states, we plot the distance dependence of the decay rates of the n=2 (biexciton) eigenstates of an array of 4 qubits, and tabulate the biexciton eigenvalues and eigenstates, and absorption frequencies, line widths, and relative intensities for polygons consisting of N=2,...,9 qubits in the long-wavelength limit.Comment: Added a figure showing how these results can be used to compute deviations from "equal collective decoherence" approximation