186 research outputs found

    Predicting Rumination from the Five Facets of Mindfulness

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    Mindfulness is defined as a process of paying attention to the moment-by-moment experience of thoughts and feelings. It is a non-elaborative, non-judgmental, present-centered awareness in which each thought, feeling or sensation that arises in the attentional field is acknowledged and accepted (Kabat-Zinn, 1990; 1998). The concept of mindfulness adopted in Western therapeutic contexts was derived from Eastern spiritual and philosophical Buddhist teachings. Since its introduction nearly 20 years ago, mindfulness-based treatments have evolved towards altering the relationship between the self and internal/external sensations to reduce multiple forms of psychological and physical morbidity (Bishop et al., 2004). Currently, it is used as a mechanism to prevent relapse of depression (Segal, Williams, & Teasdale, 2002; Scherer-Dickson, 2004), anxiety (Roemer & Orsillo, 2002), eating disorders (Telech, Agras, Stewart, & Linehan, 2001), and a variety of other psychological disorders (see Kabat-Zinn, 1990 for review). Much of the literature have provided empirical support for the effectiveness of these treatments but have not explored the roles that the five facets of mindfulness play in predicting or reducing the minute features of mental illness. The purpose of the current study was to replicate results supporting the effectiveness of mindfulness in reducing rumination while examining the specific facets of mindfulness that facilitate this change. In addition, rumination was tested as a possible mediator to ascertain the nature of mindfulness\u27 influence on the states of depression and anger. Two forms of rumination were examined: depressive and anger rumination. They are distinct forms of the same maladaptive coping mechanism (Whitmer & Banich, 2007). One hundred thirty-two Eastern Illinois University students participated in the study. Their levels of mindfulness, depressive/anger rumination, and depressive/anger states were measured. Overall, mindfulness exhibited inverse relationships with both depressive and anger rumination. The mindfulness facet of \u27non-judgment\u27 primarily accounted for the lower levels of depressive and anger rumination. In addition, the facets of \u27non-reactivity\u27 and \u27observation\u27 were associated with anger rumination (though \u27observation\u27 was unexpectedly positively correlated with anger rumination). Subsequent analyses examining the relationship between mindfulness and depressive/anger emotional states found depressive rumination to be a partial mediator of the relationship of mindfulness with depression, while anger rumination fully mediated the relationship with anger. Clinical implications of this research, limitations and suggestions for future studies were discussed

    Accelerated Springtime Melt of Snow on Tundra Downwind from Northern Alaska River Systems Resulting from Niveo-aeolian Deposition Events

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    It is well known that light-absorbing particulate matter (PM) enhances absorption of sunlight when deposited on ice and snow. Such increased absorption is due to a reduction in surface albedo, resulting in accelerated melt of frozen surfaces. In isolation, earlier melt enhances Arctic warming since dark surfaces underlying snow and ice are exposed and absorb additional solar energy. Here, we combine various observational tools to demonstrate that aeolian deposition of PM along fluvial features on the North Slope of Alaska resulted in a notable reduction of surface albedo in the spring of 2016, from values typical for snow (~0.8) to around 0.35 on average. This reduction resulted in accelerated snow and ice melt by up to three weeks compared to unaffected areas. This phenomenon was observed to some degree in 12 other years dating back to 2003. Deposition generally was found to occur near particular sections of the rivers, with several areas affected by events in multiple years. In all years, the deposition is attributed to high wind events. The extreme case in 2016 is linked to unusually strong and extraordinarily persistent winds during April. The deposited material is thought to be the natural sediment carried by the rivers, resulting in a seasonally replenished source of PM. These findings indicate a previously unreported impact of both fluvial and atmospheric processes on the seasonal melt of northern Alaska rivers.Il s’agit d’un fait bien connu que la matière particulaire photo-absorbante rehausse l’absorption de la lumière solaire lorsqu’elle est déposée sur la glace et la neige. Cette absorption accrue est attribuable à la réduction de l’albédo de la surface, ce qui se traduit par la fonte accélérée des surfaces glacées. Individuellement, la fonte hâtive augmente le réchauffement de l’Arctique parce que les surfaces sombres se trouvant sous la neige et la glace sont exposées et absorbent l’énergie solaire supplémentaire. Ici, nous recourons à divers outils d’observation pour montrer que le dépôt éolien de matière particulaire le long des caractéristiques fluviales de la North Slope de l’Alaska a entraîné une réduction notable de l’albédo de la surface au printemps de 2016, passant de valeurs typiques pour la neige de (~ 0,8) à environ 0,35 en moyenne. Cette réduction a donné lieu à l’accélération de la fonte de la neige et de la glace dans une mesure de trois semaines comparativement aux endroits qui n’ont pas été touchés par la réduction. Ce phénomène a été observé dans une certaine mesure pendant 12 autres années, remontant en 2003. De manière générale, des dépôts se sont ramassés près de segments particuliers des cours d’eau, et plusieurs des secteurs ont été touchés par des événements au cours de plusieurs années. Dans l’ensemble, les dépôts sont attribués à des vents violents. Le cas extrême de 2016 découle de vents inhabituellement forts et extraordinairement persistants en avril. La matière déposée serait peut-être du sédiment naturel transporté par les cours d’eau, ce qui donne lieu au réapprovisionnement saisonnier de la source de matière particulaire. Ces constatations mènent à une incidence antérieurement non déclarée des processus fluviaux et atmosphériques sur la fonte saisonnière des cours d’eau du nord de l’Alaska

    Measurements of Isoprene-Derived Organosulfates in Ambient Aerosols by Aerosol Time-of-Flight Mass Spectrometry—Part 2: Temporal Variability and Formation Mechanisms

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    Organosulfate species have recently gained attention for their potentially significant contribution to secondary organic aerosol (SOA); however, their temporal behavior in the ambient atmosphere has not been probed in detail. In this work, organosulfates derived from isoprene were observed in single particle mass spectra in Atlanta, GA during the 2002 Aerosol Nucleation and Characterization Experiment (ANARChE) and the 2008 August Mini-Intensive Gas and Aerosol Study (AMIGAS). Real-time measurements revealed that the highest organosulfate concentrations occurred at night under a stable boundary layer, suggesting gas-to-particle partitioning and subsequent aqueous-phase processing of the organic precursors played key roles in their formation. Further analysis of the diurnal profile suggests possible contributions from multiple production mechanisms, including acid-catalysis and radical-initiation. This work highlights the potential for additional SOA formation pathways in biogenically influenced urban regions to enhance the organic aerosol burden

    Contrasting local and long-range-transported warm ice-nucleating particles during an atmospheric river in coastal California, USA

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    Ice-nucleating particles (INPs) have been found to influence the amount, phase and efficiency of precipitation from winter storms, including atmospheric rivers.Warm INPs, those that initiate freezing at temperatures warmer than -10°C, are thought to be particularly impactful because they can create primary ice in mixed-phase clouds, enhancing precipitation efficiency. The dominant sources of warm INPs during atmospheric rivers, the role of meteorology in modulating transport and injection of warm INPs into atmospheric river clouds, and the impact of warm INPs on mixed-phase cloud properties are not well-understood. In this case study, time-resolved precipitation samples were collected during an atmospheric river in northern California, USA, during winter 2016. Precipitation samples were collected at two sites, one coastal and one inland, which are separated by about 35 km. The sites are sufficiently close that air mass sources during this storm were almost identical, but the inland site was exposed to terrestrial sources of warm INPs while the coastal site was not. Warm INPs were more numerous in precipitation at the inland site by an order of magnitude. Using FLEXPART (FLEXible PARTicle dispersion model) dispersion modeling and radar-derived cloud vertical structure, we detected influence from terrestrial INP sources at the inland site but did not find clear evidence of marine warm INPs at either site.We episodically detected warm INPs from long-range-transported sources at both sites. By extending the FLEXPART modeling using a meteorological reanalysis, we demonstrate that long-range-transported warm INPs were observed only when the upper tropospheric jet provided transport to cloud tops. Using radar-derived hydrometeor classifications, we demonstrate that hydrometeors over the terrestrially influenced inland site were more likely to be in the ice phase for cloud temperatures between 0 and -10°C. We thus conclude that terrestrial and long-rangetransported aerosol were important sources of warm INPs during this atmospheric river. Meteorological details such as transport mechanism and cloud structure were important in determining (i) warm INP source and injection temperature and (ii) ultimately the impact of warm INPs on mixed-phase cloud properties

    Measurements of Isoprene-Derived Organosulfates in Ambient Aerosols by Aerosol Time-of-Flight Mass Spectrometry - Part 1: Single Particle Atmospheric Observations in Atlanta

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    Organosulfate species have recently been identified as a potentially significant class of secondary organic aerosol (SOA) species, yet little is known about their behavior in the atmosphere. In this work, organosulfates were observed in individual ambient aerosols using single particle mass spectrometry in Atlanta, GA during the 2002 Aerosol Nucleation and Characterization Experiment (ANARChE) and the 2008 August Mini-Intensive Gas and Aerosol Study (AMIGAS). Organosulfates derived from biogenically produced isoprene were detected as deprotonated molecular ions in negative-ion spectra measured by aerosol time-of-flight mass spectrometry; comparison to high-resolution mass spectrometry data obtained from filter samples corroborated the peak assignments. The size-resolved chemical composition measurements revealed that organosulfate species were mostly detected in submicrometer aerosols and across a range of aerosols from different sources, consistent with secondary reaction products. Detection of organosulfates in a large fraction of negative-ion ambient spectra − ca. 90−95% during ANARChE and ~65% of submicrometer particles in AMIGAS − highlights the ubiquity of organosulfate species in the ambient aerosols of biogenically influenced urban environments

    Impact of Asian Aerosols on Precipitation Over California: An Observational and Model Based Approach

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    Dust and pollution emissions from Asia are often transported across the Pacific Ocean to over the western United States. Therefore, it is essential to fully understand the impact of these aerosols on clouds and precipitation forming over the eastern Pacific and western United States, especially during atmospheric river events that account for up to half of California's annual precipitation and can lead to widespread flooding. In order for numerical modeling simulations to accurately represent the present and future regional climate of the western United States, we must account for the aerosol-cloud-precipitation interactions associated with Asian dust and pollution aerosols. Therefore, we have constructed a detailed study utilizing multi-sensor satellite observations, NOAA-led field campaign measurements, and targeted numerical modeling studies where Asian aerosols interacted with cloud and precipitation processes over the western United States. In particular, we utilize aerosol optical depth retrievals from the NASA Moderate Resolution Imaging Spectroradiometer (MODIS), NOAA Geostationary Operational Environmental Satellite (GOES-11), and Japan Meteorological Agency (JMA) Multi-functional Transport Satellite (MTSAT) to effectively detect and monitor the trans-Pacific transport of Asian dust and pollution. The aerosol optical depth (AOD) retrievals are used in assimilating the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) in order to provide the model with an accurate representation of the aerosol spatial distribution across the Pacific. We conduct WRF-Chem model simulations of several cold-season atmospheric river events that interacted with Asian aerosols and brought significant precipitation over California during February-March 2011 when the NOAA CalWater field campaign was ongoing. The CalWater field campaign consisted of aircraft and surface measurements of aerosol and precipitation processes that help extensively validate our WRF-Chem model simulations. After validating the capability of the WRF-Chem in realistically simulating the aerosol-cloud precipitation interactions, we conduct sensitivity studies where the AOD is doubled to diagnose whether an increasing concentration of Asian aerosols over the western United States will lead to further impacts on the cloud and precipitation processes over California. We also perform sensitivity studies where the aerosols will be partitioned into dust-only and pollution-only in order to separate the impacts of the differing Asian aerosol species. The results of our WRF-Chem model simulations aim to show that the trans-Pacific transport of Asian aerosols influence the precipitation associated with atmospheric river events that can ultimately impact the regional climate of the western United States. 1 Universit

    Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location

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    Aerosols that serve as ice nucleating particles (INPs) have the potential to modulate cloud microphysical properties and can therefore impact cloud radiative forcing (CRF) and precipitation formation processes. In remote regions such as the Arctic, aerosol–cloud interactions are severely understudied yet may have significant implications for the surface energy budget and its impact on sea ice and snow surfaces. Further, uncertainties in model representations of heterogeneous ice nucleation are a significant hindrance to simulating Arctic mixed-phase cloud processes. We present results from a campaign called INPOP (Ice Nucleating Particles at Oliktok Point), which took place at a US Department of Energy Atmospheric Radiation Measurement (DOE ARM) facility in the northern Alaskan Arctic. Three time- and size-resolved aerosol impactors were deployed from 1 March to 31 May 2017 for offline ice nucleation and chemical analyses and were co-located with routine measurements of aerosol number and size. The largest particles (i.e., ≥&thinsp;3&thinsp;µm or “coarse mode”) were the most efficient INPs by inducing freezing at the warmest temperatures. During periods with snow- and ice-covered surfaces, coarse mode INP concentrations were very low (maximum of 6&thinsp;×&thinsp;10−4&thinsp;L−1 at −15&thinsp;∘C), but higher concentrations of warm-temperature INPs were observed during late May (maximum of 2&thinsp;×&thinsp;10−2&thinsp;L−1 at −15&thinsp;∘C). These higher concentrations were attributed to air masses originating from over open Arctic Ocean water and tundra surfaces. To our knowledge, these results represent the first INP characterization measurements in an Arctic oilfield location and demonstrate strong influences from mineral and marine sources despite the relatively high springtime pollution levels. Ultimately, these results can be used to evaluate the anthropogenic and natural influences on aerosol composition and Arctic cloud properties.</p

    Contrasting local and long-range-transported warm ice-nucleating particles during an atmospheric river in coastal California, USA

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    Ice-nucleating particles (INPs) have been found to influence the amount, phase and efficiency of precipitation from winter storms, including atmospheric rivers. Warm INPs, those that initiate freezing at temperatures warmer than −10&thinsp;∘C, are thought to be particularly impactful because they can create primary ice in mixed-phase clouds, enhancing precipitation efficiency. The dominant sources of warm INPs during atmospheric rivers, the role of meteorology in modulating transport and injection of warm INPs into atmospheric river clouds, and the impact of warm INPs on mixed-phase cloud properties are not well-understood. In this case study, time-resolved precipitation samples were collected during an atmospheric river in northern California, USA, during winter 2016. Precipitation samples were collected at two sites, one coastal and one inland, which are separated by about 35&thinsp;km. The sites are sufficiently close that air mass sources during this storm were almost identical, but the inland site was exposed to terrestrial sources of warm INPs while the coastal site was not. Warm INPs were more numerous in precipitation at the inland site by an order of magnitude. Using FLEXPART (FLEXible PARTicle dispersion model) dispersion modeling and radar-derived cloud vertical structure, we detected influence from terrestrial INP sources at the inland site but did not find clear evidence of marine warm INPs at either site. We episodically detected warm INPs from long-range-transported sources at both sites. By extending the FLEXPART modeling using a meteorological reanalysis, we demonstrate that long-range-transported warm INPs were observed only when the upper tropospheric jet provided transport to cloud tops. Using radar-derived hydrometeor classifications, we demonstrate that hydrometeors over the terrestrially influenced inland site were more likely to be in the ice phase for cloud temperatures between 0 and −10&thinsp;∘C. We thus conclude that terrestrial and long-range-transported aerosol were important sources of warm INPs during this atmospheric river. Meteorological details such as transport mechanism and cloud structure were important in determining (i) warm INP source and injection temperature and (ii) ultimately the impact of warm INPs on mixed-phase cloud properties.</p

    The relative impact of cloud condensation nuclei and ice nucleating particle concentrations on phase partitioning in Arctic mixed-phase stratocumulus clouds

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    This study investigates the interactions between cloud dynamics and aerosols in idealized large-eddy simulations (LES) of Arctic mixed-phase stratocumulus clouds (AMPS) observed at Oliktok Point, Alaska, in April 2015. This case was chosen because it allows the cloud to form in response to radiative cooling starting from a cloud-free state, rather than requiring the cloud ice and liquid to adjust to an initial cloudy state. Sensitivity studies are used to identify whether there are buffering feedbacks that limit the impact of aerosol perturbations. The results of this study indicate that perturbations in ice nucleating particles (INPs) dominate over cloud condensation nuclei (CCN) perturbations; i.e., an equivalent fractional decrease in CCN and INPs results in an increase in the cloud-top longwave cooling rate, even though the droplet effective radius increases and the cloud emissivity decreases. The dominant effect of ice in the simulated mixed-phase cloud is a thinning rather than a glaciation, causing the mixed-phase clouds to radiate as a grey body and the radiative properties of the cloud to be more sensitive to aerosol perturbations. It is demonstrated that allowing prognostic CCN and INPs causes a layering of the aerosols, with increased concentrations of CCN above cloud top and increased concentrations of INPs at the base of the cloud-driven mixed layer. This layering contributes to the maintenance of the cloud liquid, which drives the dynamics of the cloud system.</p
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