Ground-state and decay properties of neutron-rich Nb 106

The ground-state properties of neutron-rich Nb106 and its β decay into Mo106 have been studied using the CARIBU radioactive-ion-beam facility at Argonne National Laboratory. Niobium-106 ions were extracted from a Cf252 fission source and mass separated before being delivered as low-energy beams to the Canadian Penning Trap, as well as the X-Array and SATURN β-decay-spectroscopy station. The measured Nb106 ground-state mass excess of -66202.0(13) keV is consistent with a recent measurement but has three times better precision; this work also rules out the existence of a second long-lived, β-decaying state in Nb106 above 5 keV in excitation energy. The decay half-life of Nb106 was measured to be 1.097(21) s, which is 8% longer than the adopted value. The level scheme of the decay progeny, Mo106, has been expanded up to ≈4MeV. The distribution of decay strength and considerable population of excited states in Mo106 of J≥3 emphasizes the need to revise the adopted Jπ=1- ground-state spin-parity assignment of Nb106; it is more likely to be J≥3

Masses and β -Decay Spectroscopy of Neutron-Rich Odd-Odd Eu 160,162 Nuclei: Evidence for a Subshell Gap with Large Deformation at N=98

The structure of deformed neutron-rich nuclei in the rare-earth region is of significant interest for both the astrophysics and nuclear structure fields. At present, a complete explanation for the observed peak in the elemental abundances at A∼160 eludes astrophysicists, and models depend on accurate quantities, such as masses, lifetimes, and branching ratios of deformed neutron-rich nuclei in this region. Unusual nuclear structure effects are also observed, such as the unexpectedly low energies of the first 2+ levels in some even-even nuclei at N=98. In order to address these issues, mass and β-decay spectroscopy measurements of the Eu97160 and Eu99162 nuclei were performed at the Californium Rare Isotope Breeder Upgrade radioactive beam facility at Argonne National Laboratory. Evidence for a gap in the single-particle neutron energies at N=98 and for large deformation (β2∼0.3) is discussed in relation to the unusual phenomena observed at this neutron number

Masses and β -Decay Spectroscopy of Neutron-Rich Odd-Odd Eu 160,162 Nuclei: Evidence for a Subshell Gap with Large Deformation at N=98

The structure of deformed neutron-rich nuclei in the rare-earth region is of significant interest for both the astrophysics and nuclear structure fields. At present, a complete explanation for the observed peak in the elemental abundances at A∼160 eludes astrophysicists, and models depend on accurate quantities, such as masses, lifetimes, and branching ratios of deformed neutron-rich nuclei in this region. Unusual nuclear structure effects are also observed, such as the unexpectedly low energies of the first 2+ levels in some even-even nuclei at N=98. In order to address these issues, mass and β-decay spectroscopy measurements of the Eu97160 and Eu99162 nuclei were performed at the Californium Rare Isotope Breeder Upgrade radioactive beam facility at Argonne National Laboratory. Evidence for a gap in the single-particle neutron energies at N=98 and for large deformation (β2∼0.3) is discussed in relation to the unusual phenomena observed at this neutron number

Recent advances in β-decay spectroscopy at CARIBU

β-decay spectroscopy of nuclei far from stability can provide powerful insight into a broad variety of topics in nuclear science, ranging from exotic nuclear structure phenomena, stellar nucleosynthesis processes, and applied topics such as quantifying "decay heat" discrepancies for advanced nuclear fuel cycles. Neutronrich nuclei approaching the drip-line are difficult to access experimentally, leaving many key examples largely under studied. The CARIBU radioactive beam facility at Argonne National Laboratory exploits spontaneous fission of 252Cf in production of such beams. The X-Array and SATURN decay station have been commissioned to perform detailed decay spectroscopy of low-energy CARIBU beams. An extended science campaign was started during 2015; with projects investigating nuclear shape changes, collective octupole vibrations, β-delayed neutron emission, and decay-scheme properties which could explain the reactor antineutrino puzzle. In this article we review the current status of the setup, update on the first results and recent hardware upgrades, and look forward to future possibilities

γ -soft Ba 146 and the role of nonaxial shapes at N≈90

Low-spin states in the neutron-rich, N=90 nuclide Ba146 were populated following β decay of Cs146, with the goal of clarifying the development of deformation in barium isotopes through delineation of their nonyrast structures. Fission fragments of Cs146 were extracted from a 1.7-Ci Cf252 source and mass selected using the CAlifornium Rare Ion Breeder Upgrade (CARIBU) facility. Low-energy ions were deposited at the center of a box of thin β detectors, surrounded by a highly efficient high-purity Ge array. The new Ba146 decay scheme now contains 31 excited levels extending up to ∼2.5 MeV excitation energy, double what was previously known. These data are compared to predictions from the interacting boson approximation (IBA) model. It appears that the abrupt shape change found at N=90 in Sm and Gd is much more gradual in Ba and Ce, due to an enhanced role of the γ degree of freedom

gamma-soft Ba-146 and the role of nonaxial shapes at N approximate to 90

Low-spin states in the neutron-rich, N=90 nuclide Ba146 were populated following β decay of Cs146, with the goal of clarifying the development of deformation in barium isotopes through delineation of their nonyrast structures. Fission fragments of Cs146 were extracted from a 1.7-Ci Cf252 source and mass selected using the CAlifornium Rare Ion Breeder Upgrade (CARIBU) facility. Low-energy ions were deposited at the center of a box of thin β detectors, surrounded by a highly efficient high-purity Ge array. The new Ba146 decay scheme now contains 31 excited levels extending up to ∼2.5 MeV excitation energy, double what was previously known. These data are compared to predictions from the interacting boson approximation (IBA) model. It appears that the abrupt shape change found at N=90 in Sm and Gd is much more gradual in Ba and Ce, due to an enhanced role of the γ degree of freedom

B-decay half-lives of ¹³⁴ ̓ ¹³⁴ᴹSb and their isomeric yield ratio produced by the spontaneous fission of ²⁵²Cf

A number of fission products possess isomeric states which have a nuclear spin significantly different from that of the ground state. The yield ratio of these states following fission is influenced by the angular momentum present in the fissioning system. The 134m,134Sb yield ratio had not been previously measured in the spontaneous fission of 252Cf; however, it had previously been observed to favor the (7−) isomer over the (0−) ground state in 235 U (nth,f) and 232 Th (25 MeV p,f). Using a mass-separated beam of low-energy 134, 134m Sb ions produced by 252 Cf spontaneous fission at the CARIBU facility, β particles and γ rays were detected using the SATURN/X-Array decay station to determine the fission-yield ratio and β-decay half-lives. The 134m Sb to 134Sb fission yield was determined to be 2.03 ±0.05 and the half-lives of 134m Sb and 134Sb were found to be 9.87±0.08s and 0.674±0.004s, respectively. These results represent the first isomeric yield ratio measurement for this nucleus, and improved measurements of the 134 Sb ground state and the 134m Sb isomer half-lives.This material is based upon work supported by the National Science Foundation, under Grant No. PHY-1419765 (University of Notre Dame); Department of Energy, National Nuclear Security Administration, under Award Nos. DE-NA0000979 (NSSC), DE-AC52-07NA27344 (LLNL), FOA LAB 17- 1763; Office of Nuclear Physics Contract No. DE-AC02- 06CH11357 (ANL), and Grants No. DE-FG02-94ER40848 (UML), DE-AC02-98CH10886 (BNL); NSERC, Canada, under Application No. 216974; Australian Research Council, Grant No. DP130104176 (ANU)

High-K, two-quasiparticle states in Gd-160

Excited states in Gd-160 were populated via beta decay from the low- and high-spin isomers in Eu-160. The highspin, K-pi = 5(-) state feeds several two-quasiparticle levels, as well as a sequence associated with a. vibration and a K-pi = 4(+), hexadecapole vibrational structure. The decay scheme was significantly improved with the observation of new transitions and states when compared with the two competing level schemes from over four decades ago. Configuration assignments for some of the multiquasiparticle levels have been suggested, based upon decay properties, systematics from neighboring nuclei, and comparisons with theoretical calculations. In addition, 15 new low-spin states and approximately 60 new transitions were observed resulting from the decay of the low-spin Eu-160 isomer

Recent advances in ?-decay spectroscopy at CARIBU

β-decay spectroscopy of nuclei far from stability can provide powerful insight into a broad variety of topics in nuclear science, ranging from exotic nuclear structure phenomena, stellar nucleosynthesis processes, and applied topics such as quantifying "decay heat" discrepancies for advanced nuclear fuel cycles. Neutronrich nuclei approaching the drip-line are difficult to access experimentally, leaving many key examples largely under studied. The CARIBU radioactive beam facility at Argonne National Laboratory exploits spontaneous fission of 252Cf in production of such beams. The X-Array and SATURN decay station have been commissioned to perform detailed decay spectroscopy of low-energy CARIBU beams. An extended science campaign was started during 2015; with projects investigating nuclear shape changes, collective octupole vibrations, β-delayed neutron emission, and decay-scheme properties which could explain the reactor antineutrino puzzle. In this article we review the current status of the setup, update on the first results and recent hardware upgrades, and look forward to future possibilitie