1,337 research outputs found
Intensity dependences of the nonlinear optical excitation of plasmons in graphene
Recently, we demonstrated an all-optical coupling
scheme for plasmons, which takes advantage of the
intrinsic nonlinear optical response of graphene.
Frequency mixing using free-space, visible light
pulses generates surface plasmons in a planar
graphene sample, where the phase matching
condition can define both the wavevector and energy
of surface waves and intraband transitions. Here,
we also show that the plasmon generation process is
strongly intensity-dependent, with resonance features
washed out for absorbed pulse fluences greater than
0.1 J m−2. This implies a subtle interplay between the
nonlinear generation process and sample heating. We
discuss these effects in terms of a non-equilibrium
charge distribution using a two-temperature model.Peer ReviewedPostprint (author's final draft
Practice of spirometry among physicians caring for children with asthma in Portugal - The EspiroPed survey
info:eu-repo/semantics/publishedVersio
Origins of All-Optical Generation of Plasmons in Graphene
This is the final version. Available on open access from Nature Research via the DOI in this recordGraphene, despite its centrosymmetric structure, is predicted to have a substantial second order nonlinearity, arising from
non-local effects. However, there is disagreement between several published theories and experimental data. Here we derive an
expression for the second order conductivity of graphene in the non-local regime using perturbation theory, concentrating on the
difference frequency mixing process, and compare our results with those already published. We find a second-order conductivity
(σ
(2)≈ 10−17AmV−2
) that is approximately three orders of magnitude less than that estimated from recent experimental results.
This indicates that nonlinear optical coupling to plasmons in graphene cannot be described perturbatively through the electronic
nonlinearity, as previously thought. We also show that this discrepancy cannot be attributed to the bulk optical nonlinearity of the
substrate. As a possible alternative, we present a simple theoretical model of how a non-linearity can arise from phFundacio Privada Cellex, Spanish MINECO Severo Ochoa ProgrammeCERCA Programme/Generalitat de CatalunyaEngineering and Physical Sciences Research Council (EPSRC)Royal SocietyTATAEuropean Commissio
Light pollution is associated with earlier tree budburst across the United Kingdom
ArticleThe ecological impact of night-time lighting is of concern because of its well-demonstrated effects on animal behaviour. However, the potential of light pollution to change plant phenology and its corresponding knock-on effects on associated herbivores are less clear. Here, we test if artificial lighting can advance the timing of budburst in trees. We took a UK-wide 13 year dataset of spatially referenced budburst data from four deciduous tree species and matched it with both satellite imagery of night-time lighting and average spring temperature. We find that budburst occurs up to 7.5 days earlier in brighter areas, with the relationship being more pronounced for later-budding species. Excluding large urban areas from the analysis showed an even more pronounced advance of budburst, confirming that the urban ‘heat-island’ effect is not the sole cause of earlier urban budburst. Similarly, the advance in budburst across all sites is too large to be explained by increases in temperature alone. This dramatic advance of budburst illustrates the need for further experimental investigation into the impact of artificial night-time lighting on plant phenology and subsequent species interactions. As light pollution is a growing global phenomenon, the findings of this study are likely to be applicable to a wide range of species interactions across the world.R.S.-Y. was supported by a GWR-ESF Studentship awarded
by the University of Exeter to R.H.f.-C. The study was also founded
by a BBSRC grant to R.H.f-C
New first trimester crown-rump length's equations optimized by structured data collection from a French general population
--- Objectives --- Prior to foetal karyotyping, the likelihood of Down's
syndrome is often determined combining maternal age, serum free beta-HCG,
PAPP-A levels and embryonic measurements of crown-rump length and nuchal
translucency for gestational ages between 11 and 13 weeks. It appeared
important to get a precise knowledge of these scan parameters' normal values
during the first trimester. This paper focused on crown-rump length. ---
METHODS --- 402 pregnancies from in-vitro fertilization allowing a precise
estimation of foetal ages (FA) were used to determine the best model that
describes crown-rump length (CRL) as a function of FA. Scan measures by a
single operator from 3846 spontaneous pregnancies representative of the general
population from Northern France were used to build a mathematical model linking
FA and CRL in a context as close as possible to normal scan screening used in
Down's syndrome likelihood determination. We modeled both CRL as a function of
FA and FA as a function of CRL. For this, we used a clear methodology and
performed regressions with heteroskedastic corrections and robust regressions.
The results were compared by cross-validation to retain the equations with the
best predictive power. We also studied the errors between observed and
predicted values. --- Results --- Data from 513 spontaneous pregnancies allowed
to model CRL as a function of age of foetal age. The best model was a
polynomial of degree 2. Datation with our equation that models spontaneous
pregnancies from a general population was in quite agreement with objective
datations obtained from 402 IVF pregnancies and thus support the validity of
our model. The most precise measure of CRL was when the SD was minimal
(1.83mm), for a CRL of 23.6 mm where our model predicted a 49.4 days of foetal
age. Our study allowed to model the SD from 30 to 90 days of foetal age and
offers the opportunity of using Zscores in the future to detect growth
abnormalities. --- Conclusion --- With powerful statistical tools we report a
good modeling of the first trimester embryonic growth in the general population
allowing a better knowledge of the date of fertilization useful in the
ultrasound screening of Down's syndrome. The optimal period to measure CRL and
predict foetal age was 49.4 days (9 weeks of gestational age). Our results open
the way to the detection of foetal growth abnormalities using CRL Zscores
throughout the first trimester
Fabrication of photonic band gap crystal using microtransfer molded templates
We have proposed and demonstrated an economical technique to fabricate a three-dimensional layer-by-layer photonic band gapstructure in the infrared wavelengths. An organic polymer template structure, an inverse layer-by-layer photonic crystalstructure, is assembled using the microtransfer molding technique. This template is infiltrated with sol-gel or nanoparticle titanium oxide slurry, then later removed by heat treatment at a temperature range of 550–800 °C. This method can be extended to fabricatephotonic crystals operating at optical and ultraviolet frequencies
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Development of a Calicum-Based Sorbent for Hot Gas Cleanup.
Further review of the technical literature has provided additional information which will support the development of a superior calcium-based sorbent for hot gas cleanup in IGCC systems. Two general methods of sorbent preparation are being investigated. One method involves impregnating a porous refractory substrate with calcium while another method involves pelletizing lime or other calcium containing materials with a suitable binder. Several potential substrates, which are made of alumina and are commercially available, have been characterized by various methods. The surface area and apparent density of the materials have been measured, and it has been shown that some of the high surface area materials (i.e., 200-400 m{sub 2}/g) undergo a large decrease in surface area when heated to higher temperatures. Some of the lower surface area materials (i.e., 1-30 m{sub 2}/g) have been successfully impregnated with calcium by soaking them in a calcium nitrate solution and then heat treating them to decompose the nitrate. Potentially useful sorbents have also been prepared by pelletizing type I Portland cement and mixtures of cement and lime
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