Extreme Ultraviolet Beam Enhancement by Relativistic Surface Plasmons

The emission of high-order harmonics in the extreme ultraviolet range from the interaction of a short, intense laser pulse with a grating target is investigated experimentally. When resonantly exciting a surface plasmon, both the intensity and the highest order observed for the harmonic emission along the grating surface increase with respect to a flat target. Harmonics are obtained when a suitable density gradient is preformed at the target surface, demonstrating the possibility to manipulate the grating profile on a nanometric scale without preventing the surface plasmon excitation. In support of this, the harmonic emission is spatiotemporally correlated to the acceleration of multi-MeV electron bunches along the grating surface. Particle-in-cell simulations reproduce the experimental results and give insight on the mechanism of high harmonic generation in the presence of surface plasmons

Interaction of Ultraintense Laser Vortices with Plasma Mirrors

International audienceLaser beams carrying orbital angular momentum (OAM) have found major applications in a variety of scientific fields, and their potential for ultrahigh-intensity laser-matter interactions has since recently been considered theoretically. We present an experiment where such beams interact with plasma mirrors up to laser intensities such that the motion of electrons in the laser field is relativistic. By measuring the spatial intensity and phase profiles of the high-order harmonics generated in the reflected beam, we obtain evidence for the helical wavefronts of the high-intensity laser at focus, and study the conservation of OAM in highly nonlinear optical processes at extreme laser intensities. The physical effects determining the field mode content of the twisted harmonic beams are elucidate

Sub-laser-cycle control of relativistic plasma mirrors

Letter - Open AccessInternational audienceWe present measurements of high-order harmonics and relativistic electrons emitted into the vacuum from a plasma mirror driven by temporally-shaped ultra-intense laser waveforms, produced by collinearly combining the main laser field with its second harmonic. We experimentally show how these observables are influenced by the phase delay between these two frequencies at the attosecond timescale, and relate these observations to the underlying physics through an advanced analysis of 1D/2D Particle-In-Cell simulations. These results demonstrate that sub-cycle shaping of the driving laser field provides fine control on the properties of the relativistic electron bunches responsible for harmonic and particle emission from plasma mirrors

Sub-laser-cycle control of relativistic plasma mirrors

Letter - Open AccessInternational audienceWe present measurements of high-order harmonics and relativistic electrons emitted into the vacuum from a plasma mirror driven by temporally-shaped ultra-intense laser waveforms, produced by collinearly combining the main laser field with its second harmonic. We experimentally show how these observables are influenced by the phase delay between these two frequencies at the attosecond timescale, and relate these observations to the underlying physics through an advanced analysis of 1D/2D Particle-In-Cell simulations. These results demonstrate that sub-cycle shaping of the driving laser field provides fine control on the properties of the relativistic electron bunches responsible for harmonic and particle emission from plasma mirrors

Interaction of ultraintense radially-polarized laser pulses with plasma mirrors

International audienceWe present experimental results of vacuum laser acceleration (VLA) of electrons using radially polarized laser pulses interacting with a plasma mirror. Tightly focused, radially polarized laser pulses have been proposed for electron acceleration because of their strong longitudinal electric field, making them ideal for VLA. However, experimental results have been limited until now because injecting electrons into the laser field has remained a considerable challenge. Here, we demonstrate experimentally that using a plasma mirror as an injector solves this problem and permits us to inject electrons at the ideal phase of the laser, resulting in the acceleration of electrons along the laser propagation direction while reducing the electron beam divergence compared to the linear polarization case. We obtain electron bunches with few-MeV energies and a 200-pC charge, thus demonstrating, for the first time, electron acceleration to relativistic energies using a radially polarized laser. High-harmonic generation from the plasma surface is also measured, and it provides additional insight into the injection of electrons into the laser field upon its reflection on the plasma mirror. Detailed comparisons between experimental results and full 3D simulations unravel the complex physics of electron injection and acceleration in this new regime: We find that electrons are injected into the radially polarized pulse in the form of two spatially separated bunches emitted from the p-polarized regions of the focus. Finally, we leverage on the insight brought by this study to propose and validate a more optimal experimental configuration that can lead to extremely peaked electron angular distributions and higher energy beams

Identification of Coupling Mechanisms between Ultraintense Laser Light and Dense Plasmas

The interaction of intense laser beams with plasmas created on solid targets involves a rich nonlinear physics. Because such dense plasmas are reflective for laser light, the coupling with the incident beam occurs within a thin layer at the interface between plasma and vacuum. One of the main paradigms used to understand this coupling, known as the Brunel mechanism, is expected to be valid only for very steep plasma surfaces. Despite innumerable studies, its validity range remains uncertain, and the physics involved for smoother plasma-vacuum interfaces is unclear, especially for ultrahigh laser intensities. We report the first comprehensive experimental and numerical study of the laser-plasma coupling mechanisms as a function of the plasma interface steepness, in the relativistic interaction regime. Our results reveal a clear transition from the temporally periodic Brunel mechanism to a chaotic dynamic associated to stochastic heating. By revealing the key signatures of these two distinct regimes on experimental observables, we provide an important landmark for the interpretation of future experiments

Laser-dressed photoionization for the temporal characterization of attosecond pulses generated from plasma mirrors

We report on the implementation of a laser-dressed photoionization method aimed at measuring the temporal structure of high-order harmonics generated from plasma mirrors at the attosecond timescale. Using numerical simulations, we show that the infrared dressing pulse induces up-down asymmetry on the angular distribution of photoelectrons. Experimentally single-shot photoelectron spectra with angular resolution were successfully detected with a velocity-map imaging spectrometer. However, the impact of the infrared dressing field in the photoelectron spectra could not be observed. We discuss several issues that potentially hampered these observations and suggest corresponding setup improvements