1,629 research outputs found
Anomalous relaxation kinetics and charge density wave correlations in underdoped BaPb1-xBixO3
Superconductivity often emerges in proximity of other symmetry-breaking
ground states, such as antiferromagnetism or charge-density-wave (CDW) order.
However, the subtle inter-relation of these phases remains poorly understood,
and in some cases even the existence of short-range correlations for
superconducting compositions is uncertain. In such circumstances, ultrafast
experiments can provide new insights, by tracking the relaxation kinetics
following excitation at frequencies related to the broken symmetry state. Here,
we investigate the transient terahertz conductivity of BaPb1-xBixO3 - a
material for which superconductivity is adjacent to a competing CDW phase -
after optical excitation tuned to the CDW absorption band. In insulating BaBiO3
we observed an increase in conductivity and a subsequent relaxation, which are
consistent with quasiparticles injection across a rigid semiconducting gap. In
the doped compound BaPb0.72Bi0.28O3 (superconducting below Tc=7K), a similar
response was also found immediately above Tc. This observation evidences the
presence of a robust gap up to T=40 K, which is presumably associated with
short-range CDW correlations. A qualitatively different behaviour was observed
in the same material fo T>40 K. Here, the photo-conductivity was dominated by
an enhancement in carrier mobility at constant density, suggestive of melting
of the CDW correlations rather than excitation across an optical gap. The
relaxation displayed a temperature dependent, Arrhenius-like kinetics,
suggestive of the crossing of a free-energy barrier between two phases. These
results support the existence of short-range CDW correlations above Tc in
underdoped BaPb1-xBixO3, and provide new information on the dynamical interplay
between superconductivity and charge order.Comment: 19 pages, 4 figure
A river model of space
Within the theory of general relativity gravitational phenomena are usually
attributed to the curvature of four-dimensional spacetime. In this context we
are often confronted with the question of how the concept of ordinary physical
three-dimensional space fits into this picture. In this work we present a
simple and intuitive model of space for both the Schwarzschild spacetime and
the de Sitter spacetime in which physical space is defined as a specified set
of freely moving reference particles. Using a combination of orthonormal basis
fields and the usual formalism in a coordinate basis we calculate the physical
velocity field of these reference particles. Thus we obtain a vivid description
of space in which space behaves like a river flowing radially toward the
singularity in the Schwarzschild spacetime and radially toward infinity in the
de Sitter spacetime. We also consider the effect of the river of space upon
light rays and material particles and show that the river model of space
provides an intuitive explanation for the behavior of light and particles at
and beyond the event horizons associated with these spacetimes.Comment: 22 pages, 5 figure
Pressure tuning of light-induced superconductivity in K3C60
Optical excitation at terahertz frequencies has emerged as an effective means
to manipulate complex solids dynamically. In the molecular solid K3C60,
coherent excitation of intramolecular vibrations was shown to transform the
high temperature metal into a non-equilibrium state with the optical
conductivity of a superconductor. Here we tune this effect with hydrostatic
pressure, and we find it to disappear around 0.3 GPa. Reduction with pressure
underscores the similarity with the equilibrium superconducting phase of K3C60,
in which a larger electronic bandwidth is detrimental for pairing. Crucially,
our observation excludes alternative interpretations based on a high-mobility
metallic phase. The pressure dependence also suggests that transient, incipient
superconductivity occurs far above the 150 K hypothesised previously, and
rather extends all the way to room temperature.Comment: 33 pages, 17 figures, 2 table
Dynamics of photo-induced ferromagnetism in oxides with orbital degeneracy
By using intense coherent electromagnetic radiation, it may be possible to manipulate the properties of quantum materials very quickly, or even induce new and potentially useful phases that are absent in equilibrium. For instance, ultrafast control of magnetic dynamics is crucial for a number of proposed spintronic devices and can also shed light on the possible dynamics of correlated phases out of equilibrium. Inspired by recent experiments on spin-orbital ferromagnet YTiO3 we consider the nonequilibrium dynamics of Heisenberg ferromagnetic insulator with low-lying orbital excitations. We model the dynamics of the magnon excitations in this system following an optical pulse which resonantly excites infrared-active phonon modes. As the phonons ring down they can dynamically couple the orbitals with the low-lying magnons, leading to a dramatically modified effective bath for the magnons. We show this transient coupling can lead to a dynamical acceleration of the magnetization dynamics, which is otherwise bottlenecked by small anisotropy. Exploring the parameter space more we find that the magnon dynamics can also even completely reverse, leading to a negative relaxation rate when the pump is blue-detuned with respect to the orbital bath resonance. We therefore show that by using specially targeted optical pulses, one can exert a much greater degree of control over the magnetization dynamics, allowing one to optically steer magnetic order in this system. We conclude by discussing interesting parallels between the magnetization dynamics we find here and recent experiments on photo-induced superconductivity, where it is similarly observed that depending on the initial pump frequency, an apparent metastable superconducting phase emerges
Achieving geodetic motion for LISA test masses: ground testing result
The low-frequency resolution of space-based gravitational wave observatories
such as LISA (Laser Interferometry Space Antenna) hinges on the orbital purity
of a free-falling reference test mass inside a satellite shield. We present
here a torsion pendulum study of the forces that will disturb an orbiting test
mass inside a LISA capacitive position sensor. The pendulum, with a measured
torque noise floor below 10 fNm/sqrt{Hz} from 0.6 to 10 mHz, has allowed
placement of an upper limit on sensor force noise contributions, measurement of
the sensor electrostatic stiffness at the 5% level, and detection and
compensation of stray DC electrostatic biases at the mV level.Comment: 4 pages (revtex4) with 4 figure
Phase-Based Binocular Perception of Motion in Depth: Cortical-Like Operators and Analog VLSI Architectures
We present a cortical-like strategy to obtain reliable estimates of the motions of objects in a scene toward/away from the observer (motion in depth), from local measurements of binocular parameters derived from direct comparison of the results of monocular spatiotemporal filtering operations performed on stereo image pairs. This approach is suitable for a hardware implementation, in which such parameters can be gained via a feedforward computation (i.e., collection, comparison, and punctual operations) on the outputs of the nodes of recurrent VLSI lattice networks, performing local computations. These networks act as efficient computational structures for embedded analog filtering operations in smart vision sensors. Extensive simulations on both synthetic and real-world image sequences prove the validity of the approach that allows to gain high-level information about the 3D structure of the scene, directly from sensorial data, without resorting to explicit scene reconstruction
Generalized observers and velocity measurements in General Relativity
To resolve some unphysical interpretations related to velocity measurements
by static observers, we discuss the use of generalized observer sets, give a
prescription for defining the speed of test particles relative to those
observers and show that, for any locally inertial frame, the speed of a freely
falling material particle is always less than the speed of light at the
Schwarzschild black hole surface.Comment: 20 pages, 1 figure, submitted to General Relativity and Gravitatio
Softening of the insulating phase near Tc for the photo-induced insulator-to-metal phase transition in vanadium dioxide
We use optical-pump terahertz-probe spectroscopy to investigate the
near-threshold behavior of the photoinduced insulator-to-metal (IM) transition
in vanadium dioxide thin films. Upon approaching Tc a reduction in the fluence
required to drive the IM transition is observed, consistent with a softening of
the insulating state due to an increasing metallic volume fraction (below the
percolation limit). This phase coexistence facilitates the growth of a
homogeneous metallic conducting phase following superheating via
photoexcitation. A simple dynamic model using Bruggeman effective medium theory
describes the observed initial condition sensitivity.Comment: accepted for publication in Physical Review Letter
Ultrafast changes in lattice symmetry probed by coherent phonons
The electronic and structural properties of a material are strongly
determined by its symmetry. Changing the symmetry via a photoinduced phase
transition offers new ways to manipulate material properties on ultrafast
timescales. However, in order to identify when and how fast these phase
transitions occur, methods that can probe the symmetry change in the time
domain are required. We show that a time-dependent change in the coherent
phonon spectrum can probe a change in symmetry of the lattice potential, thus
providing an all-optical probe of structural transitions. We examine the
photoinduced structural phase transition in VO2 and show that, above the phase
transition threshold, photoexcitation completely changes the lattice potential
on an ultrafast timescale. The loss of the equilibrium-phase phonon modes
occurs promptly, indicating a non-thermal pathway for the photoinduced phase
transition, where a strong perturbation to the lattice potential changes its
symmetry before ionic rearrangement has occurred.Comment: 14 pages 4 figure
Quantum interference between charge excitation paths in a solid state Mott insulator
The competition between electron localization and de-localization in Mott
insulators underpins the physics of strongly-correlated electron systems.
Photo-excitation, which re-distributes charge between sites, can control this
many-body process on the ultrafast timescale. To date, time-resolved studies
have been performed in solids in which other degrees of freedom, such as
lattice, spin, or orbital excitations come into play. However, the underlying
quantum dynamics of bare electronic excitations has remained out of reach.
Quantum many-body dynamics have only been detected in the controlled
environment of optical lattices where the dynamics are slower and lattice
excitations are absent. By using nearly-single-cycle near-IR pulses, we have
measured coherent electronic excitations in the organic salt ET-F2TCNQ, a
prototypical one-dimensional Mott Insulator. After photo-excitation, a new
resonance appears on the low-energy side of the Mott gap, which oscillates at
25 THz. Time-dependent simulations of the Mott-Hubbard Hamiltonian reproduce
the oscillations, showing that electronic delocalization occurs through quantum
interference between bound and ionized holon-doublon pairs.Comment: 4 figures and supplementary informatio
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