50 research outputs found

    Avalanches from charged domain wall motion in BaTiO3 during ferroelectric switching

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    We report two methods for direct observations of avalanches in ferroelectric materials during the motion of domain walls. In the first method, we use optical imaging techniques to derive changes in domain structures under an electric field. All changes occur through small jumps (jerks) that obey avalanche statistics. In the second method, we analyze jerks by their displacement current. Both methods reveal a power law distribution with an energy exponent of 1.6, in agreement with previous acoustic emission measurements, and integrated mean field theory. This new combination of methods allows us to probe both polarization and strain variations during the motion of domain walls and can be used for a much wider class of ferroelectrics, including ceramic samples, than acoustic emission

    Untangling the contributions of cerium and iron to the magnetism of Ce-doped yttrium iron garnet

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    The remarkable magnetic properties of yttrium iron garnets (YIGs) underpin the use of these materials in a broad scope of spintronic and photonic applications. In particular, the addition of rare earth metals in the structure enhances to a great extent the magneto-optical activity, which is beneficial for the development of nonreciprocal optical devices. Exploiting the wavelength selectivity of magneto-optics, we have identified a range of frequencies at which one can unravel the individual contributions to the magnetism and gyrotropic response arising from cerium and iron. We envision that this outcome may pave the way to further experiments to assess quantitatively the effect on the optical properties of rare earth incorporation into YIG.This work was supported by the Spanish Government by the MAT2011-29269-C03, MAT2014-56063-C2-1-R, and the Severo Ochoa SEV-2015-0496 Projects and the Generalitat de Catalunya (2014 SGR 734 Project). B.C. acknowledges his grant FPI BES-2012-059023 and R.C. acknowledges his fellowship from CNPq - Brazil. S.G., M.O., and R.G. thank T. Brenninger and E. Zamburg for technical support. We also acknowledge the contribution of C. Rubio in preliminary structural and magnetic characterization of thin films as well as Dr. F. Sanchez for scientific guiding and discussions on materials issues.Peer Reviewe

    Avalanche criticality during ferroelectric/ferroelastic switching

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    Field induced domain wall displacements define ferroelectric/ferroelastic hysteresis loops, which are at the core of piezoelectric, magnetoelectric and memristive devices. These collective displacements are scale invariant jumps with avalanche characteristics. Here, we analyse the spatial distribution of avalanches in ferroelectrics with different domain and transformation patterns: Pb(Mg1/3Nb2/3)O3–PbTiO3 contains complex domains with needles and junction patterns, while BaTiO3 has parallel straight domains. Nevertheless, their avalanche characteristics are indistinguishable. The energies, areas and perimeters of the switched regions are power law distributed with exponents close to predicted mean field values. At the coercive field, the area exponent decreases, while the fractal dimension increases. This fine structure of the switching process has not been detected before and suggests that switching occurs via criticality at the coercive field with fundamentally different switching geometries at and near this critical point. We conjecture that the domain switching process in ferroelectrics is universal at the coercive field

    A Novel chip for cyclic stretch and intermittent hypoxia cell exposures mimicking obstructive sleep apnea

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    Intermittent hypoxia (IH), a hallmark of obstructive sleep apnea (OSA), plays a critical role in the pathogenesis of OSA-associated morbidities, especially in the cardiovascular and respiratory systems. Oxidative stress and inflammation induced by IH are suggested as main contributors of end-organ dysfunction in OSA patients and animal models. Since the molecular mechanisms underlying these in vivo pathological responses remain poorly understood, implementation of experimental in vitro cell-based systems capable of inducing high-frequency IH would be highly desirable. Here, we describe the design, fabrication, and validation of a versatile chip for subjecting cultured cells to fast changes in gas partial pressure and to cyclic stretch. The chip is fabricated with polydimethylsiloxane (PDMS) and consists of a cylindrical well-covered by a thin membrane. Cells cultured on top of the membrane can be subjected to fast changes in oxygen concentration (equilibrium time similar to 6 s). Moreover, cells can be subjected to cyclic stretch at cardiac or respiratory frequencies independently or simultaneously. Rat bone marrow-derived mesenchymal stem cells (MSCs) exposed to IH mimicking OSA and cyclic stretch at cardiac frequencies revealed that hypoxia-inducible factor 1 alpha (HIF-1 alpha) expression was increased in response to both stimuli. Thus, the chip provides a versatile tool for the study of cellular responses to cyclical hypoxia and stretch

    Qu­antification of propagating and standing surface acoustic waves by stroboscopic X-ray photoemission electron microscopy

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    The quantification of surface acoustic waves (SAWs) in LiNbO3 piezoelectric crystals by stroboscopic X-ray photoemission electron microscopy (XPEEM), with a temporal smearing below 80 ps and a spatial resolution below 100 nm, is reported. The contrast mechanism is the varying piezoelectric surface potential associated with the SAW phase. Thus, kinetic energy spectra of photoemitted secondary electrons measure directly the SAW electrical amplitude and allow for the quantification of the associated strain. The stroboscopic imaging combined with a deliberate detuning allows resolving and quantifying the respective standing and propagating components of SAWs from a superposition of waves. Furthermore, standing-wave components can also be imaged by low-energy electron microscopy (LEEM). Our method opens the door to studies that quantitatively correlate SAWs excitation with a variety of sample electronic, magnetic and chemical properties
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