138 research outputs found
X-ray method to study temperature-dependent stripe domains in MnAs/GaAs(001)
MnAs films grown on GaAs (001) exhibit a progressive transition between
hexagonal (ferromagnetic) and orthorhombic (paramagnetic) phases at wide
temperature range instead of abrupt transition during the first-order phase
transition. The coexistence of two phases is favored by the anisotropic strain
arising from the constraint on the MnAs films imposed by the substrate. This
phase coexistence occurs in ordered arrangement alternating periodic terrace
steps. We present here a method to study the surface morphology throughout this
transition by means of specular and diffuse scattering of soft x-rays, tuning
the photon energy at the Mn 2p resonance. The results show the long-range
arrangement of the periodic stripe-like structure during the phase coexistence
and its period remains constant, in agreement with previous results using other
techniques.Comment: 4 pages, 4 figures, submitted to Applied Physics Letter
Magnetic reconfiguration of MnAs/GaAs(001) observed by Magnetic Force Microscopy and Resonant Soft X-ray Scattering
We investigated the thermal evolution of the magnetic properties of MnAs
epitaxial films grown on GaAs(001) during the coexistence of
hexagonal/orthorhombic phases using polarized resonant (magnetic) soft X-ray
scattering and magnetic force microscopy. The results of the diffuse satellite
X-ray peaks were compared to those obtained by magnetic force microscopy and
suggest a reorientation of ferromagnetic terraces as temperature rises. By
measuring hysteresis loops at these peaks we show that this reorientation is
common to all ferromagnetic terraces. The reorientation is explained by a
simple model based on the shape anisotropy energy. Demagnetizing factors were
calculated for different configurations suggested by the magnetic images. We
noted that the magnetic moments flip from an in-plane mono-domain orientation
at lower temperatures to a three-domain out-of-plane configuration at higher
temperatures. The transition was observed when the ferromagnetic stripe width L
is equal to 2.9 times the film thickness d. This is in good agreement with the
expected theoretical value of L = 2.6d.Comment: 16 pages in PD
VUV and X-ray coherent light with tunable polarization from single-pass free-electron lasers
Tunable polarization over a wide spectral range is a required feature of
light sources employed to investigate the properties of local symmetry in both
condensed and low-density matter. Among new-generation sources, free-electron
lasers possess a unique combination of very attractive features, as they allow
to generate powerful and coherent ultra-short optical pulses in the VUV and
X-ray spectral range. However, the question remains open about the possibility
to freely vary the light polarization of a free-electron laser, when the latter
is operated in the so-called nonlinear harmonic-generation regime. In such
configuration, one collects the harmonics of the free-electron laser
fundamental emission, gaining access to the shortest possible wavelengths the
device can generate. In this letter we provide the first experimental
characterization of the polarization of the harmonic light produced by a
free-electron laser and we demonstrate a method to obtain tunable polarization
in the VUV and X-ray spectral range. Experimental results are successfully
compared to those obtained using a theoretical model based on the paraxial
solution of Maxwell's equations. Our findings can be expected to have a deep
impact on the design and realization of experiments requiring full control of
light polarization to explore the symmetry properties of matter samples
Synchrotron radiation photoionization mass spectrometry of laser ablated species
The present paper describes an experimental apparatus suitable to create and study free clusters by combining laser ablation and synchrotron radiation. First tests on sulfur samples, S, showed the production, through laser ablation, of neutral Sn clusters (n = 1–8). These clusters were ionized using synchrotron radiation at photon energies from 160 eV to 175 eV, across the S 2p core edge. The feasibility of such combined ablation–synchrotron radiation experiments is demonstrated, opening new possibilities on the investigation of free clusters and radical
Two-colour generation in a chirped seeded Free-Electron Laser
We present the experimental demonstration of a method for generating two
spectrally and temporally separated pulses by an externally seeded, single-pass
free-electron laser operating in the extreme-ultraviolet spectral range. Our
results, collected on the FERMI@Elettra facility and confirmed by numerical
simulations, demonstrate the possibility of controlling both the spectral and
temporal features of the generated pulses. A free-electron laser operated in
this mode becomes a suitable light source for jitter-free, two-colour
pump-probe experiments
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