Global large-scale stratosphere–troposphere exchange in modern reanalyses

Stratosphere–troposphere exchange (STE) has important impacts on the chemical and radiative properties of the upper troposphere and lower stratosphere. This study presents a 15-year climatology of global large-scale STE from four modern reanalyses: ERA-Interim, JRA-55, MERRA-2, and MERRA. STE is separated into three regions (tropics, subtropics, and extratropics) and two transport directions (stratosphere-to-troposphere transport or STT and troposphere-to-stratosphere transport or TST) in an attempt to identify the significance of known transport mechanisms. The extratropics and tropics are separated by the tropopause break. Any STE occurring between the tropics and the extratropics through the tropopause break is considered subtropical exchange (i.e., in the vicinity of the subtropical jet). In addition, this study employs a method to identify STE as that which crosses the lapse-rate tropopause (LRT), while most previous studies have used a potential vorticity (PV) isosurface as the troposphere–stratosphere boundary. PV-based and LRT-based STE climatologies are compared using the ERA-Interim reanalysis output. The comparison reveals quantitative and qualitative differences, particularly for TST in the polar regions. Based upon spatiotemporal integrations, we find STE to be STT dominant in ERA-Interim and JRA-55 and TST dominant in MERRA and MERRA-2. The sources of the differences are mainly attributed to inconsistencies in the representation of STE in the subtropics and extratropics. Time series during the 15-year analysis period show long-term changes that are argued to correspond with changes in the Brewer–Dobson circulation

Global tropopause altitudes in radiosondes and reanalyses

Accurate depictions of the tropopause and its changes are important for studies on stratosphere–troposphere exchange and climate change. Here, the fidelity of primary lapse-rate tropopause altitudes and double tropopause frequencies in four modern reanalyses (ERA-Interim, JRA-55, MERRA-2, and CFSR) is examined using global radiosonde observations. In addition, long-term trends (1981–2015) in these tropopause properties are diagnosed in both the reanalyses and radiosondes. It is found that reanalyses reproduce observed tropopause altitudes with little bias (typically less than ±150&thinsp;m) and error comparable to the model vertical resolution. All reanalyses underestimate the double tropopause frequency (up to 30&thinsp;% lower than observed), with the largest biases found in JRA-55 and the smallest in CFSR. The underestimates in double tropopause frequency are primarily attributable to the coarse vertical resolution of the reanalyses. Significant increasing trends in both tropopause altitude (40–120&thinsp;m per decade) and double tropopause frequency (≥3&thinsp;% per decade) were found in both the radiosonde observations and the reanalyses over the 35-year analysis period (1981–2015). ERA-Interim, JRA-55, and MERRA-2 broadly reproduce the patterns and signs of observed significant trends, while CFSR is inconsistent with the remaining datasets. Trends were diagnosed in both the native Eulerian coordinate system of the reanalyses (fixed longitude and latitude) and in a coordinate system where latitude is defined relative to the mean latitude of the tropopause break (the discontinuity in tropopause altitude between the tropics and extratropics) in each hemisphere. The coordinate relative to the tropopause break facilitates the evaluation of tropopause behavior within the tropical and extratropical reservoirs and revealed significant differences in trend estimates compared to the traditional Eulerian analysis. Notably, increasing tropopause altitude trends were found to be of greater magnitude in coordinates relative to the tropopause break, and increasing double tropopause frequency trends were found to occur primarily poleward of the tropopause break in each hemisphere.</p

Commentary on using equivalent latitude in the upper troposphere and lower stratosphere

We discuss the use of potential vorticity (PV) based equivalent latitude (EqLat) and potential temperature (&lt;i&gt;&amp;theta;&lt;/i&gt;) coordinates in the upper troposphere and lower stratosphere (UTLS) for chemical transport studies. The main objective is to provide a cautionary note on using EqLat-&lt;i&gt;&amp;theta;&lt;/i&gt; coordinates for aggregating chemical tracers in the UTLS. Several examples are used to show 3-D distributions of EqLat together with chemical constituents for a range of &lt;i&gt;&amp;theta;&lt;/i&gt;. We show that the use of PV-&lt;i&gt;&amp;theta;&lt;/i&gt; coordinates may not be suitable for several reasons when tropospheric processes are an important part of a study. Due to the different static stability structures between the stratosphere and troposphere, the use of &lt;i&gt;&amp;theta;&lt;/i&gt; as a vertical coordinate does not provide equal representations of the UT and LS. Since the &lt;i&gt;&amp;theta;&lt;/i&gt; surfaces in the troposphere often intersect the surface of the Earth, the &lt;i&gt;&amp;theta;&lt;/i&gt; variable does not work well distinguishing the UT from the boundary layer when used globally as a vertical coordinate. We further discuss the duality of PV/EqLat as a tracer versus as a coordinate variable. Using an example, we show that while PV/EqLat serves well as a transport tracer in the UTLS region, it may conceal the chemical structure associated with wave breaking when used as a coordinate to average chemical tracers. Overall, when choosing these coordinates, considerations need to be made not only based on the time scale of PV being a conservative tracer, but also the specific research questions to be addressed

It's Time for Color Vision Deficiency Friendly Color Maps in the Radar Community

Color Vision Deficiency (CVD) is a decreased ability to discern between particular colors. 8% of men and 0.4% of women have some form of CVD. An informal poll of AGU and AMS twitter followers yielded 10% of 70 respondents self identifying as having CVD. When presenting data on a two-dimensional plane it is common to use colors to represent values, the mapping between values and colors is known as a colormap. Colormap choice is personal and is influenced by: (1) Ability to highlight scientifically interesting data. (2) Institutional choices (supervisor insists on a certain colormap). (3) Domain dominance of a particular colormap (common in the radar community). Colormap choice should be influenced by: (1) Ability to highlight scientifically interesting data. (2) Perceptual uniformity (thus not creating artificial structure). (3) Approachability by those with visual impairments (CVD). (4) Ideally, but not always achievable, reproducibility in greyscale

Wet scavenging of soluble gases in DC3 deep convective storms using WRF-Chem simulations and aircraft observations

We examine wet scavenging of soluble trace gases in storms observed during the Deep Convective Clouds and Chemistry (DC3) field campaign. We conduct high-resolution simulations with the Weather Research and Forecasting model with Chemistry (WRF-Chem) of a severe storm in Oklahoma. The model represents well the storm location, size, and structure as compared with Next Generation Weather Radar reflectivity, and simulated CO transport is consistent with aircraft observations. Scavenging efficiencies (SEs) between inflow and outflow of soluble species are calculated from aircraft measurements and model simulations. Using a simple wet scavenging scheme, we simulate the SE of each soluble species within the error bars of the observations. The simulated SEs of all species except nitric acid (HNO_3) are highly sensitive to the values specified for the fractions retained in ice when cloud water freezes. To reproduce the observations, we must assume zero ice retention for formaldehyde (CH_2O) and hydrogen peroxide (H_2O_2) and complete retention for methyl hydrogen peroxide (CH_3OOH) and sulfur dioxide (SO_2), likely to compensate for the lack of aqueous chemistry in the model. We then compare scavenging efficiencies among storms that formed in Alabama and northeast Colorado and the Oklahoma storm. Significant differences in SEs are seen among storms and species. More scavenging of HNO_3 and less removal of CH_3OOH are seen in storms with higher maximum flash rates, an indication of more graupel mass. Graupel is associated with mixed-phase scavenging and lightning production of nitrogen oxides (NO_x), processes that may explain the observed differences in HNO_3 and CH_3OOH scavenging

Convective transport and scavenging of peroxides by thunderstorms observed over the central U.S. during DC3

One of the objectives of the Deep Convective Clouds and Chemistry (DC3) field experiment was to determine the scavenging of soluble trace gases by thunderstorms. We present an analysis of scavenging of hydrogen peroxide (H_2O_2) and methyl hydrogen peroxide (CH_3OOH) from six DC3 cases that occurred in Oklahoma and northeast Colorado. Estimates of H_2O_2 scavenging efficiencies are comparable to previous studies ranging from 79 to 97% with relative uncertainties of 5–25%. CH_3OOH scavenging efficiencies ranged from 12 to 84% with relative uncertainties of 18–558%. The wide range of CH_3OOH scavenging efficiencies is surprising, as previous studies suggested that CH_3OOH scavenging efficiencies would be <10%. Cloud chemistry model simulations of one DC3 storm produced CH_3OOH scavenging efficiencies of 26–61% depending on the ice retention factor of CH_3OOH during cloud drop freezing, suggesting ice physics impacts CH_3OOH scavenging. The highest CH_3OOH scavenging efficiencies occurred in two severe thunderstorms, but there is no obvious correlation between the CH_3OOH scavenging efficiency and the storm thermodynamic environment. We found a moderate correlation between the estimated entrainment rates and CH_3OOH scavenging efficiencies. Changes in gas-phase chemistry due to lightning production of nitric oxide and aqueous-phase chemistry have little effect on CH_3OOH scavenging efficiencies. To determine why CH_3OOH can be substantially removed from storms, future studies should examine effects of entrainment rate, retention of CH_3OOH in frozen cloud particles during drop freezing, and lightning-NO_x production

Summary and Highlights of the SPARC-Reanalysis Intercomparison Project

The climate research community uses global atmospheric reanalysis data sets to understand a wide range of processes and variability in the atmosphere; they are a particularly powerful tool for studying phenomena that cannot be directly observed. Different reanalyses may give very different results for the same diagnostics. The Stratosphere troposphere Processes And their Role in Climate (SPARC) Reanalysis Intercomparison Project (S-RIP) is a coordinated activity to compare key diagnostics that are important for stratospheric processes and their tropospheric connections among available reanalyses. S-RIP has been identifying differences among reanalyses and their underlying causes, providing guidance on appropriate usage of reanalysis products in scientific studies (particularly those of relevance to SPARC), and contributing to future improvements in the reanalysis products by establishing collaborative links between reanalysis centres and data users. S-RIP emphasizes diagnostics of the upper troposphere, stratosphere, and lower mesosphere. The draft S-RIP final report is expected to be completed in 2018. This poster gives a summary of the S-RIP project and presents highlights including results on the Brewer-Dobson circulation, stratosphere/troposphere dynamical coupling, the extra-tropical upper troposphere / lower stratosphere, the tropical tropopause layer, the quasi-biennial oscillation, lower stratospheric polar processing, and the upper stratosphere/lower mesosphere

Effects of Scavenging, Entrainment, and Aqueous Chemistry on Peroxides and Formaldehyde in Deep Convective Outflow over the Central and Southeast U.S.

Deep convective transport of gaseous precursors to ozone (O3) and aerosols to the upper troposphere is affected by liquid- and mixed-phase scavenging, entrainment of free tropospheric air, and aqueous chemistry. The contributions of these processes are examined using aircraft measurements obtained in storm inflow and outflow during the 2012 Deep Convective Clouds and Chemistry (DC3) experiment combined with high resolution (dx <= 3 km) WRF-Chem simulations of a severe storm, an airmass storm, and a mesoscale convective system (MCS). The simulation results for the MCS suggest that formaldehyde (CH2O) is not retained in ice when cloud water freezes, in agreement with previous studies of the severe storm. By analyzing WRF-Chem trajectories, the effects of scavenging, entrainment, and aqueous chemistry on outflow mixing ratios of CH2O, methyl hydroperoxide (CH3OOH), and hydrogen peroxide (H2O2) are quantified. Liquid-phase microphysical scavenging was the dominant process reducing CH2O and H2O2 outflow mixing ratios in all three storms. Aqueous chemistry did not significantly affect outflow mixing ratios of all three species. In the severe storm and MCS, the higher than expected reductions in CH3OOH mixing ratios in the storm cores were primarily due to entrainment of low background CH3OOH. In the airmass storm, lower CH3OOH and H2O2 scavenging efficiencies (SEs) than in the MCS were partly due to entrainment of higher background CH3OOH and H2O2. Overestimated rain and hail production in WRF-Chem reduces the confidence in ice retention fraction values determined for the peroxides and CH2O

Vertical Transport, Entrainment, and Scavenging Processes Affecting Trace Gases in a Modeled and Observed SEAC⁴RS Case Study

The convectively driven transport of soluble trace gases from the lower to the upper troposphere can occur on timescales of less than an hour, and recent studies suggest that microphysical scavenging is the dominant removal process of tropospheric ozone precursors. We examine the processes responsible for vertical transport, entrainment, and scavenging of soluble ozone precursors (formaldehyde and peroxides) for midlatitude convective storms sampled on 2 September 2013 during the Studies of Emissions, Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC⁴RS) study. Cloud‐resolving simulations using the Weather Research and Forecasting with Chemistry model combined with aircraft measurements were performed to understand the effect of entrainment, scavenging efficiency (SE), and ice physics processes on these trace gases. Analysis of the observations revealed that the SEs of formaldehyde (43–53%) and hydrogen peroxide (~80–90%) were consistent between SEAC⁴RS storms and the severe convection observed during the Deep Convective Clouds and Chemistry Experiment (DC3) campaign. However, methyl hydrogen peroxide SE was generally smaller in the SEAC⁴RS storms (4%–27%) compared to DC3 convection. Predicted ice retention factors exhibit different values for some species compared to DC3, and we attribute these differences to variations in net precipitation production. The analyses show that much larger production of precipitation between condensation and freezing levels for DC3 severe convection compared to smaller SEAC⁴RS storms is largely responsible for the lower amount of soluble gases transported to colder temperatures, reducing the amount of soluble gases which eventually interact with cloud ice particles