283 research outputs found
Probing quantum nanostructures with near-field optical microscopy and (vice versa)
A theory is presented to show how near-field optical microscopy can be used
to probe quantum nanostructures. Calculations are done for a quantum dot.
Results for different tip/dot configurations and sizes show that near-field
excitation can enhance light-hole transitions, excite selection-rule breaking
transitions with rates comparable to allowed transitions, and map electron-hole
pair wave functions. Conversely, dot response can be used to characterize tip
near-fields.Comment: 8 pages of ReVTex, 5 ps figures, submitted to Appl. Phys. Let
Diacritical study of light, electrons, and sound scattering by particles and holes
We discuss the differences and similarities in the interaction of scalar and
vector wave-fields with particles and holes. Analytical results are provided
for the transmission of isolated and arrayed small holes as well as surface
modes in hole arrays for light, electrons, and sound. In contrast to the
optical case, small-hole arrays in perforated perfect screens cannot produce
acoustic or electronic surface-bound states. However, unlike electrons and
light, sound is transmitted through individual holes approximately in
proportion to their area, regardless their size. We discuss these issues with a
systematic analysis that allows exploring both common properties and unique
behavior in wave phenomena for different material realizations.Comment: 3 figure
Extension of Bethe's diffraction model to conical Geometry: application to near field optics
The generality of the Bethe's two dipole model for light diffraction through
a subwavelength aperture in a conducting plane is studied in the radiation zone
for coated conical fiber tips as those used in near field scanning optical
microscopy. In order to describe the angular radiated power of the tip
theoretically, we present a simple, analytical model for small apertures
(radius < 40 nm) based on a multipole expansion. Our model is able to reproduce
the available experimental results. It proves relatively insensitive to cone
angle and aperture radius and contains, as a first approximation, the empirical
two-dipole model proposed earlier
Diffraction of light by a planar aperture in a metallic screen
We present a complete derivation of the formula of Smythe [Phys.Rev.72, 1066
(1947)] giving the electromagnetic field diffracted by an aperture created in a
perfectly conducting plane surface. The reasoning, valid for any excitating
field and any hole shape, makes use only of the free scalar Green function for
the Helmoltz equation without any reference to a Green dyadic formalism. We
compare our proof with the one previously given by Jackson and connect our
reasoning to the general Huygens Fresnel theorem.Comment: J. Math. Phys. 47, 072901 (2006
Evaluation of thermal evaporation conditions used in coating aluminum on near-field fiber-optic probes
This is the published version, also available here: http://dx.doi.org/10.1063/1.1148836.The effects that the thermal evaporation conditions have on the roughness of aluminum-coated near-field fiber-optic probes were investigated using the high-resolution capabilities of atomic force microscopy. The coating conditions studied include the effects of background gas composition, base vacuum pressure, and aluminum evaporation rate. The effects of aging on the aluminum-coated tips were also evaluated. The results from topography measurements of the resulting aluminumfilm indicated that the most dramatic improvements in the tip coatings can be achieved using high aluminum evaporation rates at base vacuum pressures below 10−5 Torr. These results agree with other studies on thin aluminumfilms and reflect a decrease in oxide formation. For demanding applications of near-field microscopy requiring maximal resolution, the results presented here indicate that it may also be necessary to reduce oxygen and/or water from the vacuum chamber prior to coating
Multipole Expansion of Bremsstrahlung in Intermediate Energy Heavy Ion Collisions
Using a multipole expansion of the radiated field generated by a classical
electric current, we present a way to interprete the bremsstrahlung spectra of
low energy heavy ion collisions. We perform the calculation explicitely for the
system ^{12}C+ ^{12}C at 84AMeV and compare the result with the experimental
data of E. Grosse et al. Using simple model assumptions for the electromagnetic
source current we are able to describe the measured data in terms of coherent
photon emission. In this context, the information contained in the measured
data is discussed.Comment: LaTex, 4 Figure
Remote optical addressing of single nano-objects
We present a scheme for remotely addressing single nano-objects by means of
near-field optical microscopy that makes only use of one of the most
fundamental properties of electromagnetic radiation: its polarization. A medium
containing optically active nano-objects is covered with a thin metallic film
presenting sub-wavelength holes. When the optical tip is positioned some
distance away from a hole, surface plasmons in the metal coating are generated
which, by turning the polarization plane of the excitation light, transfer the
excitation towards a chosen hole and induce emission from the underlying
nano-objects. The method, easily applicable to other systems, is demonstrated
for single quantum dots (QDs) at low temperature. It may become a valuable tool
for future optical applications in the nanoworld
Theory of imaging a photonic crystal with transmission near-field optical microscopy
While near-field scanning optical microscopy (NSOM) can provide optical
images with resolution much better than the diffraction limit, analysis and
interpretation of these images is often difficult. We present a theory of
imaging with transmission NSOM that includes the effects of tip field,
tip/sample coupling, light propagation through the sample and light collection.
We apply this theory to analyze experimental NSOM images of a nanochannel glass
(NCG) array obtained in transmission mode. The NCG is a triangular array of
dielectric rods in a dielectric glass matrix with a two-dimensional photonic
band structure. We determine the modes for the NCG photonic crystal and
simulate the observed data. The calculations show large contrast at low
numerical aperture (NA) of the collection optics and detailed structure at high
NA consistent with the observed images. We present calculations as a function
of NA to identify how the NCG photonic modes contribute to and determine the
spatial structure in these images. Calculations are presented as a function of
tip/sample position, sample index contrast and geometry, and aperture size to
identify the factors that determine image formation with transmission NSOM in
this experiment.Comment: 28 pages of ReVTex, 14 ps figures, submitted to Phys. Rev.
Diffraction by a small aperture in conical geometry: Application to metal coated tips used in near-field scanning optical microscopy
Light diffraction through a subwavelength aperture located at the apex of a
metallic screen with conical geometry is investigated theoretically. A method
based on a multipole field expansion is developed to solve Maxwell's equations
analytically using boundary conditions adapted both for the conical geometry
and for the finite conductivity of a real metal. The topological properties of
the diffracted field are discussed in detail and compared to those of the field
diffracted through a small aperture in a flat screen, i. e. the Bethe problem.
The model is applied to coated, conically tapered optical fiber tips that are
used in Near-Field Scanning Optical Microscopy. It is demonstrated that such
tips behave over a large portion of space like a simple combination of two
effective dipoles located in the apex plane (an electric dipole and a magnetic
dipole parallel to the incident fields at the apex) whose exact expressions are
determined. However, the large "backward" emission in the P plane - a salient
experimental fact that remained unexplained so far - is recovered in our
analysis which goes beyond the two-dipole approximation.Comment: 21 pages, 6 figures, published in PRE in 200
Probing single molecule orientations in model lipid membranes with near-field scanning optical microscopy
This is the published version, also available here: http://dx.doi.org/10.1063/1.481367.Single molecule near-field fluorescence measurements are utilized to characterize the molecular level structure in Langmuir–Blodgett monolayers of L-α-dipalmitoylphosphatidylcholine (DPPC).Monolayers incorporating 3×10−4 mol % of the fluorescent lipid analog N-(6-tetramethylrhodaminethiocarbamoyl)-1,2-dihexadecanoyl-sn- glycero-3-phosphoethanolamine, triethylammonium salt (TRITC–DHPE) are transferred onto a freshly cleaved mica surface at low (π=8 mN/m) and high (π=30 mN/m)surfacepressures. The near-field fluorescence images exhibit shapes in the single molecule images that are indicative of the lipid analog probe orientation within the films. Modeling the fluorescence patterns yields the single molecule tilt angle distribution in the monolayers which indicates that the majority of the molecules are aligned with their absorption dipole moment pointed approximately normal to the membrane plane. Histograms of the data indicate that the average orientation of the absorption dipole moment is 2.2° (σ=4.8°) in monolayers transferred at π=8 mN/m and 2.4° (σ=5.0°) for monolayers transferred at π=30 mN/m. There is no statistical difference in the mean tilt angle or distribution for the two monolayer conditions studied. The insensitivity of tilt angle to filmsurfacepressure may arise from small chromophore doped domains of trapped liquid-expanded lipid phase remaining at high surfacepressure. There is no evidence in the near-field fluorescence images for probe molecules oriented with their dipole moment aligned parallel with the membrane plane. We do, however, find a small but significant population of probe molecules (∼13%) with tilt angles greater than 16°. Comparison of the simultaneously collected near-field fluorescence and force images suggests that these large angle orientations are not the result of significant defects in the films. Instead, this small population may represent a secondary insertion geometry for the probe molecule into the lipidmonolayer
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