The marine kd and water/sediment interaction problem

The behavior of marine distribution coefficients is analyzed with the help of numerical experiments and ana-lytical solutions of equations describing kinetic models for uptake/release of radionuclides. The difficulties in measuring true kd in a marine environment perturbed by an external radionuclide source are highlighted. Differences between suspended matter and bed sediment kd are analyzed. The performances of different kinetic models (1-step/2step; single-layer/multi-layer) are studied in model/model and model/experiment compar-isons. Implications for the use of models to assess radioactive contamination after an emergency are given; as well as recommendations when kd data are compiled in order to create a useful databaseInternational Atomic Energy Agency (IAEA) KIOST PE9961

Electric field inside a "Rossky cavity" in uniformly polarized water

Electric field produced inside a solute by a uniformly polarized liquid is strongly affected by dipolar polarization of the liquid at the interface. We show, by numerical simulations, that the electric "cavity" field inside a hydrated non-polar solute does not follow the predictions of standard Maxwell's electrostatics of dielectrics. Instead, the field inside the solute tends, with increasing solute size, to the limit predicted by the Lorentz virtual cavity. The standard paradigm fails because of its reliance on the surface charge density at the dielectric interface determined by the boundary conditions of the Maxwell dielectric. The interface of a polar liquid instead carries a preferential in-plane orientation of the surface dipoles thus producing virtually no surface charge. The resulting boundary conditions for electrostatic problems differ from the traditional recipes, affecting the microscopic and macroscopic fields based on them. We show that relatively small differences in cavity fields propagate into significant differences in the dielectric constant of an ideal mixture. The slope of the dielectric increment of the mixture versus the solute concentration depends strongly on which polarization scenario at the interface is realized. A much steeper slope found in the case of Lorentz polarization also implies a higher free energy penalty for polarizing such mixtures.Comment: 9 pages, 8 figure

Excess free energy and Casimir forces in systems with long-range interactions of van-der-Waals type: General considerations and exact spherical-model results

We consider systems confined to a $d$-dimensional slab of macroscopic lateral extension and finite thickness $L$ that undergo a continuous bulk phase transition in the limit $L\to\infty$ and are describable by an O(n) symmetrical Hamiltonian. Periodic boundary conditions are applied across the slab. We study the effects of long-range pair interactions whose potential decays as $b x^{-(d+\sigma)}$ as $x\to\infty$, with $2<\sigma<4$ and $2<d+\sigma\leq 6$, on the Casimir effect at and near the bulk critical temperature $T_{c,\infty}$, for $2<d<4$. For the scaled reduced Casimir force per unit cross-sectional area, we obtain the form L^{d} {\mathcal F}_C/k_BT \approx \Xi_0(L/\xi_\infty) + g_\omega L^{-\omega}\Xi\omega(L/\xi_\infty) + g_\sigma L^{-\omega_\sigm a} \Xi_\sigma(L \xi_\infty). The contribution $\propto g_\sigma$ decays for $T\neq T_{c,\infty}$ algebraically in $L$ rather than exponentially, and hence becomes dominant in an appropriate regime of temperatures and $L$. We derive exact results for spherical and Gaussian models which confirm these findings. In the case $d+\sigma =6$, which includes that of nonretarded van-der-Waals interactions in $d=3$ dimensions, the power laws of the corrections to scaling $\propto b$ of the spherical model are found to get modified by logarithms. Using general RG ideas, we show that these logarithmic singularities originate from the degeneracy $\omega=\omega_\sigma=4-d$ that occurs for the spherical model when $d+\sigma=6$, in conjunction with the $b$ dependence of $g_\omega$.Comment: 28 RevTeX pages, 12 eps figures, submitted to PR

Ab initio van der Waals interactions in simulations of water alter structure from mainly tetrahedral to high-density-like

The structure of liquid water at ambient conditions is studied in ab initio molecular dynamics simulations using van der Waals (vdW) density-functional theory, i.e. using the new exchange-correlation functionals optPBE-vdW and vdW-DF2. Inclusion of the more isotropic vdW interactions counteracts highly directional hydrogen-bonds, which are enhanced by standard functionals. This brings about a softening of the microscopic structure of water, as seen from the broadening of angular distribution functions and, in particular, from the much lower and broader first peak in the oxygen-oxygen pair-correlation function (PCF), indicating loss of structure in the outer solvation shells. In combination with softer non-local correlation terms, as in the new parameterization of vdW-DF, inclusion of vdW interactions is shown to shift the balance of resulting structures from open tetrahedral to more close-packed. The resulting O-O PCF shows some resemblance with experiment for high-density water (A. K. Soper and M. A. Ricci, Phys. Rev. Lett., 84:2881, 2000), but not directly with experiment for ambient water. However, an O-O PCF consisting of a linear combination of 70% from vdW-DF2 and 30% from experiment on low-density liquid water reproduces near-quantitatively the experimental O-O PCF for ambient water, indicating consistency with a two-liquid model with fluctuations between high- and low-density regions

Measurements of Branching Fractions and Time-dependent CP Violating Asymmetries in B0→D(∗)±D∓B^{0} \to D^{(*)\pm}D^{\mp} Decays

We report measurements of branching fractions and time-dependent CP asymmetries in $B^{0} \to D^{+}D^{-}$ and $B^{0} \to D^{*\pm}D^{\mp}$ decays using a data sample that contains $(772 \pm 11)\times 10^6 B\bar{B}$ pairs collected at the $\Upsilon(4S)$ resonance with the Belle detector at the KEKB asymmetric-energy $e^+ e^-$ collider. We determine the branching fractions to be $\mathcal{B}(B^{0} \to D^{+}D^{-})=(2.12 \pm 0.16 \pm 0.18)\times 10^{-4}$ and $\mathcal{B}(B^{0} \to D^{*\pm}D^{\mp}=(6.14 \pm 0.29 \pm 0.50)\times 10^{-4}$. We measure CP asymmetry parameters $\mathcal{S}_{D^{+}D^{-}} = -1.06_{-0.14}^{+0.21} \pm 0.08$ and $\mathcal{C}_{D^{+}D^{-}} = -0.43 \pm 0.16 \pm 0.05$ in $B^{0} \to D^{+}D^{-}$ and $\mathcal{A}_{D^{*}D} = +0.06 \pm 0.05 \pm 0.02$, $\mathcal{S}_{D^{*}D} = -0.78 \pm 0.15 \pm 0.05$, $\mathcal{C}_{D^{*}D} = -0.01 \pm 0.11 \pm 0.04$, $\Delta\mathcal{S}_{D^{*}D} = -0.13 \pm 0.15 \pm 0.04$ and $\Delta\mathcal{C}_{D^{*}D} = +0.12 \pm 0.11 \pm 0.03$ in $B^{0} \to D^{*\pm}D^{\mp}$, where the first uncertainty is statistical and the second is systematic. We exclude the conservation of CP symmetry in both decays at equal to or greater than $4\sigma$ significance.Comment: 7 pages, 2 figure

Search for Time-Dependent CPT Violation in Hadronic and Semileptonic B Decays

We report a new sensitive search for CPT violation, which includes improved measurements of the CPT-violating parameter z and the total decay-width difference normalized to the averaged width DeltaGamma_d/Gamma_d of the two Bd mass eigenstates. The results are based on a data sample of 535 x 10^6 BBbar pairs collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e^+e^- collider. We obtain Re(z) = [+1.9 +/- 3.7 (stat) +/- 3.3 (syst)] x 10^{-2}, Im(z) = [-5.7 +/- 3.3 (stat) +/- 3.3 (syst)] x 10^{-3}, and DeltaGamma_d/Gamma_d = [-1.7 +/- 1.8 (stat) +/- 1.1 (syst)] x 10^{-2}, all of which are consistent with zero. This is the most precise single measurement of these parameters in the neutral B-meson system to date.Comment: 7 pages, 3 figures, 2 tables, LaTeX; addition of supplemental information, corrections of typos, results unchange

Observation of Bs0→J/ψf0(980)B_s^0\to J/\psi f_0(980) and Evidence for Bs0→J/ψf0(1370)B_s^0\to J/\psi f_0(1370)

We report the first observation of $B_s^0\to J/\psi f_0(980)$ and first evidence for $B_s^0\to J/\psi f_0(1370)$, which are CP eigenstate decay modes. These results are obtained from $121.4\;\mathrm{fb}^{-1}$ of data collected at the $\Upsilon(5S)$ resonance with the Belle detector at the KEKB $e^+e^-$ collider. We measure the branching fractions $\mathcal{B}(B_s^0\to J/\psi f_0(980);f_0(980)\to\pi^+\pi^-)=(1.16^{+0.31}_{-0.19}(\mathrm{stat.})^{+0.15}_{-0.17}(\mathrm{syst.})^{+0.26}_{-0.18}(N_{B_s^{(*)}\bar B_s^{(*)}})) \times 10^{-4}$ with a significance of $8.4\sigma$, and $\mathcal{B}(B_s^0\to J/\psi f_0(1370);f_0(1370)\to\pi^+\pi^-)=(0.34^{+0.11}_{-0.14}(\mathrm{stat.})^{+0.03}_{-0.02}(\mathrm{syst.})^{+0.08}_{-0.05}(N_{B_s^{(*)}\bar B_s^{(*)}})) \times 10^{-4}$ with a significance of $4.2\sigma$. The last error listed is due to uncertainty in the number of produced $B_s^{(*)}\bar B_s^{(*)}$ pairs.Comment: 5 pages, 2 figures, 2 tables, published in PR

First observation of CP violation and improved measurement of the branching fraction and polarization of B0 -> D*+ D*- decays

We report the measurement of the branching fraction, the polarization, and the parameters of the time-dependent CP violation in B0 -> D*+ D*- decays using a data sample of 772 million BB pairs, collected at the Y(4S) resonance with the Belle detector at the KEKB asymmetric-energy e+e- collider. We obtain a branching fraction of B = (7.82 +- 0.38 +- 0.63) x10^{-4}, a CP-odd fraction of R_\perp = 0.138 +- 0.024 +- 0.006 and, additionally, a fraction of the longitudinal component in the transversity base of R_0 = 0.624 +- 0.029 +- 0.011. The measured values of the parameters of the CP violation are S_{D*+ D*-} = -0.79 +- 0.13 +- 0.03 and A_{D*+ D*-} = 0.15 +- 0.08 +- 0.04

First Observation of Radiative B^0 -> \phi K^0 \gamma Decays and Measurements of Their Time-Dependent CP Violation

We report the first observation of the radiative decay B^0 -> \phi K^0 \gamma using a data sample of 772 x 10^6 B B-bar pairs collected at the \Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e^+e^- collider. We observe a signal of 37+/-8 events with a significance of 5.4 standard deviations including systematic uncertainties. The measured branching fraction is ${\cal B}(B^0 -> \phi K^0 \gamma) = (2.74\pm 0.60 \pm 0.32) \times 10^{-6}$, where the uncertainties are statistical and systematic, respectively. We also report the first measurements of time-dependent CP violation parameters: ${\mathcal S}_{\phi K_S^0 \gamma} = +0.74^{+0.72}_{-1.05} (stat)^{+0.10}_{-0.24} (syst)$ and ${\mathcal A}_{\phi K_S^0 \gamma} = +0.35 +/- 0.58 (stat)^{+0.23}_{-0.10} (syst)$. Furthermore, we measure ${\mathcal B}(B^+ -> \phi K^+ \gamma) = (2.48 +/- 0.30 +/- 0.24) x 10^{-6}$, ${\mathcal A}_{CP} = -0.03 +/- 0.11 +/- 0.08$ and find that the signal is concentrated in the M_{\phi K} mass region near threshold.Comment: 6 pages, 3 figures, Modified version is to be published in PRD(RC