Competition Between Exchange and Anisotropy in a Pyrochlore Ferromagnet

The Ising-like spin ice model, with a macroscopically degenerate ground state, has been shown to be approximated by several real materials. Here we investigate a model related to spin ice, in which the Ising spins are replaced by classical Heisenberg spins. These populate a cubic pyrochlore lattice and are coupled to nearest neighbours by a ferromagnetic exchange term J and to the local axes by a single-ion anisotropy term D. The near neighbour spin ice model corresponds to the case D/J infinite. For finite D/J we find that the macroscopic degeneracy of spin ice is broken and the ground state is magnetically ordered into a four-sublattice structure. The transition to this state is first-order for D/J > 5 and second-order for D/J < 5 with the two regions separated by a tricritical point. We investigate the magnetic phase diagram with an applied field along [1,0,0] and show that it can be considered analogous to that of a ferroelectric.Comment: 7 pages, 4 figure

Universal Magnetic Fluctuations with a Field Induced Length Scale

We calculate the probability density function for the order parameter fluctuations in the low temperature phase of the 2D-XY model of magnetism near the line of critical points. A finite correlation length, \xi, is introduced with a small magnetic field, h, and an accurate expression for \xi(h) is developed by treating non-linear contributions to the field energy using a Hartree approximation. We find analytically a series of universal non-Gaussian distributions with a finite size scaling form and present a Gumbel-like function that gives the PDF to an excellent approximation. We propose the Gumbel exponent, a(h), as an indirect measure of the length scale of correlations in a wide range of complex systems.Comment: 7 pages, 4 figures, 1 table. To appear in Phys. Rev.

Statistics of extremal intensities for Gaussian interfaces

The extremal Fourier intensities are studied for stationary Edwards-Wilkinson-type, Gaussian, interfaces with power-law dispersion. We calculate the probability distribution of the maximal intensity and find that, generically, it does not coincide with the distribution of the integrated power spectrum (i.e. roughness of the surface), nor does it obey any of the known extreme statistics limit distributions. The Fisher-Tippett-Gumbel limit distribution is, however, recovered in three cases: (i) in the non-dispersive (white noise) limit, (ii) for high dimensions, and (iii) when only short-wavelength modes are kept. In the last two cases the limit distribution emerges in novel scenarios.Comment: 15 pages, including 7 ps figure

Ordered Phase of the Dipolar Spin Ice under [110]-Magnetic Fields

We find that the true ground state of the dipolar spin ice system under [110]-magnetic fields is the ``Q=X'' structure, which is consistent with both experiments and Monte Carlo simulations. We then perform a Monte Carlo simulation to confirm that there exists a first order phase transition under the [110]-field. In particular this result indicates the existence of the first order phase transition to the ``Q=X'' phase in the field above 0.35 T for Dy2Ti2O7. We also show the magnetic field-temperature phase diagram to summarize the ordered states of this system.Comment: 4 pages, 5 figures, in RevTex4, submitted to J. Phys. Soc. Jp

Static Correlation and Dynamical Properties of Tb3+-moments in Tb2Ti2O7 -Neutron Scattering Study-

Static and dynamical properties of the magnetic moment system of pyrochlore compound Tb2Ti2O7 with strong magnetic frustration, have been investigated down to the temperature T=0.4 K by neutron scattering on a single crystal sample. The scattering vector (Q)-dependence of the magnetic scattering intensity becomes appreciable with decreasing T at around 30 K, indicating the development of the magnetic correlation. From the observed energy profiles, the elastic, quasi elastic and inelastic components have been separately obtained. The quasi elastic component corresponds to the diffusive motion of the magnetic moments within the lowest states, which are formed of the lowest energy levels of Tb3+ ions. Magnetic correlation pattern which can roughly reproduce the Q-dependence of the scattering intensities of the elastic and quasi elastic component is discussed based on the trial calculations for clusters of 7 moments belonging to two corner-sharing tetrahedra. A possible origin of the glassy state, which develops at around 1.5 K with decreasing T is discussed.Comment: 10 pages, 12 figures, to be published in J. Phys. Soc. Jpn. 71(2002)No.2 59

Space-time Thermodynamics of the Glass Transition

We consider the probability distribution for fluctuations in dynamical action and similar quantities related to dynamic heterogeneity. We argue that the so-called "glass transition" is a manifestation of low action tails in these distributions where the entropy of trajectory space is sub-extensive in time. These low action tails are a consequence of dynamic heterogeneity and an indication of phase coexistence in trajectory space. The glass transition, where the system falls out of equilibrium, is then an order-disorder phenomenon in space-time occurring at a temperature T_g which is a weak function of measurement time. We illustrate our perspective ideas with facilitated lattice models, and note how these ideas apply more generally.Comment: 5 pages, 4 figure

Finite size scaling in the 2D XY-model and generalized universality

In recent works (BHP), a generalized universality has been proposed, linking phenomena as dissimilar as 2D magnetism and turbulence. To test these ideas, we performed a MC study of the 2D XY-model. We found that the shape of the probability distribution function for the magnetization M is non Gaussian and independent of the system size --in the range of the lattice sizes studied-- below the Kosterlitz-Thoules temperature. However, the shape of these distributions does depend on the temperature, contrarily to the BHP's claim. This behavior is successfully explained by using an extended finite-size scaling analysis and the existence of bounds for M.Comment: 7 pages, 5 figures. Submitted to Phys. Rev. Lett. Details of changes: 1. We emphasized in the abstract the range of validity of our results. 2. In the last paragraph the temperature dependence of the PDF was slightly re-formulate

Temperature dependent fluctuations in the two-dimensional XY model

We present a detailed investigation of the probability density function (PDF) of order parameter fluctuations in the finite two-dimensional XY (2dXY) model. In the low temperature critical phase of this model, the PDF approaches a universal non-Gaussian limit distribution in the limit T-->0. Our analysis resolves the question of temperature dependence of the PDF in this regime, for which conflicting results have been reported. We show analytically that a weak temperature dependence results from the inclusion of multiple loop graphs in a previously-derived graphical expansion. This is confirmed by numerical simulations on two controlled approximations to the 2dXY model: the Harmonic and ``Harmonic XY'' models. The Harmonic model has no Kosterlitz-Thouless-Berezinskii (KTB) transition and the PDF becomes progressively less skewed with increasing temperature until it closely approximates a Gaussian function above T ~ 4\pi. Near to that temperature we find some evidence of a phase transition, although our observations appear to exclude a thermodynamic singularity.Comment: 15 pages, 5 figures and 1 tabl

Reply to Comment on " Universal Fluctuations in Correlated Systems"

Reply to the comment, cond-mat/0209398 by by N.W. Watkins, S.C. Chapman, and G. RowlandsComment: To appear In Physical Review Letter

Temperature Dependence of the Magnetic Penetration Depth in the Vortex State of the Pyrochlore Superconductor, Cd2Re2O7

We report transverse field and zero field muon spin rotation studies of the superconducting rhenium oxide pyrochlore, Cd2Re2O7. Transverse field measurements (H=0.007 T) show line broadening below Tc, which is characteristic of a vortex state, demonstrating conclusively the type-II nature of this superconductor. The penetration depth is seen to level off below about 400 mK (T/Tc~0.4), with a rather large value of lambda (T=0)~7500A. The temperature independent behavior below ~ 400 mK is consistent with a nodeless superconducting energy gap. Zero-field measurements indicate no static magnetic fields developing below the transition temperature.Comment: 4 pages, 4 figures, REVTEX 4, submitted to PR