413 research outputs found
The ionization of Mg by electron impact at 1000 eV studied by (e, 2e) experiments
The ionization of Mg 3s and 2p and He 1s has been studied in (e, 2e) experiments at about 1000 eV incident energy and 20 eV ejected electron energy for a momentum transfer between 0.5 and 2.1 au. The comparison with the predictions of the distorted wave Born approximation model shows a generally good agreement between experiment and theory. The differences observed between the He and Mg angular distributions can be explained as an initial state effect and are attributed to the differences between the He 1s and Mg 3s wavefunctions in the momentum space
Near--K-edge double and triple detachment of the F- negative ion: observation of direct two-electron ejection by a single photon
Double and triple detachment of the F-(1s2 2s2 2p6) negative ion by a single
photon have been investigated in the photon energy range 660 to 1000 eV. The
experimental data provide unambiguous evidence for the dominant role of direct
photo-double-detachment with a subsequent single-Auger process in the reaction
channel leading to F2+ product ions. Absolute cross sections were determined
for the direct removal of a (1s+2p) pair of electrons from F- by the absorption
of a single photon
Magnetoelastic nature of solid oxygen epsilon-phase structure
For a long time a crystal structure of high-pressure epsilon-phase of solid
oxygen was a mistery. Basing on the results of recent experiments that have
solved this riddle we show that the magnetic and crystal structure of
epsilon-phase can be explained by strong exchange interactions of
antiferromagnetic nature. The singlet state implemented on quaters of O2
molecules has the minimal exchange energy if compared to other possible singlet
states (dimers, trimers). Magnetoelastic forces that arise from the spatial
dependence of the exchange integral give rise to transformation of 4(O2)
rhombuses into the almost regular quadrates. Antiferromagnetic character of the
exchange interactions stabilizes distortion of crystal lattice in epsilon-phase
and impedes such a distortion in long-range alpha- and delta-phases.Comment: 11 pages, 4 figures, Changes: corrected typos, reference to the
recent paper is adde
Quantum analogue of the spin-flop transition for a spin pair
Quantum (step-like) magnetization curves are studies for a spin pair with
antiferromagnetic coupling in the presence of a magnetic field parallel to the
easy axis of the magnetic anisotropy. The consideration is done both
analytically and numerically for a wide range of the anisotropy constants and
spins up to . Depending on the origin of the anisotropy
(exchange or single-ion), the magnetization curve can demonstrate the jumps
more than unity and the concentration of the unit jumps in a narrow range of
the field. We also point the region of the problem parameters, where the
behavior is quasiclassical for , and where system is substantially
quantum in the limit .Comment: 5 pages, 5 figure
The Missing Link in the Magnetism of Hybrid Cobalt Layered Hydroxides: The Odd-Even Effect of the Organic Spacer
A dramatic change in the magnetic behaviour, which solely depends on the parity of the organic linker molecules, has been found in a family of layered Co-II hydroxides covalently functionalized with dicarboxylic molecules. These layered hybrid materials have been synthesized at room temperature using a one-pot procedure through the epoxide route. While hybrids connected by odd alkyl chains exhibit coercive fields (H-c) below ca. 3500 Oe and show spontaneous magnetization at temperatures (T-M) below 20 K, hybrids functionalized with even alkyl chains behave as hard magnets with H(c)5500 Oe and display a T-M higher than 55 K. This intriguing behaviour was studied by density functional theory with the incorporation of a Hubbard term (DFT+U) calculations, unveiling the structural subtleties underlying this observation. Indeed, the different molecular orientation exhibited by the even/odd alkyl chains, and the orientation of the covalently linked carboxylic groups modify the intensity of the magnetic coupling of both octahedral and tetrahedral in-plane sublattices, thus strongly affecting the magnetic properties of the hybrid. These findings offer an outstanding level of tuning in the molecular design of hybrid magnetic materials based on layered hydroxides
Weak ferromagnetism and field-induced spin reorientation in K2V3O8
Magnetization and neutron diffraction measurements indicate long-range
antiferromagnetic ordering below TN=4 K in the 2D, S=1/2 Heisenberg
antiferromagnet K2V3O8. The ordered state exhibits ``weak ferromagnetism'' and
novel, field-induced spin reorientations. These experimental observations are
well described by a classical, two-spin Heisenberg model incorporating
Dzyaloshinskii-Moriya interactions and an additional c-axis anisotropy. This
additional anisotropy can be accounted for by inclusion of the symmetric
anisotropy term recently described by Kaplan, Shekhtman, Entin-Wohlman, and
Aharony. This suggests that K2V3O8 may be a very unique system where the
qualitative behavior relies on the presence of this symmetric anisotropy.Comment: 5 pages, 4 ps figures, REVTEX, submitted to PR
Dzyaloshinsky-Moriya antisymmetric exchange coupling in cuprates: Oxygen effects
We revisit a problem of Dzyaloshinsky-Moriya antisymmetric exchange coupling
for a single bond in cuprates specifying the local spin-orbital contributions
to Dzyaloshinsky vector focusing on the oxygen term. The Dzyaloshinsky vector
and respective weak ferromagnetic moment is shown to be a superposition of
comparable and, sometimes, competing local Cu and O contributions. The
intermediate oxygen O Knight shift is shown to be an effective tool to
inspect the effects of Dzyaloshinsky-Moriya coupling in an external magnetic
field. We predict the effect of oxygen weak antiferromagnetism in
edge-shared CuO chains due to uncompensated oxygen Dzyaloshinsky vectors.
Finally, we revisit the effects of symmetric spin anisotropy, in particular,
those directly induced by Dzyaloshinsky-Moriya coupling.Comment: 12 pages, 2 figures, submitted to JET
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