54 research outputs found
Correlated trends of coexisting magnetism and superconductivity in optimally electron-doped oxy-pnictides
We report on the recovery of the short-range static magnetic order and on the
concomitant degradation of the superconducting state in optimally F-doped
SmFe_(1-x)Ru_(x)AsO_0.85F_0.15 for 0.1< x<0.6. The two reduced order parameters
coexist within nanometer-size domains in the FeAs layers and finally disappear
around a common critical threshold x_c=0.6. Superconductivity and magnetism are
shown to be closely related to two distinct well-defined local electronic
environments of the FeAs layers. The two transition temperatures, controlled by
the isoelectronic and diamagnetic Ru substitution, scale with the volume
fraction of the corresponding environments. This fact indicates that
superconductivity is assisted by magnetic fluctuations, which are frozen
whenever a short-range static order appears, and totally vanish above the
magnetic dilution threshold x_c.Comment: Approved for publication in Phys. Rev. Letter
The onset of magnetism peaked around x=1/4 in optimally electron-doped LnFe(1-x)Ru(x)AsO(1-y)F(y) (Ln = La, Nd or Sm) superconductors
The appearance of static magnetism, nanoscopically coexisting with
superconductivity, is shown to be a general feature of optimally electron-doped
LnFe(1-x)Ru(x)AsO(1-y)F(y) superconductor (Ln - lanthanide ion) upon isovalent
substitution of Fe by Ru. The magnetic ordering temperature T_N and the
magnitude of the internal field display a dome-like dependence on x, peaked
around x=1/4, with higher T_N values for those materials characterized by a
larger z cell coordinate of As. Remarkably, the latter are also those with the
highest superconducting transition temperature (T_c) for x=0. The reduction of
T_c(x) is found to be significant in the x region of the phase diagram where
the static magnetism develops. Upon increasing the Ru content superconductivity
eventually disappears, but only at x=0.6.Comment: accepted for publication in PR
High pressure magnetic state of MnP probed by means of muon-spin rotation
We report a detailed SR study of the pressure evolution of the magnetic
order in the manganese based pnictide MnP, which has been recently found to
undergo a superconducting transition under pressure once the magnetic ground
state is suppressed. Using the muon as a volume sensitive local magnetic probe,
we identify a ferromagnetic state as well as two incommensurate helical states
(with propagation vectors aligned along the crystallographic and
directions, respectively) which transform into each other through first
order phase transitions as a function of pressure and temperature. Our data
appear to support that the magnetic state from which superconductivity develops
at higher pressures is an incommensurate helical phase.Comment: 11 pages, 9 figure
Slow magnetic fluctuations and superconductivity in fluorine-doped NdFeAsO
Among the widely studied superconducting iron-pnictide compounds belonging to
the Ln1111 family (with Ln a lanthanide), a systematic investigation of the
crossover region between the superconducting and the antiferromagnetic phase
for the Ln = Nd case has been missing. We fill this gap by focusing on the
intermediate doping regime of NdFeAsO(1-x)F(x) by means of dc-magnetometry and
muon-spin spectroscopy measurements. The long-range order we detect at low
fluorine doping is replaced by short-range magnetic interactions at x = 0.08,
where also superconductivity appears. In this case, longitudinal-field
muon-spin spectroscopy experiments show clear evidence of slow magnetic
fluctuations that disappear at low temperatures. This fluctuating component is
ascribed to the glassy-like character of the magnetically ordered phase of
NdFeAsO at intermediate fluorine doping
Understanding the SR spectra of MnSi without magnetic polarons
Transverse-field muon-spin rotation (SR) experiments were performed on a
single crystal sample of the non-centrosymmetric system MnSi. The observed
angular dependence of the muon precession frequencies matches perfectly the one
of the Mn-dipolar fields acting on the muons stopping at a 4a position of the
crystallographic structure. The data provide a precise determination of the
magnetic dipolar tensor. In addition, we have calculated the shape of the field
distribution expected below the magnetic transition temperature at the 4a
muon-site when no external magnetic field is applied. We show that this field
distribution is consistent with the one reported by zero-field SR studies.
Finally, we present ab initio calculations based on the density-functional
theory which confirm the position of the muon stopping site inferred from
transverse-field SR. In view of the presented evidence we conclude that
the SR response of MnSi can be perfectly and fully understood without
invoking a hypothetical magnetic polaron state.Comment: 10 pages, 12 figure
Magnetic ground state and spin fluctuations in MnGe chiral magnet as studied by Muon Spin Rotation
We have studied by muon spin resonance ({\mu}SR) the helical ground state and
fluctuating chiral phase recently observed in the MnGe chiral magnet. At low
temperature, the muon polarization shows double period oscillations at short
time scales. Their analysis, akin to that recently developed for MnSi [A. Amato
et al., Phys. Rev. B 89, 184425 (2014)], provides an estimation of the field
distribution induced by the Mn helical order at the muon site. The refined muon
position agrees nicely with ab initio calculations. With increasing
temperature, an inhomogeneous fluctuating chiral phase sets in, characterized
by two well separated frequency ranges which coexist in the sample. Rapid and
slow fluctuations, respectively associated with short range and long range
ordered helices, coexist in a large temperature range below T = 170 K. We
discuss the results with respect to MnSi, taking the short helical period,
metastable quenched state and peculiar band structure of MnGe into account.Comment: 13 pages, 11 figure
Common effect of chemical and external pressures on the magnetic properties of RECoPO (RE = La, Pr)
We report a detailed investigation of RECoPO (RE = La, Pr) and LaCoAsO
materials performed by means of muon spin spectroscopy. Zero-field measurements
show that the electrons localized on the Pr ions do not play any role in
the static magnetic properties of the compounds. Magnetism at the local level
is indeed fully dominated by the weakly-itinerant ferromagnetism from the Co
sublattice only. The increase of the chemical pressure triggered by the
different ionic radii of La and Pr, on the other hand, plays a
crucial role in enhancing the value of the magnetic critical temperature and
can be mimicked by the application of external hydrostatic pressure up to 24
kbar. A sharp discontinuity in the local magnetic field at the muon site in
LaCoPO at around 5 kbar suggests a sizeable modification in the band structure
of the material upon increasing pressure. This scenario is qualitatively
supported by \emph{ab-initio} density-functional theory calculations.Comment: 13 pages, 10 figure
Magnetic glassy phase in FeSeTe single crystals
The evolution of the magnetic order in FeSeTe crystals as a function of Se
content was investigated by means of ac/dc magnetometry and muon-spin
spectroscopy. Experimental results and self-consistent DFT calculations both
indicate that muons are implanted in vacant iron-excess sites, where they probe
a local field mainly of dipolar origin, resulting from an antiferromagnetic
(AFM) bicollinear arrangement of iron spins. This long-range AFM phase
disorders progressively with increasing Se content. At the same time all the
tested samples manifest a marked glassy character that vanishes for high Se
contents. The presence of local electronic/compositional inhomogeneities most
likely favours the growth of clusters whose magnetic moment "freezes" at low
temperature. This glassy magnetic phase justifies both the coherent muon
precession seen at short times in the asymmetry data, as well as the glassy
behaviour evidenced by both dc and ac magnetometry.Comment: Approved for publication in J. Phys.: Condens. Matte
Fast recovery of the pristine magnetic and structural phases in superconducting LaFeAsOF by Mn/Fe substitution
We report on an experimental study of the effect of Mn impurities in the
optimally doped LaFeAsOF compound. The results show that a
very tiny amount of Mn, of the order of 0.1\%, is enough to destroy
superconductivity and to recover at low temperatures both the magnetic ground
state and the orthorhombic structure of the pristine LaFeAsO parent compound.
The results are discussed within a model where electron correlations enhance
the Ruderman-Kittel-Kasuya-Yosida interaction among impurities
Charge doping versus disorder in CeFeAsO: do the in- and out-of-plane dilutions play the same role?
We provide direct experimental evidence for the identical effect of the
in-plane FeCo and of the out-of-plane OF chemical
dilutions on the itinerant spin-density-wave (SDW) magnetic phase in CeFeAsO.
Remarkably, the suppression of SDW is not sensitive at all to the different
kinds of disorder introduced in the two cases. Still, it is clearly shown that
the sizeable in-plane disorder induced by the FeCo substitution
is highly effective in suppressing . Differently from what is
observed in CeFeAsOF, the ordered magnetic phase of the Ce
sublattice is preserved throughout the whole phase diagram in
CeFeCoAsO (). An intriguing effect is encountered,
whereby the magnetic coupling among Ce ions is enhanced by the
superconducting phase.Comment: 8 pages (Main text: 4 pages. Paper merged with supplemental
information
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