251 research outputs found
Ni-Cr textured substrates with reduced ferromagnetism for coated conductor applications
A series of biaxially textured Ni(1-x)Cr(x) materials, with compositions x =
0, 7, 9, 11, and 13 at % Cr, have been studied for use as substrate materials
in coated conductor applications with high temperature superconductors. The
magnetic properties were investigated, including the hysteretic loss in a Ni-7
at % Cr sample that was controllably deformed; for comparison, the loss was
also measured in a similarly deformed pure Ni substrate. Complementary X-ray
diffraction studies show that thermo-mechanical processing produces nearly
complete {100} cube texturing, as desired for applications.Comment: PDF only; 19 pp., incl 10 figure
CeRuPO: A rare example of a Ferromagnetic Kondo lattice
We have determined the physical ground state properties of the compounds
CeRuPO and CeOsPO by means of magnetic susceptibility chi(T), specific heat
C(T), electrical resistivity rho(T), and thermopower S(T) measurements. chi(T)
reveals a trivalent 4f1 cerium state in both compounds. For CeRuPO a pronounced
decrease of rho(T) below 50K indicates the onset of coherent Kondo scattering
which is confirmed by enhanced S(T). The temperature and magnetic field
dependence of chi(T) and C(T) evidence ferromagnetic (FM) order at TC=15K.
Thus, CeRuPO seems to be one of the rare example of a FM Kondo lattice. In
contrast, CeOsPO shows antiferromagnetic order at TN=4.4K despite only minor
changes in lattice parameters and electronic configuration. Additional 31P NMR
results support these scenarios. LSDA+U calculations evidence a quasi two
dimensional electronic band structure, reflecting a strong covalent bonding
within the CeO and RuP layers and a weak ionic like bonding between the layers.Comment: accepted in Phys. Rev. B, high quality figures:
http://www.cpfs.mpg.de/~krellner
Specific heat of heavy fermion CePd2Si2 in high magnetic fields
We report specific heat measurements on the heavy fermion compound CePd2Si2
in magnetic fields up to 16 T and in the temperature range 1.4-16 K. A sharp
peak in the specific heat signals the antiferromagnetic transition at T_N ~ 9.3
K in zero field. The transition is found to shift to lower temperatures when a
magnetic field is applied along the crystallographic a-axis, while a field
applied parallel to the tetragonal c-axis does not affect the transition. The
magnetic contribution to the specific heat below T_N is well described by a sum
of a linear electronic term and an antiferromagnetic spin wave contribution.
Just below T_N, an additional positive curvature, especially at high fields,
arises most probably due to thermal fluctuations. The field dependence of the
coefficient of the low temperature linear term, gamma_0, extracted from the
fits shows a maximum at about 6 T, at the point where an anomaly was detected
in susceptibility measurements. The relative field dependence of both T_N and
the magnetic entropy at T_N scales as [1-(B/B_0)^2] for B // a, suggesting the
disappearance of antiferromagnetism at B_0 ~ 42 T. The expected suppression of
the antiferromagnetic transition temperature to zero makes the existence of a
magnetic quantum critical point possible.Comment: to be published in Journal of Physics: Condensed Matte
Specific Heat Study of Non-Fermi Liquid Behavior in CeNi_2Ge_2: Anomalous Peak in Quasi-Particle Density-of-States
To investigate the non-Fermi liquid (NFL) behavior in a nonalloyed system
CeNi_2Ge_2, we have measured the temperature and field dependences of the
specific heat C on a CeNi_2Ge_2 single crystal. The distinctive temperature
dependence of C/T (~a-b*T^(1/2)) is destroyed in almost the same manner for
both field directions of B//c-axis and B//a-axis. The overall behavior of
C(T,B) and the low-temperature upturn in magnetic susceptibility can be
reproduced, assuming an anomalous peak of the quasi-particle-band
density-of-states (DOS) at the Fermi energy possessing (epsilon)^(1/2) energy
dependence. Absence of residual entropy around T=0 K in B~0 T has been
confirmed by the magnetocaloric effect measurements, which are consistent with
the present model. The present model can also be applied to the NFL behavior in
CeCu_{5.9}Au_{0.1} using a ln(epsilon)-dependent peak in the DOS. Possible
origins of the peak in the DOS are discussed.Comment: 4 pages, LaTeX, using jpsj.sty, to be published in J. Phys. Soc. Jpn.
66 No. 10 (1997), 7 figures available at
http://494-475.phys.metro-u.ac.jp/ao/ceni2ge2.htm
Magnetic ordering of Mn sublattice, dense Kondo lattice behavior of Ce in (RPd3)8Mn (R = La, Ce)
We have synthesized two new interstitial compounds (RPd3)8Mn (R = La and Ce).
The Mn ions present in "dilute" concentration of just 3 molar percent form a
sublattice with an unusually large Mn-Mn near neighbor distance of ~ 85 nm.
While the existence of (RPd3)8M (where M is a p-block element) is already
documented in the literature, the present work reports for the first time the
formation of this phase with M being a 3d element. In (LaPd3)8Mn, the Mn
sub-lattice orders antiferromagnetically as inferred from the peaks in
low-field magnetization at 48 K and 23 K. The latter peak progressively shifts
towards lower temperatures in increasing magnetic field and disappears below
1.8 K in a field of ~ 8 kOe. On the other hand in (CePd3)8Mn the Mn sublattice
undergoes a ferromagnetic transition around 35 K. The Ce ions form a dense
Kondo-lattice and are in a paramagnetic state at least down to 1.5 K. A
strongly correlated electronic ground state arising from Kondo effect is
inferred from the large extrapolated value of C/T = 275 mJ/Ce-mol K^2 at T = 0
K. In contrast, the interstitial alloys RPd3Mnx (x = 0.03 and 0.06), also
synthesized for the first time, have a spin glass ground state due to the
random distribution of the Mn ions over the available "1b" sites in the parent
RPd3 crystal lattice.Comment: 18 figures and 20 pages of text documen
Resistivity, Hall effect and Shubnikov-de Haas oscillations in CeNiSn
The resistivity and Hall effect in CeNiSn are measured at temperatures down
to 35 mK and in magnetic fields up to 20 T with the current applied along the
{\it b} axis. The resistivity at zero field exhibits quadratic temperature
dependence below 0.16 K with a huge coefficient of the term (54
cm/K). The resistivity as a function of field shows an
anomalous maximum and dip, the positions of which vary with field directions.
Shubnikov-de Haas (SdH) oscillations with a frequency {\it F} of 100 T
are observed for a wide range of field directions in the {\it ac} and {\it bc}
planes, and the quasiparticle mass is determined to be 10-20 {\it m}.
The carrier density is estimated to be electron/Ce. In a narrow
range of field directions in the {\it ac} plane, where the
magnetoresistance-dip anomaly manifests itself clearer than in other field
directions, a higher-frequency () SdH oscillation is
found at high fields above the anomaly. This observation is discussed in terms
of possible field-induced changes in the electronic structure.Comment: 15 pages, 5 figures, to appear in Phys. Rev. B (15 Sept. 2002 issue
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