Extreme-ultraviolet vector-vortex beams from high harmonic generation

[EN]Structured light in the short-wavelength regime opens exciting avenues for the study of ultrafast spin and electronic dynamics. Here, we demonstrate theoretically and experimentally the generation of vector-vortex beams (VVB) in the extreme ultraviolet through high-order harmonic generation (HHG). The up-conversion of VVB, which are spatially tailored in their spin and orbital angular momentum, is ruled by the conservation of the topological Pancharatnam charge in HHG. Despite the complex propagation of the driving beam, high-harmonic VVB are robustly generated with smooth propagation properties. Remarkably, we find out that the conversion efficiency of high-harmonic VVB increases with the driving topological charge. Our work opens the possibility to synthesize attosecond helical structures with spatially varying polarization, a unique tool to probe spatiotemporal dynamics in inhomogeneous media or polarization-dependent systems.European Research Council (851201); Ministerio de Ciencia de Innovación y Universidades, Agencia Estatal de Investigación and European Social Fund (PID2019-106910GB-I00, RYC-2017-22745); Junta de Castilla y León and FEDER Funds (SA287P18); Université Paris-Saclay (2012-0333T-OASIS, 50110000724-OPTX, PhOM REC-2019-074-MAOHAm); Conseil Régional, Île-de-France (501100003990); Barcelona Supercomputing Center (FI-2020-3-0013)

Extreme-ultraviolet structured beams via high harmonic generation

Funding European Research Council (851201); Ministerio de Ciencia de Innovación y Universidades, Agencia Estatal de Investigaci ́on and European Social Fund (PID2019106910GB-I00, RYC-2017-22745); Junta de Castilla y León and FEDER Funds (SA287P18); Université ParisSaclay (2012-0333TOASIS, 50110000724-OPTX, PhOM REC-2019-074-MAOHAm); Conseil Régional, I ˆle-de-France (501100003990); Barcelona Supercomputing Center (FI2020-3-0013).Vigorous efforts to harness the topological properties of light have enabled a multitude of novel applications. Translating the applications of structured light to higher spatial and temporal resolutions mandates their controlled generation, manipulation, and thorough characterization in the short-wavelength regime. Here, we resort to high-order harmonic generation (HHG) in a noble gas to upconvert near-infrared (IR) vector, vortex, and vector-vortex driving beams that are tailored, respectively, in their spin angular momentum (SAM), orbital angular momentum (OAM), and simultaneously in their SAM and OAM. We show that HHG enables the controlled generation of extreme-ultraviolet (EUV) vector beams exhibiting various spatially dependent polarization distributions, or EUV vortex beams with a highly twisted phase. Moreover, we demonstrate the generation of EUV vector-vortex beams (VVB) bearing combined characteristics of vector and vortex beams. We rely on EUV wavefront sensing to unambiguously affirm the topological charge scaling of the HHG beams with the harmonic order. Interestingly, our work shows that HHG allows for a synchronous controlled manipulation of SAM and OAM. These EUV structured beams bring in the promising scenario of their applications at nanometric spatial and sub-femtosecond temporal resolutions using a table-top harmonic source

Extreme-ultraviolet structured beams via high harmonic generation

Funding European Research Council (851201); Ministerio de Ciencia de Innovación y Universidades, Agencia Estatal de Investigaci ́on and European Social Fund (PID2019106910GB-I00, RYC-2017-22745); Junta de Castilla y León and FEDER Funds (SA287P18); Université ParisSaclay (2012-0333TOASIS, 50110000724-OPTX, PhOM REC-2019-074-MAOHAm); Conseil Régional, I ˆle-de-France (501100003990); Barcelona Supercomputing Center (FI2020-3-0013).Vigorous efforts to harness the topological properties of light have enabled a multitude of novel applications. Translating the applications of structured light to higher spatial and temporal resolutions mandates their controlled generation, manipulation, and thorough characterization in the short-wavelength regime. Here, we resort to high-order harmonic generation (HHG) in a noble gas to upconvert near-infrared (IR) vector, vortex, and vector-vortex driving beams that are tailored, respectively, in their spin angular momentum (SAM), orbital angular momentum (OAM), and simultaneously in their SAM and OAM. We show that HHG enables the controlled generation of extreme-ultraviolet (EUV) vector beams exhibiting various spatially dependent polarization distributions, or EUV vortex beams with a highly twisted phase. Moreover, we demonstrate the generation of EUV vector-vortex beams (VVB) bearing combined characteristics of vector and vortex beams. We rely on EUV wavefront sensing to unambiguously affirm the topological charge scaling of the HHG beams with the harmonic order. Interestingly, our work shows that HHG allows for a synchronous controlled manipulation of SAM and OAM. These EUV structured beams bring in the promising scenario of their applications at nanometric spatial and sub-femtosecond temporal resolutions using a table-top harmonic source

Highly Scalable Multicycle THz Production with a Homemade Periodically Poled Macroscrystal

The THz regime is widely appealing across many disciplines including solid-state physics, life sciences, and increasingly in particle acceleration.Multicycle THz pulses are typically formed via optical rectification in periodically poled crystals. However the manufacturing procedures of these crystals limit their apertures to below $\sim$1 cm, which from damage limitations of the crystal, limits the total pump power which can be employed, and ultimately, the total THz power which can be produced. Here we report on the simple in-house fabrication of a periodically poled crystal using $\sim$300 $\mu$m thick wafers. Each wafer is consecutively rotated by 180$^{\circ}$ to support quasi-phase matching. We validate the concept with a Joule-class laser system operating at 10 Hz and measure up to 1.3 mJ of energy at 160~GHz, corresponding to an average peak power of approximately 35 MW and a conversion efficiency of 0.14\%. In addition, a redshifting of the pump spectrum of $\sim$50 nm is measured. Our results indicate that high-power THz radiation can be produced with existing and future high-power lasers in a scalable way, setting a course toward multi-gigawatt multicycle THz pulses

35 megawatt multicycle THz pulses from a homemade periodically poled macrocrystal

High-power multicycle THz radiation is highly sought after with applications in medicine, imaging, spectroscopy, characterization and manipulation of condensed matter, and could support the development of next-generation compact laser-based accelerators with applications in electron microscopy, ultrafast X-ray sources and sub-femtosecond longitudinal diagnostics. Multicycle THz-radiation can be generated by shooting an appropriate laser through a periodically poled nonlinear crystal, e.g. lithium niobate (PPLN). Unfortunately, the manufacturing processes of PPLNs require substantially strong electric fields $\mathcal{O}(10~kV/mm)$ across the crystal width to locally reverse the polarization domains; this limits the crystal apertures to below 1 cm. Damage threshold limitations of lithium niobate thereby limits the laser power which can be shone onto the crystal, which inherently limits the production of high-power THz pulses. Here we show that in the THz regime, a PPLN crystal can be mechanically constructed in-air by stacking lithium niobate wafers together with 180$^{\circ}$ rotations to each other. The relatively long (mm) wavelengths of the generated THz radiation compared to the small gaps ($\sim$10 $\mu$m) between wafers supports a near-ideal THz transmission between wafers. We demonstrate the concept using a Joule-class laser system with $\sim$50 mm diameter wafers and measure up to 1.3 mJ of THz radiation corresponding to a peak power of $\sim$35 MW, a 50 times increase in THz power compared to previous demonstrations. Our results indicate that high-power THz radiation can be produced with existing and future high-power lasers in a scalable way, setting a course toward multi-gigawatt THz pulses. Moreover the simplicity of the scheme provides a simple way to synthesize waveforms for a variety of applications

Experiment to observe an optically induced change of the vacuum index

International audienceQuantum electrodynamics predicts that the vacuum must behave as a nonlinear optical medium: the speed of light should be modified when the vacuum is stressed by intense electromagnetic fields. This optical phenomenon has not yet been observed. The DeLLight (deflection of light by light) experiment aims to observe the optically induced index change of vacuum, a nonlinear effect which has never been explored. The experiment is installed in the LASERIX facility at IJCLab, which delivers ultrashort intense laser pulses (2.5 J per pulse, each of 30 fs duration, with a 10 Hz repetition rate). The proposal is to measure the refraction of a probe laser pulse when crossing a transverse vacuum index gradient, produced by a very intense pump pulse. The refraction induces a transverse shift in the intensity profile of the probe, whose signal is amplified by a Sagnac interferometer. In this article we describe the experimental method and setup, and present the complete theoretical calculations for the expected signal. With a minimum waist at focus of 5μm (corresponding to a maximum intensity of ∼3×1020W/cm2), and with the nonlinear vacuum index derived from QED, the expected refraction angle is 0.13 prad. First results of the interferometer prototype are presented. It is shown that an extinction factor F=0.4×10−5 (corresponding to a signal amplification factor of 250) and a spatial resolution σy=10nm are achievable. The expected signal is then about 15 pm, and could be observed at a 5-sigma confidence level with about one month of collected data

Performance of a Sagnac interferometer to observe vacuum optical nonlinearity

International audienceIn Quantum Electrodynamics, vacuum becomes a nonlinear optical medium: its optical index should be modified in the presence of intense external electromagnetic fields. The DeLLight project (Deflection of Light by Light) aims to observe this effect using intense focused femtosecond laser pulses delivered by LASERIX. The principle is to measure with a Sagnac interferometer the deflection of a low-intensity focused pulse (probe) crossing the vacuum index gradient induced by a high-intensity pulse (pump). A Sagnac interferometer working with femtosecond laser pulses has been developed for the DeLLight project. Compared to previous prototypes, the interferometer now includes the focusing of the probe beam in the interaction area. In this article, we measure and characterize the critical experimental parameters limiting the sensitivity of the interferometer, namely the extinction factor, the spatial resolution, and the waist at focus of the probe pulse. We discuss future improvements

Interferometric measurement of the deflection of light by light in air

International audienceThe aim of the DeLLight (Deflection of Light by Light) experiment is to observe for the first time the optical nonlinearity in vacuum, as predicted by Quantum Electrodynamics, by measuring the refraction of a low-intensity focused laser pulse (probe) when crossing the effective vacuum index gradient induced by a high-intensity focused laser pulse (pump). The deflection signal is amplified by using a Sagnac interferometer. Here, we report the first measurement performed with the DeLLight pilot interferometer, of the deflection of light by light in air, with a low-intensity pump. We show that the deflection signal measured by the interferometer is amplified, and is in agreement with the expected signal induced by the optical Kerr effect in air. Moreover, we verify that the signal varies as expected as a function of the pump intensity, the temporal delay between the pump and the probe, and their relative polarisation. These results represent a proof of concept of the DeLLight experimental method based on interferometric amplification