Electronic correlations in double ionization of atoms in pump-probe experiments

The ionization dynamics of a two-electron atom in an attosecond XUV-infrared pump-probe experiment is simulated by solving the time-dependent two-electron Schr\"odinger equation. A dramatic change of the double ionization (DI) yield with variation of the pump-probe delay is reported and the governing role of electron-electron correlations is shown. The results allow for a direct control of the DI yield and of the relative strength of double and single ionization

Quantum breathing mode of trapped bosons and fermions at arbitrary coupling

An analysis of the quantum breathing behavior of few-particle Coulomb systems in one- and two-dimensional harmonic traps is presented. We report the existence of \emph{two independent breathing modes} and present exact numerical results for two particles at any coupling strength which smoothly connect the two known limits of an \emph {ideal} quantum and a strongly coupled \emph {classical} system. Substantial differences in the breathing frequency of two-dimensional fermions and bosons are observed which may be used as a sensitive experimental tool to probe confined interacting quantum systems

Efficient grid-based method in nonequilibrium Green's function calculations. Application to model atoms and molecules

We propose and apply the finite-element discrete variable representation to express the nonequilibrium Green's function for strongly inhomogeneous quantum systems. This method is highly favorable against a general basis approach with regard to numerical complexity, memory resources, and computation time. Its flexibility also allows for an accurate representation of spatially extended hamiltonians, and thus opens the way towards a direct solution of the two-time Schwinger/Keldysh/Kadanoff-Baym equations on spatial grids, including e.g. the description of highly excited states in atoms. As first benchmarks, we compute and characterize, in Hartree-Fock and second Born approximation, the ground states of the He atom, the H$_2$ molecule and the LiH molecule in one spatial dimension. Thereby, the ground-state/binding energies, densities and bond-lengths are compared with the direct solution of the time-dependent Schr\"odinger equation.Comment: 11 pages, 5 figures, submitted to Physical Review

Nonequilibrium Green function approach to photoionization processes in atoms

We present a quantum kinetic approach for the time-resolved description of many-body effects in photoionization processes in atoms. The method is based on the non-equilibrium Green functions formalism and solves the Keldysh/Kadanoff-Baym equations in second Born approximation. An approximation scheme is introduced and discussed, which provides a complete single-particle description of the continuum, while the atom is treated fully correlated.Comment: 11 pages, 6 figure