4,384 research outputs found
Comparative investigation of the coupled-tetrahedra quantum spin systems Cu2Te2O5X2, X=Cl, Br and Cu4Te5O12Cl4
We present a comparative study of the coupled-tetrahedra quantum spin systems
Cu2Te2O5X2, X=Cl, Br (Cu-2252(X)) and the newly synthesized Cu4Te5O12Cl4
(Cu-45124(Cl)) based on ab initio Density Functional Theory calculations. The
magnetic behavior of Cu-45124(Cl) with a phase transition to an ordered state
at a lower critical temperature T=13.6K than in Cu-2252(Cl) (T=18K) can
be well understood in terms of the modified interaction paths. We identify the
relevant structural changes between the two systems and discuss the
hypothetical behavior of the not yet synthesized Cu-45124(Br) with an ab initio
relaxed structure using Car-Parrinello Molecular Dynamics.Comment: 2 pages, 1 figure; submitted to Proceedings of M2S-HTSC VIII, Dresden
200
Consequences of critical interchain couplings and anisotropy on a Haldane chain
Effects of interchain couplings and anisotropy on a Haldane chain have been
investigated by single crystal inelastic neutron scattering and density
functional theory (DFT) calculations on the model compound SrNiVO.
Significant effects on low energy excitation spectra are found where the
Haldane gap (; where is the intrachain exchange
interaction) is replaced by three energy minima at different antiferromagnetic
zone centers due to the complex interchain couplings. Further, the triplet
states are split into two branches by single-ion anisotropy. Quantitative
information on the intrachain and interchain interactions as well as on the
single-ion anisotropy are obtained from the analyses of the neutron scattering
spectra by the random phase approximation (RPA) method. The presence of
multiple competing interchain interactions is found from the analysis of the
experimental spectra and is also confirmed by the DFT calculations. The
interchain interactions are two orders of magnitude weaker than the
nearest-neighbour intrachain interaction = 8.7~meV. The DFT calculations
reveal that the dominant intrachain nearest-neighbor interaction occurs via
nontrivial extended superexchange pathways Ni--O--V--O--Ni involving the empty
orbital of V ions. The present single crystal study also allows us to
correctly position SrNiVO in the theoretical - phase
diagram [T. Sakai and M. Takahashi, Phys. Rev. B 42, 4537 (1990)] showing where
it lies within the spin-liquid phase.Comment: 12 pages, 12 figures, 3 tables PRB (accepted). in Phys. Rev. B (2015
The bar PANDA focussing-lightguide disc DIRC
bar PANDA will be a fixed target experiment internal to the HESR antiproton storage ring at the future FAIR complex. The ANDA detector requires excellent particle-identification capabilities in order to achieve its scientific potential. Cherenkov counters employing the DIRC principle were chosen as PID detectors for the Target Spectrometer. The proposed Focussing-Lightguide Disc DIRC will cover the forward part of the Target Spectrometer acceptance in the angular range between 5° and 22°. Its design includes a novel approach to mitigate dispersion effects in the solid radiator of a DIRC counter using optical elements. The dispersion correction will enable the Focussing-Lightguide Disc DIRC to provide pion-kaon identification for momenta well above 3.5 GeV/c
X-ray absorption spectroscopy on layered cobaltates Na_xCoO_2
Measurements of polarization and temperature dependent soft x-ray absorption
have been performed on Na_xCoO_2 single crystals with x=0.4 and x=0.6. They
show a deviation of the local trigonal symmetry of the CoO_6 octahedra, which
is temperature independent in a temperature range between 25 K and 372 K. This
deviation was found to be different for Co^{3+} and Co^{4+} sites. With the
help of a cluster calculation we are able to interpret the Co L_{23}-edge
absorption spectrum and find a doping dependent energy splitting between the
t_{2g} and the e_g levels (10Dq) in Na_xCoO_2.Comment: 7 pages, 8 figure
Intrinsic peculiarities of real material realizations of a spin-1/2 kagome lattice
Spin-1/2 magnets with kagome geometry, being for years a generic object of
theoretical investigations, have few real material realizations. Recently, a
DFT-based microscopic model for two such materials, kapellasite Cu3Zn(OH)6Cl2
and haydeeite Cu3Mg(OH)6Cl2, was presented [O. Janson, J. Richter and H.
Rosner, arXiv:0806.1592]. Here, we focus on the intrinsic properties of real
spin-1/2 kagome materials having influence on the magnetic ground state and the
low-temperature excitations. We find that the values of exchange integrals are
strongly dependent on O--H distance inside the hydroxyl groups, present in most
spin-1/2 kagome compounds up to date. Besides the original kagome model,
considering only the nearest neighbour exchange, we emphasize the crucial role
of the exchange along the diagonals of the kagome lattice.Comment: 4 pages, 4 figures. A paper for the proceedings of the HFM 2008
conferenc
Comment on studying the corrections to factorization in B -> D(*) X
We propose studying the mechanism of factorization in exclusive decays of the
form B->D(*)X by examining the differential decay rate as a function of the
invariant mass of the light hadronic state X. If factorization works primarily
due to the large N_c limit then its accuracy is not expected to decrease as the
X invariant mass increases. However, if factorization is mostly a consequence
of perturbative QCD then the corrections should grow with the X invariant mass.
Combining data for hadronic tau decays and semileptonic B decays allows tests
of factorization to be made for a variety of final states. We discuss the
examples of B->D^*\pi^+\pi^-\pi^-\pi^0 and B->D^*\omega\pi^-. The mode
B->D^*\omega\pi^- will allow a precision study of the dependence of the
corrections to factorization on the invariant mass of the light hadronic state.Comment: 7 pages, minor clarifications to tex
Reconstruction methods — P‾ANDA focussing-light guide disc DIRC
The Focussing-Lightguide Disc DIRC will provide crucial Particle Identification (PID) information for the P‾ANDA experiment at FAIR, GSI. This detector presents a challenging environment for reconstruction due to the complexity of the expected hit patterns and the operating conditions of the P‾ANDA experiment. A discussion of possible methods to reconstruct PID from this detector is given here. Reconstruction software is currently under development
Structure and magnetism of Cr2BP3O12: Towards the quantum-classical crossover in a spin-3/2 alternating chain
Magnetic properties of the spin-3/2 Heisenberg system Cr2BP3O12 are
investigated by magnetic susceptibility chi(T) measurements, electron spin
resonance, neutron diffraction, and density functional theory (DFT)
calculations, as well as classical and quantum Monte Carlo (MC) simulations.
The broad maximum of chi(T) at 85K and the antiferromagnetic Weiss temperature
of 139 K indicate low-dimensional magnetic behavior. Below TN = 28 K, Cr2BP3O12
is antiferromagnetically ordered with the k = 0 propagation vector and an
ordered moment of 2.5 muB/Cr. DFT calculations, including DFT+U and hybrid
functionals, yield a microscopic model of spin chains with alternating
nearest-neighbor couplings J1 and J1' . The chains are coupled by two
inequivalent interchain exchanges of similar strength (~1-2 K), but different
sign (antiferromagnetic and ferromagnetic). The resulting spin lattice is
quasi-one-dimensional and not frustrated. Quantum MC simulations show excellent
agreement with the experimental data for the parameters J1 ~= 50 K and J1'/J1
~= 0.5. Therefore, Cr2BP3O12 is close to the gapless critical point (J1'/J1 =
0.41) of the spin-3/2 bond-alternating Heisenberg chain. The applicability
limits of the classical approximation are addressed by quantum and classical MC
simulations. Implications for a wide range of low-dimensional S = 3/2 materials
are discussed.Comment: Published version: 13 pages, 7 figures, 5 tables + Supplementary
informatio
Tight-binding parameters and exchange integrals of Ba_2Cu_3O_4Cl_2
Band structure calculations for Ba_2Cu_3O_4Cl_2 within the local density
approximation (LDA) are presented. The investigated compound is similar to the
antiferromagnetic parent compounds of cuprate superconductors but contains
additional Cu_B atoms in the planes. Within the LDA, metallic behavior is found
with two bands crossing the Fermi surface (FS). These bands are built mainly
from Cu 3d_{x^2-y^2} and O 2p_{x,y} orbitals, and a corresponding tight-binding
(TB) model has been parameterized. All orbitals can be subdivided in two sets
corresponding to the A- and B-subsystems, respectively, the coupling between
which is found to be small. To describe the experimentally observed
antiferromagnetic insulating state, we propose an extended Hubbard model with
the derived TB parameters and local correlation terms characteristic for
cuprates. Using the derived parameter set we calculate the exchange integrals
for the Cu_3O_4 plane. The results are in quite reasonable agreement with the
experimental values for the isostructural compound Sr_2Cu_3O_4Cl_2.Comment: 5 pages (2 tables included), 4 ps-figure
Technical Design Report for the PANDA Micro Vertex Detector
This document illustrates the technical layout and the expected performance of the Micro Vertex Detector (MVD) of the PANDA experiment. The MVD will detect charged particles as close as possible to the interaction zone. Design criteria and the optimisation process as well as the technical solutions chosen are discussed and the results of this process are subjected to extensive Monte Carlo physics studies. The route towards realisation of the detector is
outlined
- …