315 research outputs found
Universal Properties of Ferroelectric Domains
Basing on Ginzburg-Landau approach we generalize the Kittel theory and derive
the interpolation formula for the temperature evolution of a multi-domain
polarization profile P(x,z). We resolve the long-standing problem of the
near-surface polarization behavior in ferroelectric domains and demonstrate the
polarization vanishing instead of usually assumed fractal domain branching. We
propose an effective scaling approach to compare the properties of different
domain-containing ferroelectric plates and films.Comment: Phys. Rev. Lett. to be publishe
Domain enhanced interlayer coupling in ferroelectric/paraelectric superlattices
We investigate the ferroelectric phase transition and domain formation in a
periodic superlattice consisting of alternate ferroelectric (FE) and
paraelectric (PE) layers of nanometric thickness. We find that the polarization
domains formed in the different FE layers can interact with each other via the
PE layers. By coupling the electrostatic equations with those obtained by
minimizing the Ginzburg-Landau functional we calculate the critical temperature
of transition Tc as a function of the FE/PE superlattice wavelength and
quantitatively explain the recent experimental observation of a thickness
dependence of the ferroelectric transition temperature in KTaO3/KNbO3
strained-layer superlattices.Comment: Latest version as was published in PR
Nonradiating anapole modes in dielectric nanoparticles
Nonradiating current configurations attract attention of physicists for many years as possible models of stable atoms. One intriguing example of such a nonradiating source is known as 'anapole'. An anapole mode can be viewed as a composition of electric and toroidal dipole moments, resulting in destructive interference of the radiation fields due to similarity of their far-field scattering patterns. Here we demonstrate experimentally that dielectric nanoparticles can exhibit a radiationless anapole mode in visible. We achieve the spectral overlap of the toroidal and electric dipole modes through a geometry tuning, and observe a highly pronounced dip in the far-field scattering accompanied by the specific near-field distribution associated with the anapole mode. The anapole physics provides a unique playground for the study of electromagnetic properties of nontrivial excitations of complex fields, reciprocity violation and Aharonov-Bohm like phenomena at optical frequencies.The work of A.E.M. was supported by the Australian Research Council via Future
Fellowship program (FT110100037). The authors at DSI were supported by DSI core
funds. Fabrication, Scanning Electron Microscope Imaging and NSOM works were
carried out in facilities provided by SnFPC@DSI (SERC Grant 092 160 0139). Zhen Ying
Pan (DSI) is acknowledged for SEM imaging. Yi Zhou (DSI) is acknowledged for silicon
film growth. Leonard Gonzaga (DSI), Yeow Teck Toh (DSI) and Doris Ng (DSI) are
acknowledged for development of the silicon nanofabrication procedure. B.N.C.
acknowledges support from the Government of Russian Federation, Megagrant No.
14.B25.31.0019
Boosting the Figure Of Merit of LSPR-based refractive index sensing by phase-sensitive measurements
Localized surface plasmon resonances possess very interesting properties for
a wide variety of sensing applications. In many of the existing applications
only the intensity of the reflected or transmitted signals is taken into
account, while the phase information is ignored. At the center frequency of a
(localized) surface plasmon resonance, the electron cloud makes the transition
between in- and out-of-phase oscillation with respect to the incident wave.
Here we show that this information can experimentally be extracted by
performing phase-sensitive measurements, which result in linewidths that are
almost one order of magnitude smaller than those for intensity based
measurements. As this phase transition is an intrinsic property of a plasmon
resonance, this opens up many possibilities for boosting the figure of merit
(FOM) of refractive index sensing by taking into account the phase of the
plasmon resonance. We experimentally investigated this for two model systems:
randomly distributed gold nanodisks and gold nanorings on top of a continuous
gold layer and a dielectric spacer and observed FOM values up to 8.3 and 16.5
for the respective nanoparticles
Possible Fractional Quantum Hall Effect in Graphite
Measurements of basal plane longitudinal rho_b(B) and Hall rho_H(B)
resistivities were performed on highly oriented pyrolytic graphite (HOPG)
samples in pulsed magnetic field up to B = 50 T applied perpendicular to
graphene planes, and temperatures 1.5 K 30 T and for all
studied samples, we observed a sign change in rho_H(B) from electron- to
hole-like. For our best quality sample, the measurements revealed the
enhancement in rho_b(B) for B > 34 T (T = 1.8 K), presumably associated with
the field-driven charge density wave or Wigner crystallization transition.
Besides, well defined plateaus in rho_H(B) were detected in the ultra-quantum
limit revealing the signatures of fractional quantum Hall effect in graphite.Comment: 15 pages, including 4 figure
Synthesis of Glass Nanofibers Using Femtosecond Laser Radiation Under Ambient Condition
We report the unique growth of nanofibers in silica and borosilicate glass using femtosecond laser radiation at 8 MHz repetition rate and a pulse width of 214 fs in air at atmospheric pressure. The nanofibers are grown perpendicular to the substrate surface from the molten material in laser-drilled microvias where they intertwine and bundle up above the surface. The fibers are few tens of nanometers in thickness and up to several millimeters in length. Further, it is found that at some places nanoparticles are attached to the fiber surface along its length. Nanofiber growth is explained by the process of nanojets formed in the molten liquid due to pressure gradient induced from the laser pulses and subsequently drawn into fibers by the intense plasma pressure. The attachment of nanoparticles is due to the condensation of vapor in the plasma
Basal-plane Incommensurate Phases in HCP Structures
An Ising model with competing interaction is used to study the appearance of
incommensurate phases in the basal plane of an hexagonal closed-packed
structure. The calculated mean-field phase diagram reveals various
1q-incommensurate and lock-in phases. The results are applied to explain the
basal-plane incommensurate phase in some compounds of the A'A"BX_4 family, like
K_2MoO_4, K_2WO_4, Rb_2WO4 and to describe the sequence of high-temperature
phase transitions in other compounds of this family.Comment: 8 pages, RevTeX + 4 ps figure
Fano resonances in plasmonic core-shell particles and the Purcell effect
Despite a long history, light scattering by particles with size comparable
with the light wavelength still unveils surprising optical phenomena, and many
of them are related to the Fano effect. Originally described in the context of
atomic physics, the Fano resonance in light scattering arises from the
interference between a narrow subradiant mode and a spectrally broad radiation
line. Here, we present an overview of Fano resonances in coated spherical
scatterers within the framework of the Lorenz-Mie theory. We briefly introduce
the concept of conventional and unconventional Fano resonances in light
scattering. These resonances are associated with the interference between
electromagnetic modes excited in the particle with different or the same
multipole moment, respectively. In addition, we investigate the modification of
the spontaneous-emission rate of an optical emitter at the presence of a
plasmonic nanoshell. This modification of decay rate due to electromagnetic
environment is referred to as the Purcell effect. We analytically show that the
Purcell factor related to a dipole emitter oriented orthogonal or tangential to
the spherical surface can exhibit Fano or Lorentzian line shapes in the near
field, respectively.Comment: 28 pages, 10 figures; invited book chapter to appear in "Fano
Resonances in Optics and Microwaves: Physics and Application", Springer
Series in Optical Sciences (2018), edited by E. O. Kamenetskii, A. Sadreev,
and A. Miroshnichenk
Magnetic skyrmions and their lattices in triplet superconductors
Complete topological classification of solutions in SO(3) symmetric
Ginzburg-Landau free energy has been performed and a new class of solutions in
weak external magnetic field carrying two units of magnetic flux has been
identified. These solutions, magnetic skyrmions, do not have singular core like
Abrikosov vortices and at low magnetic field become lighter for strongly type
II superconductors. As a consequence, the lower critical magnetic field Hc1 is
reduced by a factor of log(kappa). Magnetic skyrmions repel each other as 1/r
at distances much larger then magnetic penetration depth forming relatively
robust triangular lattice. Magnetic induction near Hc1 increases gradually as
(H-Hc1)^2. This agrees very well with experiments on heavy fermion
superconductor UPt3. Newly discovered Ru based compounds Sr2RuO4 and
Sr2YRu(1-x)Cu(x)O6 are other possible candidates to possess skyrmion lattices.
Deviations from exact SO(3) symmetry are also studied.Comment: 23 pages, 10 eps figure
Plasmonically Enhanced Reflectance of Heat Radiation from Low-Bandgap Semiconductor Microinclusions
Increased reflectance from the inclusion of highly scattering particles at
low volume fractions in an insulating dielectric offers a promising way to
reduce radiative thermal losses at high temperatures. Here, we investigate
plasmonic resonance driven enhanced scattering from microinclusions of
low-bandgap semiconductors (InP, Si, Ge, PbS, InAs and Te) in an insulating
composite to tailor its infrared reflectance for minimizing thermal losses from
radiative transfer. To this end, we compute the spectral properties of the
microcomposites using Monte Carlo modeling and compare them with results from
Fresnel equations. The role of particle size-dependent Mie scattering and
absorption efficiencies, and, scattering anisotropy are studied to identify the
optimal microinclusion size and material parameters for maximizing the
reflectance of the thermal radiation. For composites with Si and Ge
microinclusions we obtain reflectance efficiencies of 57 - 65% for the incident
blackbody radiation from sources at temperatures in the range 400 - 1600
{\deg}C. Furthermore, we observe a broadbanding of the reflectance spectra from
the plasmonic resonances due to charge carriers generated from defect states
within the semiconductor bandgap. Our results thus open up the possibility of
developing efficient high-temperature thermal insulators through use of the
low-bandgap semiconductor microinclusions in insulating dielectrics.Comment: Main article (8 Figures and 2 Tables) + Supporting Information (8
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