Low-temperature kinetics of exciton-exciton annihilation of weakly localized one-dimensional Frenkel excitons

We present results of numerical simulations of the kinetics of exciton-exciton annihilation of weakly localized one-dimensional Frenkel excitons at low temperatures. We find that the kinetics is represented by two well-distinguished components: a fast short-time decay and a very slow long-time tail. The former arises from excitons that initially reside in states belonging to the same localization segment of the chain, while the slow component is caused by excitons created on different localization segments. We show that the usual bi-molecular theory fails in the description of the behavior found. We also present a qualitative analytical explanation of the non-exponential behavior observed in both the short- and the long-time decay components.Comment: Published in J. Chem. Phys. 114, 1 April (2001

Photon recoil momentum in a Bose-Einstein condensate of a dilute gas

We develop a "minimal" microscopic model to describe a two-pulse-Ramsay-interferometer-based scheme of measurement of the photon recoil momentum in a Bose-Einstein condensate of a dilute gas [Campbell et al., Phys. Rev. Lett. 94, 170403 (2005)]. We exploit the truncated coupled Maxwell-Schroedinger equations to elaborate the problem. Our approach provides a theoretical tool to reproduce essential features of the experimental results. Additionally, we enable to calculate the quantum-mechanical mean value of the recoil momentum and its statistical distribution that provides a detailed information about the recoil event.Comment: 6 pages, 4 figure

Photon Recoil in Light Scattering by a Bose-Einstein Condensate of a Dilute Gas

Abstract: Photon recoil upon light scattering by a Bose–Einstein condensate (BEC) of a dilute atomic gas is analyzed theoretically accounting for a weak interatomic interaction. Our approach is based on the Gross–Pitaevskii equation for the condensate, which is coupled to the Maxwell equation for the field. The dispersion relations of recoil energy and momentum are calculated, and the effect of weak nonideality of the condensate on the photon recoil is ubraveled. A good agreement between the theory and experiment [7] on the measurement of the photon recoil momentum in a dispersive medium is demonstrated

Investigation of pulse shape neutron-gamma discrimination

The role of neutron beam investigation is significant not only for fundamental science but also for various fields of applied science. This work is dedicated to the formation of neutron beams using the external 18-MeV proton beam of IBA cyclotron C18/18 with a beam current of up to 100 µA. The facility is located at the A. Alikhanyan National Science Laboratory (Yerevan Physics Institute). The possibility to obtain thermal or epithermal neutron beams using the external proton beam of the cyclotron is studied using Geant4 simulations. In this case, a quasimonoenergetic neutron source 9Be (p, n)9B reaction is chosen. As a result of the simulations, the optimal thickness of the 9Be beryllium isotope target is determined. The induced neutron beam is accompanied by a gamma ray background. To decrease the number of accompanying gamma rays, the lead absorber is considered. As a method of separating neutrons from gamma rays, the pulse shape discrimination (PSD) technique is developed. This study shows the possibility of neutron-gamma PSD and its applicability using the EJ-299-33A plastic scintillator

Modeling of laser-induced plasmon effects in GNS-DLC-based material for application in X-ray source array sensors

An important direction in the development of X-ray computed tomography sensors in systems with increased scanning speed and spatial resolution is the creation of an array of miniature current sources. In this paper, we describe a new material based on gold nanostars (GNS) embedded in nanoscale diamond-like carbon (DLC) films (thickness of 20 nm) for constructing a pixel current source with photoinduced electron emission. The effect of localized surface plasmon resonance in GNS on optical properties in the wavelength range from UV to near IR, peculiarities of localization of field and thermal sources, generation of high-energy hot electrons, and mechanisms of their transportation in vacuum are investigated. The advantages of the proposed material and the prospects for using X-ray computed tomography in the matrix source are evaluated

Statistics of low-energy levels of a one-dimensional weakly localized Frenkel exciton: A numerical study

Numerical study of the one-dimensional Frenkel Hamiltonian with on-site randomness is carried out. We focus on the statistics of the energy levels near the lower exciton band edge, i. e. those determining optical response. We found that the distribution of the energy spacing between the states that are well localized at the same segment is characterized by non-zero mean, i.e. these states undergo repulsion. This repulsion results in a local discrete energy structure of a localized Frenkel exciton. On the contrary, the energy spacing distribution for weakly overlapping local ground states (the states with no nodes within their localization segments) that are localized at different segments has zero mean and shows almost no repulsion. The typical width of the latter distribution is of the same order as the typical spacing in the local discrete energy structure, so that this local structure is hidden; it does not reveal itself neither in the density of states nor in the linear absorption spectra. However, this structure affects the two-exciton transitions involving the states of the same segment and can be observed by the pump-probe spectroscopy. We analyze also the disorder degree scaling of the first and second momenta of the distributions.Comment: 10 pages, 6 figure

Superradiance from an ultrathin film of three-level V-type atoms: Interplay between splitting, quantum coherence and local-field effects

We carry out a theoretical study of the collective spontaneous emission (superradiance) from an ultrathin film comprised of three-level atoms with $V$-configuration of the operating transitions. As the thickness of the system is small compared to the emission wavelength inside the film, the local-field correction to the averaged Maxwell field is relevant. We show that the interplay between the low-frequency quantum coherence within the subspace of the upper doublet states and the local-field correction may drastically affect the branching ratio of the operating transitions. This effect may be used for controlling the emission process by varying the doublet splitting and the amount of low-frequency coherence.Comment: 15 pages, 5 figure

Perioperative assessment of cardiological risk in non-cardiac surgical interventions

During the postoperative period, cardiological complications occupy the first position regarding morbidity and mortality rates. They depend on various factors such as compromised cardiovascular history and type of surgical intervention, features and type of anesthesia, water balance and postoperative care of the patient. To prevent complications, one should reply two questions: is there a risk of cardiovascular complications in the perioperative period and how to avoid them. The article presents a review of the literature on current views on the perioperative assessment of cardiac risks in patients undergoing noncardiac surgery

Energetic beams of negative and neutral hydrogen from intense laser plasma interaction

One of the most striking demonstrations of intermolecular forces is the tension at the surface of liquid n-alkanes. The prediction of surface tension is important in the design of distillation towers, extraction units and tower internals such as bubble caps and trays, since it has a considerable influence on the transfer of mass and energy across interfaces. Surface tension data are needed wherever foaming emulsification, droplet formation or wetting are involved. They are also required in a number of equations for two-phase flow calculations and for determining the flow regime. Petroleum engineers are especially interested in the surface tension in the extraction of crude oil to add surfactants to modify the interfacial properties between crude oil and the geological reservoir to improve production and increase oil yields. In this work, a simple computer program using Arrhenius-type asymptotic exponential function, Vandermoned matrix and Matlab technical computing language, is developed for the estimation of surface tension of paraffin hydrocarbons as a function of molecular weight and temperature. The surface tension is calculated for temperatures in the range of 250 to 440 K and paraffin hydrocarbons molecular weights between 30 and 250. The proposed numerical technique is superior owing to its accuracy and clear numerical background, wherein the relevant coefficients can be retuned quickly if more data become available in the future. Estimations are found to be in excellent agreement with the reliable data in the literature with average absolute deviation being less than 2%