Developments in Rare Kaon Decay Physics

We review the current status of the field of rare kaon decays. The study of rare kaon decays has played a key role in the development of the standard model, and the field continues to have significant impact. The two areas of greatest import are the search for physics beyond the standard model and the determination of fundamental standard-model parameters. Due to the exquisite sensitivity of rare kaon decay experiments, searches for new physics can probe very high mass scales. Studies of the k->pnn modes in particular, where the first event has recently been seen, will permit tests of the standard-model picture of quark mixing and CP violation.Comment: One major revision to the text is the branching ratio of KL->ppg, based on a new result from KTeV. Several references were updated, with minor modifications to the text. A total of 48 pages, with 28 figures, in LaTeX; to be published in the Annual Review of Nuclear and Particle Science, Vol. 50, December 200

Raman Adiabatic Transfer of Optical States

We analyze electromagnetically induced transparency and light storage in an ensemble of atoms with multiple excited levels (multi-Lambda configuration) which are coupled to one of the ground states by quantized signal fields and to the other one via classical control fields. We present a basis transformation of atomic and optical states which reduces the analysis of the system to that of EIT in a regular 3-level configuration. We demonstrate the existence of dark state polaritons and propose a protocol to transfer quantum information from one optical mode to another by an adiabatic control of the control fields

Energy transfer in porphyrin-functionalized graphene

We present a theoretical study on the molecule–substrate interaction within the porphyrin-functionalized graphene. Recent experiments on porphyrin-functionalized carbon nanotubes have revealed an extremely efficient energy transfer from the adsorbed molecules to the carbon substrate. To investigate the energy transfer mechanism, we have characterized the hybrid structure within the density functional theory including the calculation of the molecular transition dipole moment, which allows us to determine the Förster coupling rate. We find a strongly pronounced Förster-induced energy transfer in the range of fs−1 inline image confirming the experimental observations

Photoemission spectroscopy and sum rules in dilute electron-phonon systems

A family of exact sum rules for the one-polaron spectral function in the low-density limit is derived. An algorithm to calculate energy moments of arbitrary order of the spectral function is presented. Explicit expressions are given for the first two moments of a model with general electron-phonon interaction, and for the first four moments of the Holstein polaron. The sum rules are linked to experiments on momentum-resolved photoemission spectroscopy. The bare electronic dispersion and the electron-phonon coupling constant can be extracted from the first and second moments of spectrum. The sum rules could serve as constraints in analytical and numerical studies of electron-phonon models.Comment: 4 page

Ab-initio angle and energy resolved photoelectron spectroscopy with time-dependent density-functional theory

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that efficiently gives access to photoelectron spectroscopy in time-dependent density-functional calculations. By using a geometrical approach, we provide a simple description of momentum-resolved photoe- mission including multi-photon effects. The approach is validated by comparison with results in the literature and exact calculations. Furthermore, we present numerical photoelectron angular distributions for randomly oriented nitrogen molecules in a short near infrared intense laser pulse and helium-(I) angular spectra for aligned carbon monoxide and benzene.Comment: Accepted for publication on Phys. Rev.

Quantum coherence and carriers mobility in organic semiconductors

We present a model of charge transport in organic molecular semiconductors based on the effects of lattice fluctuations on the quantum coherence of the electronic state of the charge carrier. Thermal intermolecular phonons and librations tend to localize pure coherent states and to assist the motion of less coherent ones. Decoherence is thus the primary mechanism by which conduction occurs. It is driven by the coupling of the carrier to the molecular lattice through polarization and transfer integral fluctuations as described by the hamiltonian of Gosar and Choi. Localization effects in the quantum coherent regime are modeled via the Anderson hamiltonian with correlated diagonal and non-diagonal disorder leading to the determination of the carrier localization length. This length defines the coherent extension of the ground state and determines, in turn, the diffusion range in the incoherent regime and thus the mobility. The transfer integral disorder of Troisi and Orlandi can also be incorporated. This model, based on the idea of decoherence, allowed us to predict the value and temperature dependence of the carrier mobility in prototypical organic semiconductors that are in qualitative accord with experiments

Complete Characterization of Quantum-Optical Processes

The technologies of quantum information and quantum control are rapidly improving, but full exploitation of their capabilities requires complete characterization and assessment of processes that occur within quantum devices. We present a method for characterizing, with arbitrarily high accuracy, any quantum optical process. Our protocol recovers complete knowledge of the process by studying, via homodyne tomography, its effect on a set of coherent states, i.e. classical fields produced by common laser sources. We demonstrate the capability of our protocol by evaluating and experimentally verifying the effect of a test process on squeezed vacuum.Comment: 5 pages, 4 figure