15 research outputs found

    Temperature-Dependent Electron-Electron Interaction in Graphene on SrTiO3

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    The electron band structure of graphene on SrTiO3 substrate has been investigated as a function of temperature. The high-resolution angle-resolved photoemission study reveals that the spectral width at Fermi energy and the Fermi velocity of graphene on SrTiO3 are comparable to those of graphene on a BN substrate. Near the charge neutrality, the energy-momentum dispersion of graphene exhibits a strong deviation from the well-known linearity, which is magnified as temperature decreases. Such modification resembles the characteristics of enhanced electron-electron interaction. Our results not only suggest that SrTiO3 can be a plausible candidate as a substrate material for applications in graphene-based electronics, but also provide a possible route towards the realization of a new type of strongly correlated electron phases in the prototypical two-dimensional system via the manipulation of temperature and a proper choice of dielectric substrates.Comment: 16 pages, 3 figure

    Probing Inhomogeneous Cuprate Superconductivity by Terahertz Josephson Echo Spectroscopy

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    Inhomogeneities play a crucial role in determining the properties of quantum materials. Yet methods that can measure these inhomogeneities are few, and apply to only a fraction of the relevant microscopic phenomena. For example, the electronic properties of cuprate materials are known to be inhomogeneous over nanometer length scales, although questions remain about how such disorder influences supercurrents and their dynamics. Here, two-dimensional terahertz spectroscopy is used to study interlayer superconducting tunneling in near-optimally-doped La1.83Sr0.17CuO4. We isolate a 2 THz Josephson echo signal with which we disentangle intrinsic lifetime broadening from extrinsic inhomogeneous broadening. We find that the Josephson plasmons are only weakly inhomogeneously broadened, with an inhomogeneous linewidth that is three times smaller than their intrinsic lifetime broadening. This extrinsic broadening remains constant up to 0.7Tc, above which it is overcome by the thermally-increased lifetime broadening. Crucially, the effects of disorder on the Josephson plasma resonance are nearly two orders of magnitude smaller than the in-plane variations in the superconducting gap in this compound, which have been previously documented using Scanning Tunnelling Microscopy (STM) measurements. Hence, even in the presence of significant disorder in the superfluid density, the finite frequency interlayer charge fluctuations exhibit dramatically reduced inhomogeneous broadening. We present a model that relates disorder in the superfluid density to the observed lifetimes

    Research Update: Orbital polarization in LaNiO3-based heterostructures

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    The relative energies and occupancies of valence orbital states can dramatically influence collective electronic and magnetic phenomena in correlated transition metal oxide systems. We review the current state of research on the modification and control of these orbital properties in rare-earth nickelates, especially LaNiO3, a model degenerate d orbital system where significant recent progress has been made. Theoretical and experimental results on thin films and heterostructures are described, including the influence of electronic correlation effects. We highlight the latest approaches to achieving non-degenerate bands and discuss the outlook and applicability of this body of knowledge to other correlated metal oxide systems

    Synthesis of SnTe Nanoplates with {100} and {111} Surfaces

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    SnTe is a topological crystalline insulator that possesses spin-polarized, Dirac-dispersive surface states protected by crystal symmetry. Multiple surface states exist on the {100}, {110}, and {111} surfaces of SnTe, with the band structure of surface states depending on the mirror symmetry of a particular surface. Thus, to access surface states selectively, it is critical to control the morphology of SnTe such that only desired crystallographic surfaces are present. Here, we grow SnTe nanostructures using vapor–liquid–solid and vapor–solid growth mechanisms. Previously, SnTe nanowires and nanocrystals have been grown [Saghir et al. <i>Cryst. Growth Des.</i> <b>2014</b>, <i>14</i>, 2009–2013; Safdar et al. <i>Cryst. Growth Des.</i> <b>2014</b>, <i>14</i>, 2502–2509; Safdar et al. <i>Nano Lett.</i> <b>2013</b>, <i>13</i>, 5344–5349; Li et al. <i>Nano Lett.</i> <b>2013</b>, <i>13</i>, 5443–5448]. In this report, we demonstrate the synthesis of SnTe nanoplates with lateral dimensions spanning tens of micrometers and thicknesses of a few hundred nanometers. The top and bottom surfaces are either (100) or (111), maximizing topological surface states on these surfaces. Magnetotransport on these SnTe nanoplates shows a high bulk carrier density, consistent with bulk SnTe crystals arising due to defects such as Sn vacancies. In addition, we observe a structural phase transition in these nanoplates from the high-temperature rock salt to a low-temperature rhombohedral structure. For nanoplates with a very high carrier density, we observe a slight upturn in resistance at low temperatures, indicating electron–electron interactions

    Temperature-Dependent Electron–Electron Interaction in Graphene on SrTiO<sub>3</sub>

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    The electron band structure of graphene on SrTiO<sub>3</sub> substrate has been investigated as a function of temperature. The high-resolution angle-resolved photoemission study reveals that the spectral width at Fermi energy and the Fermi velocity of graphene on SrTiO<sub>3</sub> are comparable to those of graphene on a BN substrate. Near the charge neutrality, the energy-momentum dispersion of graphene exhibits a strong deviation from the well-known linearity, which is magnified as temperature decreases. Such modification resembles the characteristics of enhanced electron–electron interaction. Our results not only suggest that SrTiO<sub>3</sub> can be a plausible candidate as a substrate material for applications in graphene-based electronics but also provide a possible route toward the realization of a new type of strongly correlated electron phases in the prototypical two-dimensional system via the manipulation of temperature and a proper choice of dielectric substrates
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