Limit on sterile neutrino contribution from the Mainz Neutrino Mass Experiment

The recent analysis of the normalization of reactor antineutrino data, the calibration data of solar neutrino experiments using gallium targets, and the results from the neutrino oscillation experiment MiniBooNE suggest the existence of a fourth light neutrino mass state with a mass of O(eV), which contributes to the electron neutrino with a sizable mixing angle. Since we know from measurements of the width of the Z0 resonance that there are only three active neutrinos, a fourth neutrino should be sterile (i.e., interact only via gravity). The corresponding fourth neutrino mass state should be visible as an additional kink in beta-decay spectra. In this work the phase II data of the Mainz Neutrino Mass Experiment have been analyzed searching for a possible contribution of a fourth light neutrino mass state. No signature of such a fourth mass state has been found and limits on the mass and the mixing of this fourth mass states are derived

Operando real-space imaging of a structural phase transformation in a high-voltage electrode

Discontinuous solid-solid phase transformations play a pivotal role in determining properties of rechargeable battery electrodes. By leveraging operando Bragg Coherent Diffractive Imaging (BCDI), we investigate the discontinuous phase transformation in LixNi0.5Mn1.5O4 within a fully operational battery. Throughout Li-intercalation, we directly observe the nucleation and growth of the Li-rich phase within the initially charged Li-poor phase in a 500 nm particle. Supported by the microelasticity model, the operando imaging unveils an evolution from a curved coherent to planar semi-coherent interface driven by dislocation dynamics. We hypothesize these dislocations exhibit a glissile motion that facilitates interface migration without diffusion of host ions, leaving the particle defect-free post-transformation. Our data indicates negligible kinetic limitations impacting the transformation kinetics, even at discharge rates as fast as C/2. This study underscores BCDI's capability to provide operando insights into nanoscale phase transformations, offering valuable guidance for electrochemical materials design and optimization

APLIKASI TEORI PERILAKU TERENCANA: NIAT MELAKUKAN PHYSICAL EXERCISE (LATIHAN FISIK) PADA REMAJA DI SURABAYA

Alasan utama untuk rnengangkat topik ini dalarn penelitian ia1ah penulis berrnaksud untuk rneneliti variabel-variabel yang rnelatarbelakangi perilaku physical exercise yang dilakukan remaja di Surabaya. Tujuannya, peneliti ingin rnenguji apakah ada hubungan antara attitude towards behavior (A TB), subjective norm (SN), dan perceived behavioral control (PBC), baik secara bersama-sama maupun secara parsial, dengan niat berperilaku physical exercise (latihan fisik) pada remaja di Surabaya. Metode angket digunakan dalarn penelitian ini, rnenggunakan teknik penskalaan sernantik diferensial. Rernaja baik pria dan wanita (N=336) di kota Surabaya berpartisipasi dalarn penelitian ini. Hasil uji hipotesis rnenujukkan bahwa : {a). Terdapat hubungan yang signifikan antara ATB, SN, dan PBC, secara bersarna-sarna terhadap niat rnelakukan Physical exersice pada remaja (F = 14.233; p = 0,000). Hasil korelasi parsial menunjukkan ATB, dan SN menjadi prediktor paling kuat terhadap niat melaku.kan Physical Exercise, sedangkan PBC tidak

Nonequilibrium structural dynamics of nanoparticles in LiNi(1/2)Mn(3/2)O4 cathode under operando conditions.

We study nonequilibrium structural dynamics in LiNi1/2Mn3/2O4 spinel cathode material during fast charge/discharge under operando conditions using coherent X-rays. Our in situ measurements reveal a hysteretic behavior of the structure upon cycling and we directly observe the interplay between different transformation mechanisms: solid solution and two-phase reactions at the single nanoparticle level. For high lithium concentrations solid solution is observed upon both charge and discharge. For low lithium concentration, we find concurrent solid solution and two-phase reactions upon charge, while a pure two-phase reaction is found upon discharge. A delithiation model based on an ionic blockade layer on the particle surface is proposed to explain the distinct structural transformation mechanisms in nonequilibrium conditions. This study addresses the controversy of why two-phase materials show exemplary kinetics and opens new avenues to understand fundamental processes underlying charge transfer, which will be invaluable for developing the next generation battery materials

Strain-induced orbital energy shift in antiferromagnetic RuO2 revealed by resonant elastic x-ray scattering

In its ground state, RuO2 was long thought to be an ordinary metallic paramagnet. Recent neutron and x-ray diffraction revealed that bulk RuO2 is an antiferromagnet (AFM) with TN above 300 K. Furthermore, epitaxial strain induces novel superconductivity in thin films of RuO2 below 2 K. Here, we present a resonant elastic x-ray scattering (REXS) study at the Ru L2 edge of the strained RuO2 films exhibiting the strain-induced superconductivity. We observe an azimuthal modulation of the 100 Bragg peak consistent with canted AFM found in bulk. Most notably, in the strained films displaying novel superconductivity, we observe a ~1 eV shift of the Ru eg orbitals to a higher energy. The energy shift is smaller in thicker, relaxed films and films with a different strain direction. Our results provide further evidence of the utility of epitaxial strain as a tuning parameter in complex oxides.Comment: 20 pages, 3 main figures, 3 supplementary figure

Disorder Dynamics in Battery Nanoparticles During Phase Transitions Revealed by Operando Single-Particle Diffraction

Structural and ion-ordering phase transitions limit the viability of sodium-ion intercalation materials in grid scale battery storage by reducing their lifetime. However, the combination of phenomena in nanoparticulate electrodes creates complex behavior that is difficult to investigate, especially on the single nanoparticle scale under operating conditions. In this work, operando single-particle x-ray diffraction (oSP-XRD) is used to observe single-particle rotation, interlayer spacing, and layer misorientation in a functional sodium-ion battery. oSP-XRD is applied to Na$_{2/3}$[Ni$_{1/3}$Mn$_{2/3}$]O$_{2}$, an archetypal P2-type sodium-ion positive electrode material with the notorious P2-O2 phase transition induced by sodium (de)intercalation. It is found that during sodium extraction, the misorientation of crystalline layers inside individual particles increases before the layers suddenly align just prior to the P2-O2 transition. The increase in the long-range order coincides with an additional voltage plateau signifying a phase transition prior to the P2-O2 transition. To explain the layer alignment, a model for the phase evolution is proposed that includes a transition from localized to correlated Jahn-Teller distortions. The model is anticipated to guide further characterization and engineering of sodium-ion intercalation materials with P2-O2 type transitions. oSP-XRD therefore opens a powerful avenue for revealing complex phase behavior in heterogeneous nanoparticulate systems.Comment: 23 pages, 4 main figures, 9 supplemental figure

Critical slowing of the spin and charge density wave order in thin film Cr following photoexcitation

We report on the evolution of the charge density wave (CDW) and spin density wave (SDW) order of a chromium film following photoexcitation with an ultrafast optical laser pulse. The CDW is measured by ultrafast time-resolved x-ray diffraction of the CDW satellite that tracks the suppression and recovery of the CDW following photoexcitation. We find that as the temperature of the film approaches a discontinuous phase transition in the CDW and SDW order, the time scales of recovery increase exponentially from the expected thermal time scales. We extend a Landau model for SDW systems to account for this critical slowing with the appropriate boundary conditions imposed by the geometry of the thin film system. This model allows us to assess the energy barrier between available CDW/SDW states with different spatial periodicities.Comment: Author typo fixe