Diffusion-induced dissipation and mode coupling in nanomechanical resonators

We study a system consisting of a particle adsorbed on a carbon nanotube resonator. The particle is allowed to diffuse along the resonator, in order to enable study of e.g. room temperature mass sensing devices. The system is initialized in a state where only the fundamental vibration mode is excited, and the ring-down of the system is studied by numerically and analytically solving the stochastic equations of motion. We find two mechanisms of dissipation, induced by the diffusing adsorbate. First, short-time correlations between particle and resonator motions means that the net effect of the former on the latter does not average out, but instead causes dissipation of vibrational energy. For vibrational amplitudes that are much larger than the thermal energy this dissipation is linear; for small amplitudes the decay takes the same form as that of a nonlinearly damped oscillator. Second, the particle diffusion mediates a coupling between vibration modes, enabling energy transfer from the fundamental mode to excited modes, which rapidly reach thermal equilibrium.Comment: 8 pages, 7 figure

Noise-tunable nonlinearity in a dispersively coupled diffusion-resonator system using superconducting circuits

The harmonic oscillator is one of the most widely used model systems in physics: an indispensable theoretical tool in a variety of fields. It is well known that otherwise linear oscillators can attain novel and nonlinear features through interaction with another dynamical system. We investigate such an interacting system: a superconducting LC-circuit dispersively coupled to a superconducting quantum interference device (SQUID). We find that the SQUID phase behaves as a classical two-level system, whose two states correspond to one linear and one nonlinear regime for the LC-resonator. As a result, the circuit's response to forcing can become multistable. The strength of the nonlinearity is tuned by the level of noise in the system, and increases with decreasing noise. This tunable nonlinearity could potentially find application in the field of sensitive detection, whereas increased understanding of the classical harmonic oscillator is relevant for studies of the quantum-to-classical crossover of Jaynes-Cummings systems.Comment: 8 pages, 8 figure

Diffraction and near-zero transmission of flexural phonons at graphene grain boundaries

Graphene grain boundaries are known to affect phonon transport and thermal conductivity, suggesting that they may be used to engineer the phononic properties of graphene. Here, the effect of two buckled grain boundaries on long-wavelength flexural acoustic phonons has been investigated as a function of angle of incidence using molecular dynamics. The flexural acoustic mode has been chosen due to its importance to thermal transport. It is found that the transmission through the boundaries is strongly suppressed for incidence angles close to 35$^\circ$. Also, the grain boundaries are found to act as diffraction gratings for the phonons

Scattering of flexural acoustic phonons at grain boundaries in graphene

We investigate the scattering of long-wavelength flexural phonons against grain boundaries in graphene using molecular dynamics simulations. Three symmetric tilt grain boundaires are considered: one with a misorientation angle of $17.9^\circ$ displaying an out-of-plane buckling 1.5 nm high and 5 nm wide, one with a misorientation angle of $9.4^\circ$ and an out-of-plane buckling 0.6 nm high and 1.7 nm wide, and one with a misorientation angle of $32.2^\circ$ and no out-of-plane buckling. At the flat grain boundary, the phonon transmission exceeds 95 % for wavelengths above 1 nm. The buckled boundaries have a substantially lower transmission in this wavelength range, with a minimum transmission of 20 % for the $17.9^\circ$ boundary and 40 % for the $9.4^\circ$ boundary. At the buckled boundaries, coupling between flexural and longitudinal phonon modes is also observed. The results indicate that scattering of long-wavelength flexural phonons at grain boundaries in graphene is mainly due to out-of-plane buckling. A continuum mechanical model of the scattering process has been developed, providing a deeper understanding of the scattering process as well as a way to calculate the effect of a grain boundary on long-wavelength flexural phonons based on the buckling size.Comment: 11 pages, 14 figure

Nonlinear phononics using atomically thin membranes

Phononic crystals and acoustic meta-materials are used to tailor phonon and sound propagation properties by facilitating artificial, periodic structures. Analogous to photonic crystals, phononic band gaps can be created, which influence wave propagation and, more generally, allow engineering of the acoustic properties of a system. Beyond that, nonlinear phenomena in periodic structures have been extensively studied in photonic crystals and atomic Bose-Einstein Condensates in optical lattices. However, creating nonlinear phononic crystals or nonlinear acoustic meta-materials remains challenging and only few examples have been demonstrated. Here we show that atomically thin and periodically pinned membranes support coupled localized modes with nonlinear dynamics. The proposed system provides a platform for investigating nonlinear phononics

Multi-phonon relaxation and generation of quantum states in a nonlinear mechanical oscillator

The dissipative quantum dynamics of an anharmonic oscillator is investigated theoretically in the context of carbon-based nano-mechanical systems. In the short-time limit, it is known that macroscopic superposition states appear for such oscillators. In the long-time limit, single and multi-phonon dissipation lead to decoherence of the non-classical states. However, at zero temperature, as a result of two-phonon losses the quantum oscillator eventually evolves into a non-classical steady state. The relaxation of this state due to thermal excitations and one-phonon losses is numerically and analytically studied. The possibility of verifying the occurrence of the non-classical state is investigated and signatures of the quantum features arising in a ring-down setup are presented. The feasibility of the verification scheme is discussed in the context of quantum nano-mechanical systems.Comment: 23 pages, 8 figures; Minor revisions; Accepted for publication in NJ

Nanoscale Elasto-Capillarity in the Graphene-Water System under Tension: Revisiting the Assumption of a Constant Wetting Angle

Wetting highly compliant surfaces can cause them to deform. Atomically thin materials, such as graphene, can have exceptionally small bending rigidities, leading to elasto-capillary lengths of a few nanometers. Using large-scale molecular dynamics (MD), we have studied the wetting and deformation of graphene due to nanometer-sized water droplets, focusing on the wetting angle near the vesicle transition. Recent continuum theories for wetting of flexible membranes reproduce our MD results qualitatively well. However, we find that when the curvature is large at the triple-phase contact line, the wetting angle increases with decreasing tension. This is in contrast to existing macroscopic theories but can be amended by allowing for a variable wetting angle

Strong mechanically-induced effects in DC current-biased suspended Josephson junctions

Superconductivity is a result of quantum coherence at macroscopic scales. Two superconductors separated by a metallic or insulating weak link exhibit the AC Josephson effect - the conversion of a DC voltage bias into an AC supercurrent. This current may be used to activate mechanical oscillations in a suspended weak link. As the DC voltage bias condition is remarkably difficult to achieve in experiments, here we analyse theoretically how the Josephson effect can be exploited to activate and detect mechanical oscillations in the experimentally relevant condition with purely DC current bias. We unveil for the first time how changing the strength of the electromechanical coupling results in two qualitatively different regimes showing dramatic effects of the oscillations on the DC current-voltage characteristic of the device. These include the apperance of Shapiro-like plateaux for weak coupling and a sudden mechanically-induced retrapping for strong coupling. Our predictions, measurable in state of the art experimental setups, allow the determination of the frequency and quality factor of the resonator using DC only techniques.Comment: 10 pages, 6 figure

FPU physics with nanomechanical graphene resonators: intrinsic relaxation and thermalization from flexural mode coupling

Thermalization in nonlinear systems is a central concept in statistical mechanics and has been extensively studied theoretically since the seminal work of Fermi, Pasta and Ulam (FPU). Using molecular dynamics and continuum modeling of a ring-down setup, we show that thermalization due to nonlinear mode coupling intrinsically limits the quality factor of nanomechanical graphene drums and turns them into potential test beds for FPU physics. We find the thermalization rate $\Gamma$ to be independent of radius and scaling as $\Gamma\sim T^*/\epsilon_{{\rm pre}}^2$, where $T^*$ and $\epsilon_{{\rm pre}}$ are effective resonator temperature and prestrain