734 research outputs found
Electron Glass Dynamics
Examples of glasses are abundant, yet it remains one of the phases of matter
whose understanding is very elusive. In recent years, remarkable experiments
have been performed on the dynamical aspects of glasses. Electron glasses offer
a particularly good example of the 'trademarks' of glassy behavior, such as
aging and slow relaxations. In this work we review the experimental literature
on electron glasses, as well as the local mean-field theoretical framework put
forward in recent years to understand some of these results. We also present
novel theoretical results explaining the periodic aging experiment.Comment: Invited review to appear in Annual Review of Condensed Matter Physic
Non-exponential relaxation for anomalous diffusion
We study the relaxation process in normal and anomalous diffusion regimes for
systems described by a generalized Langevin equation (GLE). We demonstrate the
existence of a very general correlation function which describes the relaxation
phenomena. Such function is even; therefore, it cannot be an exponential or a
stretched exponential. However, for a proper choice of the parameters, those
functions can be reproduced within certain intervals with good precision. We
also show the passage from the non-Markovian to the Markovian behaviour in the
normal diffusion regime. For times longer than the relaxation time, the
correlation function for anomalous diffusion becomes a power law for broad-band
noise.Comment: 6 pages, 2 figure
Twist glass transition in regioregulated poly(3-alkylthiophenes)s
The molecular structure and dynamics of regioregulated poly(3-butylthiophene)
(P3BT), poly(3-hexylthiophene)(P3HT), and poly(3-dodecylthiophene) (P3DDT) were
investigated using Fourier transform infrared absorption (FTIR), solid state
C nuclear magnetic resonance (NMR), and differential scanning
calorimetry (DSC) measurements. In the DSC measurements, the endothermic peak
was obtained around 340 K in P3BT, and assigned to enthalpy relaxation that
originated from the glass transition of the thiophene ring twist in crystalline
phase from results of FTIR, C cross-polarization and magic-angle
spinning (CPMAS) NMR, C spin-lattice relaxation time measurements, and
centerband-only detection of exchange (CODEX) measurements. We defined this
transition as {\it twist-glass transition}, which is analogous to the plastic
crystal - glassy crystal transition.Comment: 9 pages, 10 figures, 2 tables. Phys.Rev.B, in pres
A Hybrid model for the origin of photoluminescence from Ge nanocrystals in SiO matrix
In spite of several articles, the origin of visible luminescence from
germanium nanocrystals in SiO matrix is controversial even today. Some
authors attribute the luminescence to quantum confinement of charge carriers in
these nanocrystals. On the other hand, surface or defect states formed during
the growth process, have also been proposed as the source of luminescence in
this system. We have addressed this long standing query by simultaneous
photoluminescence and Raman measurements on germanium nanocrystals embedded in
SiO matrix, grown by two different techniques: (i) low energy
ion-implantation and (ii) atom beam sputtering. Along with our own experimental
observations, we have summarized relevant information available in the
literature and proposed a \emph{Hybrid Model} to explain the visible
photoluminescence from nanocrystalline germanium in SiO matrix.Comment: 23 pages, 8 figure
Bit-rate saving in multichannel sound:using a band-limited channel to transmit the center signal
A method is proposed to achieve full-frequency-range three-channel (left, right, and center) sound reproduction in systems that have only two full-range sound channels and some band-limited commentary channels. The low-frequency part of the center signal, which matches the bandwidth of the commentary channels, is added to the (multilingual) speech signals in each of the commentary channels. The remaining high-frequency part is added in the left and right channels as in conventional mixdowns. Sound reproduction of this signal by a conventional two-channel receiver remains unaltered. The low-frequency part of the center signal is mixed to the left and right signals together with the speech once the user has selected a commentary channel. Three-channel reproduction is obtained by routing the selected commentary channel to a central loudspeaker. Listening tests revealed that sound reproduction according to the proposed scheme could not be distinguished from original three-channel reproduction. This scheme can be applied to proposed standards such as D2MAC and MPEG2.</p
Rotational Brownian motion on the sphere surface and rotational relaxation
The spatial components of the autocorrelation function of noninteracting
dipoles are analytically obtained in terms of rotational Brownian motion on the
surface of a unit sphere using multi-level jumping formalism based on Debye's
rotational relaxation model, and the rotational relaxation functions are
evaluated.Comment: RevTex, 4 pages, submitted to Chin. Phys. Let
Relaxation properties in a lattice gas model with asymmetrical particles
We study the relaxation process in a two-dimensional lattice gas model, where
the interactions come from the excluded volume. In this model particles have
three arms with an asymmetrical shape, which results in geometrical frustration
that inhibits full packing. A dynamical crossover is found at the arm
percolation of the particles, from a dynamical behavior characterized by a
single step relaxation above the transition, to a two-step decay below it.
Relaxation functions of the self-part of density fluctuations are well fitted
by a stretched exponential form, with a exponent decreasing when the
temperature is lowered until the percolation transition is reached, and
constant below it. The structural arrest of the model seems to happen only at
the maximum density of the model, where both the inverse diffusivity and the
relaxation time of density fluctuations diverge with a power law. The dynamical
non linear susceptibility, defined as the fluctuations of the self-overlap
autocorrelation, exhibits a peak at some characteristic time, which seems to
diverge at the maximum density as well.Comment: 7 pages and 9 figure
Towards ultra-high resolution 3D reconstruction of a whole rat brain from 3D-PLI data
3D reconstruction of the fiber connectivity of the rat brain at microscopic
scale enables gaining detailed insight about the complex structural
organization of the brain. We introduce a new method for registration and 3D
reconstruction of high- and ultra-high resolution (64 m and 1.3 m
pixel size) histological images of a Wistar rat brain acquired by 3D polarized
light imaging (3D-PLI). Our method exploits multi-scale and multi-modal 3D-PLI
data up to cellular resolution. We propose a new feature transform-based
similarity measure and a weighted regularization scheme for accurate and robust
non-rigid registration. To transform the 1.3 m ultra-high resolution data
to the reference blockface images a feature-based registration method followed
by a non-rigid registration is proposed. Our approach has been successfully
applied to 278 histological sections of a rat brain and the performance has
been quantitatively evaluated using manually placed landmarks by an expert.Comment: 9 pages, Accepted at 2nd International Workshop on Connectomics in
NeuroImaging (CNI), MICCAI'201
The InfraâRed Absorption Spectrum of Propane
Of the twentyâseven internal degrees of freedom of propane, all nondegenerate, twentyâtwo may appear as fundamental absorption bands. These bands fall into three symmetry classes, designated A1, B1 and B2, and distinguishable by their characteristic contours. Because of overlapping, however, it is impossible in many cases to determine their positions precisely. This is especially true in the regions of the CâH valence and deformation frequencies. Some ten or twelve fundamental bands may be identified with confidence as well as a number of combinations. An A1 band at 870 cmâ1 and a B2 band at 748 cmâ1 have been partially resolved, the line spacing being about 1.47 cmâ1 in agreement with predictions based upon electron diffraction measurements. The fine structure of the B1 bands has not been observed (the predicted spacing is 0.5 cmâ1) but the interval between maxima of the P and R branches is approximately 26 cmâ1 as expected. With 24 cmâatmospheres of gas no bands were observed between 15ÎŒ and 35ÎŒ, although the symmetrical CâC deformation might be expected to produce a band of appreciable intensity within these limits. This frequency has apparently been observed in Raman spectra at 375 cmâ1.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/70815/2/JCPSA6-9-7-487-1.pd
The Spin Glass Transition : Exponents and Dynamics
Numerical simulations on Ising Spin Glasses show that spin glass transitions
do not obey the usual universality rules which hold at canonical second order
transitions. On the other hand the dynamics at the approach to the transition
appear to take up a universal form for all spin glasses. The implications for
the fundamental physics of transitions in complex systems are addressed.Comment: 4 pages (Latex) with 3 figures (postscript), accepted for publication
in Physica
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