Strong coupling between Eu2+ spins and Fe2As2 layers in EuFe1.9Co0.1As2 observed with NMR

A combination of x-ray diffraction, magnetization, and 75As nuclear magnetic resonance (NMR) experiments were performed on single-crystal EuFe1.9Co0.1As2. The strength of the hyperfine interaction between the 75As nuclei and the Eu^(2+) 4f states suggests a strong coupling between the Eu^(2+) moments and the Fe1.9Co0.1As2 layers. Such a strong interlayer coupling may be due to an indirect exchange interaction between the localized Eu^(2+) 4f moments, mediated by the Fe 3d conduction electrons. Magnetic susceptibility as well as 75As-NMR measurements reveal a decrease of the SDW transition temperature to T_SDW = 120 K as a result of Co doping. A change of the slope in the temperature dependence of the NMR frequency of the 75As lower-satellite line was observed at 225 K. At the same temperature also a change of the satellite line shape was found. These changes of the NMR spectra may be caused by the formation of a nematic phase below 225 K in EuFe1.9Co0.1As2.Comment: 8 pages, 7 figure

Giant microwave absorption in fine powders of superconductors

Enhanced microwave absorption, larger than that in the normal state, is observed in fine grains of type-II superconductors (MgB$_2$ and K$_3$C$_{60}$) for magnetic fields as small as a few $\%$ of the upper critical field. The effect is predicted by the theory of vortex motion in type-II superconductors, however its direct observation has been elusive due to skin-depth limitations; conventional microwave absorption studies employ larger samples where the microwave magnetic field exclusion significantly lowers the absorption. We show that the enhancement is observable in grains smaller than the penetration depth. A quantitative analysis on K$_3$C$_{60}$ in the framework of the Coffey--Clem (CC) theory explains well the temperature dependence of the microwave absorption and also allows to determine the vortex pinning force constant

Muon Spin Rotation Study of the Intercalated Graphite Superconductor CaC6 at Low Temperatures

Muon spin rotation (μSR) experiments were performed on the intercalated graphite CaC6 in the normal and superconducting state down to 20mK. In addition, AC magnetization measurements were carried out resulting in an anisotropic upper critical field $H_{\text{c2}}$ , from which the coherence lengths ξ ab (0)=36.3(1.5)nm and ξ c (0)=4.3(7)nm were estimated. The anisotropy parameter $\gamma _{H}=H_{\text{c2}}^{ab}/H_{\text{c2}}^{c}$ increases monotonically with decreasing temperature. Asingle isotropic s-wave description of superconductivity cannot account for this behavior. From magnetic field dependent μSR experiments, the absolute value of the in-plane magnetic penetration depth λ ab (0)=78(3)nm was determined. The temperature dependence of the superfluid density ρ s (T) is slightly better described by a two-gap than a single-gap mode

Generalized Elliott-Yafet theory of electron spin relaxation in metals: the origin of the anomalous electron spin life-time in MgB2

The temperature dependence of the electron spin relaxation time in MgB2 is anomalous as it does not follow the temperature dependence of the resistivity above 150 K, it has a maximum around 400 K, and it decreases for higher temperatures. This violates the well established Elliot-Yafet theory of electron spin relaxation in metals. We show that the anomaly occurs when the quasi-particle scattering rate (in energy units) becomes comparable to the energy difference between the conduction- and a neighboring band. We find that the anomalous behavior is related to the unique band structure of MgB$_2$ and the large electron-phonon coupling. The saturating spin-lattice relaxation can be regarded as the spin transport analogue of the Ioffe-Regel criterion of electron transport

Magnetic resonance in the antiferromagnetic and normal state of NH_3K_3C_60

We report on the magnetic resonance of NH_3K_3C_60 powders in the frequency range of 9 to 225 GHz. The observation of an antiferromagnetic resonance below the phase transition at 40 K is evidence for an antiferromagnetically ordered ground state. In the normal state, above 40 K, the temperature dependence of the spin-susceptibilty measured by ESR agrees with previous static measurements and is too weak to be explained by interacting localized spins in an insulator. The magnetic resonance line width has an unusual magnetic-field dependence which is large and temperature independent in the magnetically ordered state and decreases rapidly above the transition. These observations agree with the suggestion that NH_3K_3C_60 is a metal in the normal state and undergoes a Mott-Hubbard metal to insulator transition at 40 K.Comment: 4 pages, 5 figures. Submitted to Phys. Rev.

Anisotropy of superconducting MgB2 as seen in electron spin resonance and magnetization data

We have observed the conduction electron spin resonance (CESR) in fine powders of MgB2 both in the superconducting and normal states. The Pauli susceptibility is chi_s=2.0*10^{-5} emu/mole in the temperature range of 450 to 600 K. The spin relaxation rate has an anomalous temperature dependence. The CESR measured below T_c at several frequencies suggests that MgB_2 is a strongly anisotropic superconductor with the upper critical field, H_c2, ranging between 2 and 16 T. The high-field reversible magnetization data of a randomly oriented powder sample are well described assuming that MgB_2 is an anisotropic superconductor with H_c2^{ab} / H_{c2}^{c} \approx 6--9.Comment: 4 pages, 4 eps figure