146 research outputs found
A position- and time-sensitive photon-counting detector with delay-line read-out
We have developed image intensifier tubes with delay-anode read-out for time-
and position-sensitive photon counting. The timing precision is better than 1
ns with 1000x1000 pixels position resolution and up to one megacounts/s
processing rate. Large format detectors of 40 and 75 mm active diameter with
internal helical-wire delay-line anodes have been produced and specified. A
different type of 40 and 25 mm tubes with semi-conducting screen for image
charge read-out allow for an economic and robust tube design and for placing
the read-out anodes outside the sealed housing. Two types of external
delay-line anodes, i.e. pick-up electrodes for the image charge, have been
tested. We present tests of the detector and anode performance. Due to the low
background this technique is well suited for applications with very low light
intensity and especially if a precise time tagging for each photon is required.
As an example we present the application of scintillator read-out in
time-of-flight (TOF) neutron radiography. Further applications so far are
Fluorescence Life-time Microscopy (FLIM) and AstronomyComment: Proceedings of SPIE Conference "Optics and Optoelectronics", 16 - 19.
Apr.200
Molecular frame photoelectron angular distribution for oxygen 1s photoemission from CO_2 molecules
We have measured photoelectron angular distributions in the molecular frame (MF-PADs) for O 1s photoemission from CO2, using photoelectron-O+–CO+ coincidence momentum imaging. Results for the molecular axis at 0, 45 and 90° to the electric vector of the light are reported. The major features of the MF-PADs are fairly well reproduced by calculations employing a relaxed-core Hartree–Fock approach. Weak asymmetric features are seen through a plane perpendicular to the molecular axis and attributed to symmetry lowering by anti-symmetric stretching motion
Multiorbital tunneling ionization of the CO molecule
We coincidently measure the molecular frame photoelectron angular
distribution and the ion sum-momentum distribution of single and double
ionization of CO molecules by using circularly and elliptically polarized
femtosecond laser pulses, respectively. The orientation dependent ionization
rates for various kinetic energy releases allow us to individually identify the
ionizations of multiple orbitals, ranging from the highest occupied to the next
two lower-lying molecular orbitals for various channels observed in our
experiments. Not only the emission of a single electron, but also the
sequential tunneling dynamics of two electrons from multiple orbitals are
traced step by step. Our results confirm that the shape of the ionizing
orbitals determine the strong laser field tunneling ionization in the CO
molecule, whereas the linear Stark effect plays a minor role.Comment: This paper has been accepted for publication by Physical Review
Letter
Breakdown of the Two-Step Model in K-Shell Photoemission and Subsequent Decay Probed by the Molecular-Frame Photoelectron Angular Distributions of CO_2
We report results of measurements and of Hartree-Fock level calculations of molecular-frame photoelectron angular distributions (MFPADs) for C 1s photoemission from CO2. The agreement between the measured and calculated MFPADs is on average reasonable. The measured MFPADs display a weak but definite asymmetry with respect to the O+ and CO+ fragment ions at certain energies, providing evidence for an overlap of gerade and ungerade final ionic states giving rise to a partial breakdown of the two-step model of core-level photoionization and its subsequent Auger decay
Carbon K-shell photoelectron angular distribution from fixed-in-space CO2 molecules
Measurements of photoelectron angular distributions for carbon K-shell ionization of fixed-in-space CO2 molecules with the molecular axis oriented along, perpendicular and at 45 degrees to the electric vector of the light are reported. The major features of these measured spectra are fairly well reproduced by calculations employing a relaxed-core Hartree-Fock approach. In contrast to the angular distribution for K-shell ionization of N-2, which exhibits a rich structure dominated by the f-wave (l = 3) at the shape resonance, the angular distribution for carbon K-shell photoionization of CO2 is quite unstructured over the entire observed range across the shape resonance
Carbon K-shell Photo Ionization of CO: Molecular frame angular Distributions of normal and conjugate shakeup Satellites
We have measured the molecular frame angular distributions of photoelectrons
emitted from the Carbon K shell of fixed-in-space CO molecules for the case of
simultaneous excitation of the remaining molecular ion. Normal and conjugate
shake up states are observed. Photo electrons belonging to normal \Sigma
-satellite lines show an angular distribution resembling that observed for the
main photoline at the same electron energy. Surprisingly a similar shape is
found for conjugate shake up states with \Pi -symmetry. In our data we identify
shake rather than electron scattering (PEVE) as the mechanism producing the
conjugate lines. The angular distributions clearly show the presence of a
\Sigma -shape resonance for all of the satellite lines.Comment: 8 pages, 2 figure
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