50,744 research outputs found
Visualizing Exotic Orbital Texture in the Single-Layer Mott Insulator 1T-TaSe2
Mott insulating behavior is induced by strong electron correlation and can
lead to exotic states of matter such as unconventional superconductivity and
quantum spin liquids. Recent advances in van der Waals material synthesis
enable the exploration of novel Mott systems in the two-dimensional limit. Here
we report characterization of the local electronic properties of single- and
few-layer 1T-TaSe2 via spatial- and momentum-resolved spectroscopy involving
scanning tunneling microscopy and angle-resolved photoemission. Our combined
experimental and theoretical study indicates that electron correlation induces
a robust Mott insulator state in single-layer 1T-TaSe2 that is accompanied by
novel orbital texture. Inclusion of interlayer coupling weakens the insulating
phase in 1T-TaSe2, as seen by strong reduction of its energy gap and quenching
of its correlation-driven orbital texture in bilayer and trilayer 1T-TaSe2. Our
results establish single-layer 1T-TaSe2 as a useful new platform for
investigating strong correlation physics in two dimensions
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Modeling singular mineralization processes due to fluid pressure fluctuations
Mineralization in the Earth's crust can be regarded as a singular process resulting in large amounts of mass accumulation and element enrichment over short time or space scales. The elemental concentrations modeled by fractals and multifractals show self-similarity and scale-invariant properties. We take the view that fluid-pressure variations in response to earthquakes or fault rupture are primarily responsible for changes in solubility and trigger transient physical and chemical variations in ore-forming fluids that enhance the mineralization process. Based on this general concept, we investigated mineral precipitation processes driven by rapid fluid pressure reductions by coupling mineralization to a cellular automaton model to reveal the nonlinear mechanism of the orogenic gold mineralization process using simulation. In the model, fluid pressure can increase to the rock failure condition, which was set as lithostatic pressure at a depth of 10 km (270 MPa), due to either porosity reduction or dehydration reactions. Rapid drops in pressure resulting from fault rupture or local hydrofracture may induce repeated gold precipitation. The geochemical patterns generated by the model evolve from depletion to enrichment patterns, and from spatially random to spatially clustered structures quantified by multifractal models and geostatistics. Results show how metal elements self-organize to form high metal concentration patterns displaying self-similarity and scale-invariance. These transitions are attributed to the growth and coalescence of sub-networks with different fluid pressures up to the percolation threshold, resulting in a wide range of fluid pressure reductions and gold precipitation in the form of clusters. The results suggest that cyclic evolution of fluid pressure and its effects on gold precipitation systems can effectively mimic the repeated mineralization superposition process, and generate complex geochemical patterns characterized by a multifractal model. The nonlinear behavior exhibits scale-invariance and self-organized critical threshold, where mineral phase separations result from fluid pressure reductions associated with fault failure
Localization and Coherence in Nonintegrable Systems
We study the irreversible dynamics of nonlinear, nonintegrable Hamiltonian
oscillator chains approaching their statistical asympotic states. In systems
constrained by more than one conserved quantity, the partitioning of the
conserved quantities leads naturally to localized and coherent structures. If
the phase space is compact, the final equilibrium state is governed by entropy
maximization and the final coherent structures are stable lumps. In systems
where the phase space is not compact, the coherent structures can be collapses
represented in phase space by a heteroclinic connection to infinity.Comment: 41 pages, 15 figure
MITK-ModelFit: A generic open-source framework for model fits and their exploration in medical imaging -- design, implementation and application on the example of DCE-MRI
Many medical imaging techniques utilize fitting approaches for quantitative
parameter estimation and analysis. Common examples are pharmacokinetic modeling
in DCE MRI/CT, ADC calculations and IVIM modeling in diffusion-weighted MRI and
Z-spectra analysis in chemical exchange saturation transfer MRI. Most available
software tools are limited to a special purpose and do not allow for own
developments and extensions. Furthermore, they are mostly designed as
stand-alone solutions using external frameworks and thus cannot be easily
incorporated natively in the analysis workflow. We present a framework for
medical image fitting tasks that is included in MITK, following a rigorous
open-source, well-integrated and operating system independent policy. Software
engineering-wise, the local models, the fitting infrastructure and the results
representation are abstracted and thus can be easily adapted to any model
fitting task on image data, independent of image modality or model. Several
ready-to-use libraries for model fitting and use-cases, including fit
evaluation and visualization, were implemented. Their embedding into MITK
allows for easy data loading, pre- and post-processing and thus a natural
inclusion of model fitting into an overarching workflow. As an example, we
present a comprehensive set of plug-ins for the analysis of DCE MRI data, which
we validated on existing and novel digital phantoms, yielding competitive
deviations between fit and ground truth. Providing a very flexible environment,
our software mainly addresses developers of medical imaging software that
includes model fitting algorithms and tools. Additionally, the framework is of
high interest to users in the domain of perfusion MRI, as it offers
feature-rich, freely available, validated tools to perform pharmacokinetic
analysis on DCE MRI data, with both interactive and automatized batch
processing workflows.Comment: 31 pages, 11 figures URL: http://mitk.org/wiki/MITK-ModelFi
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Multi-scale cellular engineering: From molecules to organ-on-a-chip.
Recent technological advances in cellular and molecular engineering have provided new insights into biology and enabled the design, manufacturing, and manipulation of complex living systems. Here, we summarize the state of advances at the molecular, cellular, and multi-cellular levels using experimental and computational tools. The areas of focus include intrinsically disordered proteins, synthetic proteins, spatiotemporally dynamic extracellular matrices, organ-on-a-chip approaches, and computational modeling, which all have tremendous potential for advancing fundamental and translational science. Perspectives on the current limitations and future directions are also described, with the goal of stimulating interest to overcome these hurdles using multi-disciplinary approaches
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