Spin characterization and control over the regime of radiation-induced zero-resistance states

Over the regime of the radiation-induced zero-resistance states and associated oscillatory magnetoresistance, we propose a low magnetic field analog of quantum-Hall-limit techniques for the electrical detection of electron spin- and nuclear magnetic- resonance, dynamical nuclear polarization via electron spin resonance, and electrical characterization of the nuclear spin polarization via the Overhauser shift. In addition, beats observed in the radiation-induced oscillatory-magnetoresistance are developed into a method to measure and control the zero-field spin splitting due to the Bychkov-Rashba and bulk inversion asymmetry terms in the high mobility GaAs/AlGaAs system.Comment: IEEE Transactions in Nanotechnology (to be published); 10 pages, 10 color figure

Spin-flip and spin-conserving optical transitions of the nitrogen-vacancy centre in diamond

We map out the first excited state sublevel structure of single nitrogen-vacancy (NV) colour centres in diamond. The excited state is an orbital doublet where one branch supports an efficient cycling transition, while the other can simultaneously support fully allowed optical Raman spin-flip transitions. This is crucial for the success of many recently proposed quantum information applications of the NV defects. We further find that an external electric field can be used to completely control the optical properties of a single centre. Finally, a group theoretical model is developed that explains the observations and provides good physical understanding of the excited state structure

Applications of quantum cryptographic switch: Various tasks related to controlled quantum communication can be performed using Bell states and permutation of particles

Recently, several aspects of controlled quantum communication (e.g., bidirectional controlled state teleportation, controlled quantum secure direct communication, controlled quantum dialogue, etc.) have been studied using $n$-qubit ($n\geq3$) entanglement. Specially, a large number of schemes for bidirectional controlled state teleportation are proposed using $m$-qubit entanglement ($m\in\{5,6,7\}$). Here, we propose a set of protocols to illustrate that it is possible to realize all these tasks related to controlled quantum communication using only Bell states and permutation of particles (PoP). As the generation and maintenance of a Bell state is much easier than a multi-partite entanglement, the proposed strategy has a clear advantage over the existing proposals. Further, it is shown that all the schemes proposed here may be viewed as applications of the concept of quantum cryptographic switch which was recently introduced by some of us. The performances of the proposed protocols as subjected to the amplitude damping and phase damping noise on the channels are also discussed.Comment: 12 pages, 3 figure

On the group theoretic structure of a class of quantum dialogue protocols

Intrinsic symmetry of the existing protocols of quantum dialogue are explored. It is shown that if we have a set of mutually orthogonal $n$-qubit states {\normalsize $\{|\phi_{0}>,|\phi_{1}>,....,|\phi_{i}\}$ and a set of $m-qubit$ ($m\leq n$) unitary operators $\{U_{0},U_{2},...,U_{2^{n}-1}\}:U_{i}|\phi_{0}>=|\phi_{i}>$ and $\{U_{0},U_{2},...,U_{2^{n}-1}\}$ forms a group under multiplication then it would be sufficient to construct a quantum dialogue protocol using this set of quantum states and this group of unitary operators}. The sufficiency condition is used to provide a generalized protocol of quantum dialogue. Further the basic concepts of group theory and quantum mechanics are used here to systematically generate several examples of possible groups of unitary operators that may be used for implementation of quantum dialogue. A large number of examples of quantum states that may be used to implement the generalized quantum dialogue protocol using these groups of unitary operators are also obtained. For example, it is shown that GHZ state, GHZ-like state, W state, 4 and 5 qubit Cluster states, Omega state, Brown state, $Q_{4}$ state and $Q_{5}$ state can be used for implementation of quantum dialogue protocol. The security and efficiency of the proposed protocol is appropriately analyzed. It is also shown that if a group of unitary operators and a set of mutually orthogonal states are found to be suitable for quantum dialogue then they can be used to provide solutions of socialist millionaire problem.Comment: 15 page

Polytype control of spin qubits in silicon carbide

Crystal defects can confine isolated electronic spins and are promising candidates for solid-state quantum information. Alongside research focusing on nitrogen vacancy centers in diamond, an alternative strategy seeks to identify new spin systems with an expanded set of technological capabilities, a materials driven approach that could ultimately lead to "designer" spins with tailored properties. Here, we show that the 4H, 6H and 3C polytypes of SiC all host coherent and optically addressable defect spin states, including spins in all three with room-temperature quantum coherence. The prevalence of this spin coherence shows that crystal polymorphism can be a degree of freedom for engineering spin qubits. Long spin coherence times allow us to use double electron-electron resonance to measure magnetic dipole interactions between spin ensembles in inequivalent lattice sites of the same crystal. Together with the distinct optical and spin transition energies of such inequivalent spins, these interactions provide a route to dipole-coupled networks of separately addressable spins.Comment: 28 pages, 5 figures, and supplementary information and figure

Identification and tunable optical coherent control of transition-metal spins in silicon carbide

Color centers in wide-bandgap semiconductors are attractive systems for quantum technologies since they can combine long-coherent electronic spin and bright optical properties. Several suitable centers have been identified, most famously the nitrogen-vacancy defect in diamond. However, integration in communication technology is hindered by the fact that their optical transitions lie outside telecom wavelength bands. Several transition-metal impurities in silicon carbide do emit at and near telecom wavelengths, but knowledge about their spin and optical properties is incomplete. We present all-optical identification and coherent control of molybdenum-impurity spins in silicon carbide with transitions at near-infrared wavelengths. Our results identify spin $S=1/2$ for both the electronic ground and excited state, with highly anisotropic spin properties that we apply for implementing optical control of ground-state spin coherence. Our results show optical lifetimes of $\sim$60 ns and inhomogeneous spin dephasing times of $\sim$0.3 $\mu$s, establishing relevance for quantum spin-photon interfacing.Comment: Updated version with minor correction, full Supplementary Information include

Designing defect-based qubit candidates in wide-gap binary semiconductors for solid-state quantum technologies

The development of novel quantum bits is key to extend the scope of solid-state quantum information science and technology. Using first-principles calculations, we propose that large metal ion - vacancy complexes are promising qubit candidates in two binary crystals: 4H-SiC and w-AlN. In particular, we found that the formation of neutral Hf- and Zr-vacancy complexes is energetically favorable in both solids; these defects have spin-triplet ground states, with electronic structures similar to those of the diamond NV center and the SiC di-vacancy. Interestingly, they exhibit different spin-strain coupling characteristics, and the nature of heavy metal ions may allow for easy defect implantation in desired lattice locations and ensure stability against defect diffusion. In order to support future experimental identification of the proposed defects, we report predictions of their optical zero-phonon line, zero-field splitting and hyperfine parameters. The defect design concept identified here may be generalized to other binary semiconductors to facilitate the exploration of new solid-state qubits.Comment: 23 pages, 5 figures, 6 tables, Supplementary Information is added at the en