Quantum control with spectral constraints

Various constraints concerning control fields can be imposed in the realistic implementations of quantum control systems. One of the most important is the restriction on the frequency spectrum of acceptable control parameters. It is important to consider the limitations of experimental equipment when trying to find appropriate control parameters. Therefore, in this paper we present a general method of obtaining a piecewise-constant controls, which are robust with respect to spectral constraints. We consider here a Heisenberg spin chain, however the method can be applied to a system with more general interactions. To model experimental restrictions we apply an ideal low-pass filter to numerically obtained control pulses. The usage of the proposed method has negligible impact on the control quality as opposed to the standard approach, which does not take into account spectral limitations.Comment: 6 pages, 4 figure

Monotonically convergent optimal control theory of quantum systems with spectral constraints on the control field

We propose a new monotonically convergent algorithm which can enforce spectral constraints on the control field (and extends to arbitrary filters). The procedure differs from standard algorithms in that at each iteration the control field is taken as a linear combination of the control field (computed by the standard algorithm) and the filtered field. The parameter of the linear combination is chosen to respect the monotonic behavior of the algorithm and to be as close to the filtered field as possible. We test the efficiency of this method on molecular alignment. Using band-pass filters, we show how to select particular rotational transitions to reach high alignment efficiency. We also consider spectral constraints corresponding to experimental conditions using pulse shaping techniques. We determine an optimal solution that could be implemented experimentally with this technique.Comment: 16 pages, 4 figures. To appear in Physical Review

Exploring constrained quantum control landscapes

The broad success of optimally controlling quantum systems with external fields has been attributed to the favorable topology of the underlying control landscape, where the landscape is the physical observable as a function of the controls. The control landscape can be shown to contain no suboptimal trapping extrema upon satisfaction of reasonable physical assumptions, but this topological analysis does not hold when significant constraints are placed on the control resources. This work employs simulations to explore the topology and features of the control landscape for pure-state population transfer with a constrained class of control fields. The fields are parameterized in terms of a set of uniformly spaced spectral frequencies, with the associated phases acting as the controls. Optimization results reveal that the minimum number of phase controls necessary to assure a high yield in the target state has a special dependence on the number of accessible energy levels in the quantum system, revealed from an analysis of the first- and second-order variation of the yield with respect to the controls. When an insufficient number of controls and/or a weak control fluence are employed, trapping extrema and saddle points are observed on the landscape. When the control resources are sufficiently flexible, solutions producing the globally maximal yield are found to form connected `level sets' of continuously variable control fields that preserve the yield. These optimal yield level sets are found to shrink to isolated points on the top of the landscape as the control field fluence is decreased, and further reduction of the fluence turns these points into suboptimal trapping extrema on the landscape. Although constrained control fields can come in many forms beyond the cases explored here, the behavior found in this paper is illustrative of the impacts that constraints can introduce.Comment: 10 figure

Generating Polarization-Entangled Photon Pairs with Arbitrary Joint Spectrum

We present a scheme for generating polarization-entangled photons pairs with arbitrary joint spectrum. Specifically, we describe a technique for spontaneous parametric down-conversion in which both the center frequencies and the bandwidths of the down-converted photons may be controlled by appropriate manipulation of the pump pulse. The spectral control offered by this technique permits one to choose the operating wavelengths for each photon of a pair based on optimizations of other system parameters (loss in optical fiber, photon counter performance, etc.). The combination of spectral control, polarization control, and lack of group-velocity matching conditions makes this technique particularly well-suited for a distributed quantum information processing architecture in which integrated optical circuits are connected by spans of optical fiber.Comment: 6 pages, 3 figure

Tailoring laser pulses with spectral and fluence constraints using optimal control theory

Within the framework of optimal control theory we develop a simple iterative scheme to determine optimal laser pulses with spectral and fluence constraints. The algorithm is applied to a one-dimensional asymmetric double well where the control target is to transfer a particle from the ground state, located in the left well, to the first excited state, located in the right well. Extremely high occupations of the first excited state are obtained for a variety of spectral and/or energetic constraints. Even for the extreme case where no resonance frequency is allowed in the pulse the algorithm achieves an occupation of almost 100%

Optimal Dynamical Decoherence Control of a Qubit

A theory of dynamical control by modulation for optimal decoherence reduction is developed. It is based on the non-Markovian Euler-Lagrange equation for the energy-constrained field that minimizes the average dephasing rate of a qubit for any given dephasing spectrum.Comment: 6 pages, including 2 figures and an appendi

Realistic and verifiable coherent control of excitonic states in a light harvesting complex

We explore the feasibility of coherent control of excitonic dynamics in light harvesting complexes, analyzing the limits imposed by the open nature of these quantum systems. We establish feasible targets for phase and phase/amplitude control of the electronically excited state populations in the Fenna-Mathews-Olson (FMO) complex and analyze the robustness of this control with respect to orientational and energetic disorder, as well as decoherence arising from coupling to the protein environment. We further present two possible routes to verification of the control target, with simulations for the FMO complex showing that steering of the excited state is experimentally verifiable either by extending excitonic coherence or by producing novel states in a pump-probe setup. Our results provide a first step toward coherent control of these complex biological quantum systems in an ultrafast spectroscopy setup.Comment: 12 pages, 8 figure