Métrologie en ligne de faisceaux et d'optiques X de synchrotrons

Cette thèse présente des travaux de recherche de métrologie en ligne de faisceaux de rayons X dans les installations synchrotrons. Deux approches principales ont été étudiées pour extraire la phase d'un front d'onde X : les méthodes utilisant des réseaux optiques et celles utilisant l'effet speckle dans le domaine X. L'interféromètre à réseaux X est l'outil le plus répandu résentatif de la première catégorie. Ses performances et son potentiel furent étudiés dans diverses situations de métrologie en ligne. Les méthodes utilisant le speckle X sont des techniques originales développées au cours de ce projet. Elles utilisent des membranes faites de petits grains diffusants, dont seule la distribution statistique est connue, pour permettre la modulation du front d'onde. Les différentes techniques furent déployées expérimentalement sur les lignes de lumière BM05 de l'ESRF et B16 de Diamond Light Source. Leurs implémentations servirent à la caractérisation de différents composants optiques utilisés pour manipuler les faisceaux synchrotron X et à l'étude de la faisabilité de micro imagerie par contraste de phase avec les sus citées techniques.This thesis presents research and development work on synchrotron X-ray at-wavelength metrology methods. Two approaches for measuring the phase of an X-ray wavefront were studied: the grating-based and the speckle-based methods. The X-ray grating interferometer is the most widespread technique representative of the first category. Its performance and potential in various situations encountered in at-wavelength metrology was investigated. Speckle methods are X-ray phase sensing techniques newly developed during this thesis project. They make use of membranes with small statistical features to modulate the beam wavefront. The different methods were deployed experimentally at the beamlines BM05 of the ESRF and B16 of the Diamond Light Source. Their implementation permitted the characterization of various kinds of optical elements used to manipulate synchrotron X-ray beamsas well as the feasibility study of micro phase contrast imaging using the two methods described above.SAVOIE-SCD - Bib.électronique (730659901) / SudocGRENOBLE1/INP-Bib.électronique (384210012) / SudocGRENOBLE2/3-Bib.électronique (384219901) / SudocSudocFranceF

The quantitative analysis of transonic flows by holographic interferometry

This thesis explores the feasibility of routine transonic flow analysis by holographic interferometry. Holography is potentially an important quantitative flow diagnostic, because whole-field data is acquired non-intrusively without the use of particle seeding. Holographic recording geometries are assessed and an image plane specular illumination configuration is shown to reduce speckle noise and maximise the depth-of-field of the reconstructed images. Initially, a NACA 0012 aerofoil is wind tunnel tested to investigate the analysis of two-dimensional flows. A method is developed for extracting whole-field density data from the reconstructed interferograms. Fringe analysis errors axe quantified using a combination of experimental and computer generated imagery. The results are compared quantitatively with a laminar boundary layer Navier-Stokes computational fluid dynamics (CFD) prediction. Agreement of the data is excellent, except in the separated wake where the experimental boundary layer has undergone turbulent transition. A second wind tunnel test, on a cone-cylinder model, demonstrates the feasibility of recording multi-directional interferometric projections using holographic optical elements (HOE’s). The prototype system is highly compact and combines the versatility of diffractive elements with the efficiency of refractive components. The processed interferograms are compared to an integrated Euler CFD prediction and it is shown that the experimental shock cone is elliptical due to flow confinement. Tomographic reconstruction algorithms are reviewed for analysing density projections of a three-dimensional flow. Algebraic reconstruction methods are studied in greater detail, because they produce accurate results when the data is ill-posed. The performance of these algorithms is assessed using CFD input data and it is shown that a reconstruction accuracy of approximately 1% may be obtained when sixteen projections are recorded over a viewing angle of ±58°. The effect of noise on the data is also quantified and methods are suggested for visualising and reconstructing obstructed flow regions

Wavefront and nanostructure characterisation with X-ray ptychography

X-ray ptychography is a scanning diffraction microscopy technique suited for the phase-sensitive investigation of wavefronts and specimens. It returns complex-valued wave functions and transmission functions producing high-resolution (nanoscale) phase- contrast images. This work focuses on the implementation and application of X-ray ptychography in the context of synchrotron radiation facilities. It presents an experimental protocol developed for multiscale X-ray imaging and tested at the I13-1 Coherence Branchline at Diamond Light Source. This protocol combines both near-field and far-field ptychography with other imaging methods, providing a flexible way of conducting experiments on hierarchical structures at any high-brilliance X-ray facility. This work also reports ptychography experiments performed at free-electron lasers, aimed at characterising their pulsed beam. Both the average and individual wavefronts are retrieved through a novel application of a reconstruction algorithm based on singular- value decomposition, giving direct insight on pulse-to-pulse fluctuations and confirming ptychography as a powerful beam diagnostics technique. Additional ptychography experiments are also discussed, which were carried out at storage rings on flat, weakly-scattering biogenic samples to characterise their 3D nanos- tructures. Their data analysis pipeline is presented in detail, from data acquisition to rendered volumes. Furthermore, one of these last experiments constitutes the first successful 3D ptychography experiment run on real-life samples at the I13-1 Coherence Branchline at Diamond Light Source

Tile-Based Two-Dimensional Phase Unwrapping for Digital Holography Using a Modular Framework

A variety of physical and biomedical imaging techniques, such as digital holography, interferometric synthetic aperture radar (InSAR), or magnetic resonance imaging (MRI) enable measurement of the phase of a physical quantity additionally to its amplitude. However, the phase can commonly only be measured modulo 2π, as a so called wrapped phase map. Phase unwrapping is the process of obtaining the underlying physical phase map from the wrapped phase. Tile-based phase unwrapping algorithms operate by first tessellating the phase map, then unwrapping individual tiles, and finally merging them to a continuous phase map. They can be implemented computationally efficiently and are robust to noise. However, they are prone to failure in the presence of phase residues or erroneous unwraps of single tiles. We tried to overcome these shortcomings by creating novel tile unwrapping and merging algorithms as well as creating a framework that allows to combine them in modular fashion. To increase the robustness of the tile unwrapping step, we implemented a model-based algorithm that makes efficient use of linear algebra to unwrap individual tiles. Furthermore, we adapted an established pixel-based unwrapping algorithm to create a quality guided tile merger. These original algorithms as well as previously existing ones were implemented in a modular phase unwrapping C++ framework. By examining different combinations of unwrapping and merging algorithms we compared our method to existing approaches. We could show that the appropriate choice of unwrapping and merging algorithms can significantly improve the unwrapped result in the presence of phase residues and noise. Beyond that, our modular framework allows for efficient design and test of new tile-based phase unwrapping algorithms. The software developed in this study is freely available

Terahertz for subsurface imaging and metrology applications

In the area of metrology and non-destructive testing, Terahertz wavelengths have been widely researched and used. However, the lack of 2D detectors working at room temperature and high power sources prevent the widespread application of Terahertz in industry. In that context, research on the development of new Terahertz equipment is moving at a fast pace. Within the scope of this thesis, applications of newly developed Terahertz technologies were explored using the scanning of single point detectors with the objective to establish the feasibility for their full-field applications in readiness for future 2D detectors. For the first time, a frequency tuneable, all-optical Terahertz source was implemented in multi-wavelength interferometry to overcome one wavelength ambiguity in precise thickness/distance measurements with sub-millimetre resolution. Phase-shifting digital holography is another interferometry technique which allows us to reconstruct not only the amplitude of one object, but also the phase and the depth of it, using existing mathematical algorithms. Digital holography was performed successfully at Terahertz wavelengths using a multiplier/mixer Terahertz source coupled with a single point pyroelectric detector for the applications of non-destructive testing and depth measurements. The novelty is that the phase-stepping technique for digital holography was implemented in THz frequencies for the first time to remove unwanted terms in the reconstructed image in order to improve image quality compare to conventional holography. In the current experiments, recording time for one set of phase-shifting holograms (4 holograms for 4 phase-steps algorithm) was 6 hours. When the technology is ready for 2D detectors, recording time of holograms could be reduced considerably, and the technique will play an important role in full-field applications in industry metrology and/or non-destructive testing and evaluation.EPSR

High-sensitivity interferometry

High-sensitivity interferometric techniques are considered for non-destructive testing applications. The methods enable quantitative measurement of optical path variations, resulting from dynamic changes within the test object. [Continues.

Near Field Electron Ptychography

Phase imaging in the Transmission Electron Microscope (TEM) has a long history, from the implementation of off-axis holography in TEM to Differential Phase Contrast (DPC) on the Scanning Transmission Electron Microscopy (STEM). The advent of modern computing has enabled the development of iterative algorithms which attempt to recover a phase image of a specimen from measurements of the way it diffracts an incident electron beam. One of the most successful of these iterative methods is focused probe ptychography, which relies on far field diffraction pattern measurements recorded as the incident beam is scanned through a grid of locations across the specimen. Focused probe ptychography implemented in the STEM has provided the highest resolution images available to date, allows for lens-less setups avoiding the aberrations typical in older STEMs and allows for simultaneous reconstruction of the illumination and specimen. Ptychography is computationally flexible (highly constrained), allowing for additional unknowns other than the phase of the specimen to be recovered, for example positions can be refined during reconstruction. Near field ptychography is a recent variation on ptychography that replaces the far-field diffraction data with diffraction patterns recorded in the near field, or Fresnel, region. It promises to obtain a much larger field of view with fewer diffraction patterns than focused probe ptychography. The main contribution of this thesis is the implementation of a new form of near field ptychography on the Transmission Electron Microscope (TEM), using an etched silicon nitride window to structure the electron beam. Proof-of-concept results show the method quantitatively recovers megapixel phase images from as few as 9 recorded diffraction patterns, compared to many hundreds of diffraction patterns required for focused probe ptychography. Additional sets of results show how near-field ptychography can recover extremely large fields of view, deal effectively with inelastic scattering, and accommodate several sources of uncertainty in the experimental process. Further contributions in the thesis include: experiments and results from visible-light versions of near field ptychography, which explain its limitations and practical application; a description and code for analysis tools that are used to assess phase imaging performance; DigitalMicrograph (DM) code and a data collection workflow to realise TEM-based near-field ptychography; details of the design, realisation and performance of the etched silicon nitride windows; and simulation studies aimed at furthering understanding of the frequency response of the technique. Future work is outlined, focusing on potential applications in a wide range of real-world specimens and improved TEM setups to implement near field ptychography

Use of prior information and probabilistic image reconstruction for optical tomographic imaging

Preclinical bioluminescence tomographic reconstruction is underdetermined. This work addresses the use of prior information in bioluminescence tomography to improve image acquisition, reconstruction, and analysis. A structured light surface metrology method was developed to measure surface geometry and enable robust and automatic integration of mirrors into the measurement process. A mouse phantom was imaged and accuracy was measured at 0.2mm with excellent surface coverage. A sparsity-regularised reconstruction algorithm was developed to use instrument noise statistics to automatically determine the stopping point of reconstruction. It was applied to in silico and in simulacra data and successfully reconstructed and resolved two separate luminescent sources within a plastic mouse phantom. A Bayesian framework was constructed that incorporated bioluminescence properties and instrument properties. Distribution expectations and standard deviations were estimated, providing reconstructions and measures of reconstruction uncertainty. The reconstructions showed superior performance when applied to in simulacra data compared to the sparsity-based algorithm. The information content of measurements using different sets of wavelengths was quantified using the Bayesian framework via mutual information and applied to an in silico problem. Significant differences in information content were observed and comparison against a condition number-based approach indicated subtly different results