Group Theory of Circular-Polarization Effects in Chiral Photonic Crystals with Four-Fold Rotation Axes, Applied to the Eight-Fold Intergrowth of Gyroid Nets

We use group or representation theory and scattering matrix calculations to derive analytical results for the band structure topology and the scattering parameters, applicable to any chiral photonic crystal with body-centered cubic symmetry I432 for circularly-polarised incident light. We demonstrate in particular that all bands along the cubic [100] direction can be identified with the irreducible representations E+/-,A and B of the C4 point group. E+ and E- modes represent the only transmission channels for plane waves with wave vector along the ? line, and can be identified as non-interacting transmission channels for right- (E-) and left-circularly polarised light (E+), respectively. Scattering matrix calculations provide explicit relationships for the transmission and reflectance amplitudes through a finite slab which guarantee equal transmission rates for both polarisations and vanishing ellipticity below a critical frequency, yet allowing for finite rotation of the polarisation plane. All results are verified numerically for the so-called 8-srs geometry, consisting of eight interwoven equal-handed dielectric Gyroid networks embedded in air. The combination of vanishing losses, vanishing ellipticity, near-perfect transmission and optical activity comparable to that of metallic meta-materials makes this geometry an attractive design for nanofabricated photonic materials

Non-collinear long-range magnetic ordering in HgCr2S4

The low-temperature magnetic structure of \HG has been studied by high-resolution powder neutron diffraction. Long-range incommensurate magnetic order sets in at T$_N\sim$22K with propagation vector \textbf{k}=(0,0,$\sim$0.18). On cooling below T$_N$, the propagation vector increases and saturates at the commensurate value \textbf{k}=(0,0,0.25). The magnetic structure below T$_N$ consists of ferromagnetic layers in the \textit{ab}-plane stacked in a spiral arrangement along the \textit{c}-axis. Symmetry analysis using corepresentations theory reveals a point group symmetry in the ordered magnetic phase of 422 (D$_4$), which is incompatible with macroscopic ferroelectricity. This finding indicates that the spontaneous electric polarization observed experimentally cannot be coupled to the magnetic order parameter

Magnetic structure of Ba(TiO)Cu4_4(PO4_4)4_4 probed using spherical neutron polarimetry

The antiferromagnetic compound Ba(TiO)Cu$_4$(PO$_4$)$_4$ contains square cupola of corner-sharing CuO$_4$ plaquettes, which were proposed to form effective quadrupolar order. To identify the magnetic structure, we have performed spherical neutron polarimetry measurements. Based on symmetry analysis and careful measurements we conclude that the orientation of the Cu$^{2+}$ spins form a non-collinear in-out structure with spins approximately perpendicular to the CuO$_4$ motif. Strong Dzyaloshinskii-Moriya interaction naturally lends itself to explain this phenomenon. The identification of the ground state magnetic structure should serve well for future theoretical and experimental studies into this and closely related compounds.Comment: 9 pages, 4 figure

Plasmon Modes of Axisymmetric Metallic Nanoparticles: A Group Theory Analysis

We report a thorough and rigorous analysis of the plasmon modes of axisymmetric metallic nanoparticles, based on group theory techniques and block diagonalization of the scattering T matrix. In particular, we discuss plasmonic excitations under plane-wave illumination of a silver nanorod and a nanodisk, and present a detailed comparative study of elongated silver nanoparticles of different shape, but with the same length and thickness. Our methodology allows for an unambiguous classification of the eigenmodes of nonspherical particles, according to the irreducible representations of the appropriate point symmetry group, and provides a consistent explanation of relevant extinction spectra elucidating aspects of the problem to a degree that goes beyond usual interpretation

Optical chirality from dark-field illumination of planar plasmonic nanostructures

Dark-field illumination is shown to make planar chiral nanoparticle arrangements exhibit circular dichroism in extinction analogous to true chiral scatterers. Circular dichrosim is experimentally observed at the maximum scattering of single oligomers consisting rotationally symmetric arrangements of gold nanorods, with strong agreement to numerical simulation. A dipole model is developed to show that this effect is caused by a difference in the geometric projection of a nanorod onto the handed orientation of electric fields created by a circularly polarized dark-field that is normally incident on a glass substrate. Owing to this geometric origin, the wavelength of the peak chiral response is also experimentally shown to shift depending on the separation between nanoparticles. All presented oligomers have physical dimensions less than the operating wavelength, and the applicable extension to closely packed planar arrays of oligomers is demonstrated to amplify the magnitude of circular dichroism. The realization of strong chirality in these oligomers demonstrates a new path to engineer optical chirality from planar devices using dark-field illumination

Generalized Debye Sources Based EFIE Solver on Subdivision Surfaces

The electric field integral equation is a well known workhorse for obtaining fields scattered by a perfect electric conducting (PEC) object. As a result, the nuances and challenges of solving this equation have been examined for a while. Two recent papers motivate the effort presented in this paper. Unlike traditional work that uses equivalent currents defined on surfaces, recent research proposes a technique that results in well conditioned systems by employing generalized Debye sources (GDS) as unknowns. In a complementary effort, some of us developed a method that exploits the same representation for both the geometry (subdivision surface representations) and functions defined on the geometry, also known as isogeometric analysis (IGA). The challenge in generalizing GDS method to a discretized geometry is the complexity of the intermediate operators. However, thanks to our earlier work on subdivision surfaces, the additional smoothness of geometric representation permits discretizing these intermediate operations. In this paper, we employ both ideas to present a well conditioned GDS-EFIE. Here, the intermediate surface Laplacian is well discretized by using subdivision basis. Likewise, using subdivision basis to represent the sources, results in an efficient and accurate IGA framework. Numerous results are presented to demonstrate the efficacy of the approach