Experimental study of nonlinear conductance in small metallic samples

We have directly observed current-dependent, nonlinear contributions to the conductance fluctuations of phase-coherent metallic wires and loops. The fluctuations in the current-voltage curves are reproducible, asymmetric about I=0, and in qualitative agreement with theoretical predictions. In ac measurements, the nonlinear terms also generate large harmonic signals of the conductance fluctuations whose dependence on the drive current can be understood qualitatively. The spectra of harmonics from loops and wires have different dependences on the voltage across the sample

Structural Examination of Au/Ge(001) by Surface X-Ray Diffraction and Scanning Tunneling Microscopy

The one-dimensional reconstruction of Au/Ge(001) was investigated by means of autocorrelation functions from surface x-ray diffraction (SXRD) and scanning tunneling microscopy (STM). Interatomic distances found in the SXRD-Patterson map are substantiated by results from STM. The Au coverage, recently determined to be 3/4 of a monolayer of gold, together with SXRD leads to three non-equivalent positions for Au within the c(8x2) unit cell. Combined with structural information from STM topography and line profiling, two building blocks are identified: Au-Ge hetero-dimers within the top wire architecture and Au homo-dimers within the trenches. The incorporation of both components is discussed using density functional theory and model based Patterson maps by substituting Germanium atoms of the reconstructed Ge(001) surface.Comment: 5 pages, 3 figure

Length-Independent Voltage Fluctuations in Small Devices

Conductance fluctuations in one-dimensional lines of length L shorter than the phase-coherence length Lφ are not universal but diverge as L-2. Using the Onsager relations and voltage additivity, we show that the voltage fluctuations are independent of the distance between voltage probes. The antisymmetric (Hall-type) contribution to the voltage fluctuations is constant for all values of L. Measurements of the voltage fluctuations and correlation function between different regions in Au and Sb lines confirm these results

Temperature Dependence of the Normal-Metal Aharonov-Bohm Effect

The amplitude of h/e periodic oscillations in the magnetoresistance of very small normal-metal (Au) rings, as well as the harmonic h/2e, have been studied as a function of temperature. The amplitudes depend on the temperature T roughly as T-1/2, as expected from the averaging of conduction channels in the absence of inelastic scattering, but may not be entirely consistent with this model. At the lowest T, the size of the fluctuations in the conductance is about ΔG∼e2/h, as predicted recently

Ferromagnetic coupling of mononuclear Fe centers in a self-assembled metal-organic network on Au(111)

The magnetic state and magnetic coupling of individual atoms in nanoscale structures relies on a delicate balance between different interactions with the atomic-scale surrounding. Using scanning tunneling microscopy, we resolve the self-assembled formation of highly ordered bilayer structures of Fe atoms and organic linker molecules (T4PT) when deposited on a Au(111) surface. The Fe atoms are encaged in a three-dimensional coordination motif by three T4PT molecules in the surface plane and an additional T4PT unit on top. Within this crystal field, the Fe atoms retain a magnetic ground state with easy-axis anisotropy, as evidenced by X-ray absorption spectroscopy and X-ray magnetic circular dichroism. The magnetization curves reveal the existence of ferromagnetic coupling between the Fe centers

Direct Observation of Ensemble Averaging of the Aharonov-Bohm Effect in Normal-Metal Loops

Aharonov-Bohm magnetoconductance oscillations have been measured in series arrays of 1, 3, 10, and 30 submicron-diameter Ag loops. At constant temperature, the amplitude of the h/e oscillations is observed to decrease as the square root of number of loops, while the amplitude of h/2e conductance oscillations, measured in the same samples, is independent of the number of series loops. This is direct confirmation of the ensemble averaging properties of h/e oscillations in multiloop systems. The amplitude of the h/e oscillations is in good agreement with recent calculations

Universal scaling of nonlocal and local resistance fluctuations in small wires

Resistance fluctuations in small metal samples result from coherent transport of the carriers. The wave functions of the carriers extend into regions which are not accessible classically. We have directly measured the length dependence of the nonlocal magnetoresistance fluctuations in Sb and Au wires by studying regions of our samples separated from the classical current path by a distance L which varied from 3Lcphi down to 0.2Lcphi (where Lcphi is the phase coherence length for the carriers in the metal). These fluctuations decay exponentially with L/Lcphi. Measurements along the classical current paths scale more slowly with L/Lcphi than predicted by the analytical theory but are in agreement with numerical simulations. We have also studied the length dependence of the magnetic field correlation scale BC, and we find that it is in qualitative agreement with a recent model calculation that accounts for the voltage probes

Asymmetry in the Magnetoconductance of Metal Wires and Loops

Universal conductance fluctuations in wires and Aharonov-Bohm oscillations in loops are not symmetric about H=0. The observation of asymmetry in the periodic oscillations is possible when the phase-coherence length of the wave function is comparable to the separation of the voltage probes. In both cases, four-probe measurements yield resistances which depend on lead configuration. The asymmetries appear like Hall voltages, and are consistent with Onsager\u27s relations