273 research outputs found
Stationary states and quantum quench dynamics of Bose-Einstein condensates in a double-well potential
We consider the properties of stationary states and the dynamics of
Bose-Einstein condensates (BECs) in a double-well (DW) potential with pair
tunneling by using a full quantum-mechanical treatment. Furthermore, we study
the quantum quench dynamics of the DW system subjected to a sudden change of
the Peierls phase. It is shown that strong pair tunneling evidently influences
the energy spectrum structure of the stationary states. For relatively weak
repulsive interatomic interactions, the dynamics of the DW system with a
maximal initial population difference evolves from Josephson oscillations to
quantum self-trapping as one increases the pair tunneling strength, while for
large repulsion the strong pair tunneling inhibits the quantum self-trapping.
In the case of attractive interatomic interactions, strong pair tunneling tends
to destroy the Josephson oscillations and quantum self-trapping, and the system
eventually enters a symmetric regime of zero population difference. Finally,
the effect of the Peierls phase on the quantum quench dynamics of the system is
analyzed and discussed. These new features are remarkably different from the
usual dynamical behaviors of a BEC in a DW potential.Comment: 9 pages,7 figures,accepted for publication in Journal of Physics
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Numerical modeling of self-limiting and self-enhancing caprock alteration induced by CO2 storage in a depleted gas reservoir
This paper presents numerical simulations of reactive transport which may be induced in the caprock of an on-shore depleted gas reservoir by the geological sequestration of carbon dioxide. The objective is to verify that CO{sub 2} geological disposal activities currently being planned for the study area are safe and do not induce any undesired environmental impact. In our model, fluid flow and mineral alteration are induced in the caprock by penetration of high CO{sub 2} concentrations from the underlying reservoir, where it was assumed that large amounts of CO{sub 2} have already been injected at depth. The main focus is on the potential effect of precipitation and dissolution processes on the sealing efficiency of caprock formations. Concerns that some leakage may occur in the investigated system arise because the seal is made up of potentially highly-reactive rocks, consisting of carbonate-rich shales (calcite+dolomite averaging up to more than 30% of solid volume fraction). Batch simulations and multi-dimensional 1D and 2D modeling have been used to investigate multicomponent geochemical processes. Numerical simulations account for fracture-matrix interactions, gas phase participation in multiphase fluid flow and geochemical reactions, and kinetics of fluid-rock interactions. The geochemical processes and parameters to which the occurrence of high CO{sub 2} concentrations are most sensitive are investigated by conceptualizing different mass transport mechanisms (i.e. diffusion and mixed advection+diffusion). The most relevant mineralogical transformations occurring in the caprock are described, and the feedback of these geochemical processes on physical properties such as porosity is examined to evaluate how the sealing capacity of the caprock could evolve in time. The simulations demonstrate that the occurrence of some gas leakage from the reservoir may have a strong influence on the geochemical evolution of the caprock. In fact, when a free CO{sub 2}-dominated phase migrates into the caprock through fractures, or through zones with high initial porosity possibly acting as preferential flow paths for reservoir fluids, low pH values are predicted, accompanied by significant calcite dissolution and porosity enhancement. In contrast, when fluid-rock interactions occur under fully liquid-saturated conditions and a diffusion-controlled regime, pH will be buffered at higher values, and some calcite precipitation is predicted which leads to further sealing of the storage reservoir
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Incorporation of aqueous reaction kinetics and biodegradation intoTOUGHREACT: Application of a multi-region model to hydrobiogeoChemicaltransport of denitrification and sulfate reduction
The need to consider aqueous and sorption kinetics andmicrobiological processes arises in many subsurface problems. Ageneral-rate expression has been implemented into the TOUGHREACTsimulator, which considers multiple mechanisms (pathways) and includesmultiple product, Monod, and inhibition terms. This paper presents aformulation for incorporating kinetic rates among primary species intomass-balance equations. The space discretization used is based on aflexible integral finite difference approach that uses irregular griddingto model bio-geologic structures. A general multi-region model forhydrological transport interacted with microbiological and geochemicalprocesses is proposed. A 1-D reactive transport problem with kineticbiodegradation and sorption was used to test the enhanced simulator,which involves the processes that occur when a pulse of water containingNTA (nitrylotriacetate) and cobalt is injected into a column. The currentsimulation results agree very well with those obtained with othersimulators. The applicability of this general multi-region model wasvalidated by results from a published column experiment ofdenitrification and sulfate reduction. The matches with measured nitrateand sulfate concentrations were adjusted with the interficial areabetween mobile hydrological and immobile biological regions. Resultssuggest that TOUGHREACT can not only be a useful interpretative tool forbiogeochemical experiments, but also can produce insight into processesand parameters of microscopic diffusion and their interplay withbiogeochemical reactions. The geometric- and process-based multi-regionmodel may provide a framework for understanding field-scalehydrobiogeochemical heterogeneities and upscaling parameters
China actively promotes CO2 capture, utilization and storage research to achieve carbon peak and carbon neutrality
Global climate change is a common challenge facing mankind, which has evolved from a scientifific issue into a global economic and political issue of universal concern to the international community. Temperature increase, sea level rise, extreme weather and climate events caused by the climate change are becoming more and more prominent. The scientifific understanding of climate change in the international community has been deepening. The Intergovernmental Panel on Climate Change (IPCC, 2014) further strengthened the scientific conclusion that human-induced climate change is more than 95% likely to be attributed to emissions of greenhouse gases from human activities.The United Nations Climate Change Summit (held in September 2014) pointed out that climate change threatens the hard-won peace, prosperity and opportunities of all mankind, and that no one and no country is immune to its impact. Controlling global warming within 2℃ is an urgent and severe challenge faced by mankind in dealing with climate change. The awareness of all countries on the issue of climate change is gradually increasing. The 26th Conference of the Parties (held in November 2021 in Glasgow, UK) urged all countries to achieve the net zero carbon emissions by around 2050, and step up efforts to reduce carbon emission before 2030. Therefore, taking active measures to cope with climate change becomes the common aspiration and urgent need of all countries.Mitigating greenhouse gas emissions (represented by CO2) has become the consensus of the world. In September 2020, Chinese President Xi Jinping pledged at the General Debate of the 75th Session of The United Nations General Assembly that China aims to peak its CO2 emissions before 2030 and achieve carbon neutrality before 2060 (i.e., dual carbon goals), which demonstrates the responsibility of a major country.CO2 Capture, Utilization, and Storage (CCUS) is considered as an effective technology directly achieving carbon emissions mitigation, and has attracted widespread attention of the international community (Metz et al., 2005). The implementation of CCUS projects began in the 1970s, and was mainly carried out in the United States, Canada and some European countries. Those projects mainly focused on CO2 enhanced oil recovery, whereas projects with the pure purpose of CO2 sequestration are relatively rare due to their poor economy.CCUS projects in China started relatively late, and most of them were gradually implemented after 2000 (Guo et al., 2014). The initial technical routes of these projects were similar to those of projects carried out in European and American countries, which began with the geological sequestration of CO2 and enhanced oil recovery. In the past decade, CCUS projects in China began to develop in a diversified way, and there emerged a variety of carbon dioxide capture, storage and utilization technologies, including pre-combustion capture of power plants, CO2 chemical and biological utilization, etc.The realization of the dual carbon goals not only requires revolutionary changes in industrial technology, but also largely depends on the formulation of relevant policies and capital investment. The National Natural Science Foundation of China launched a special research program “Major Basic Science Issues and Countermeasures for National Carbon neutrality” in 2021 to meet the needs of basic science research for the national carbon neutrality strategy. Focusing on the two core issues of “carbon emission mitigation” and “carbon sink increase”, the special program includes a total of 28 research projects, with an average funding of about 3 million RMB per project.This special research program aims to reveal the oceans and terrestrial carbon sinks, the process mechanism, evolution trend and its mutual feedback mechanism with the climate system, delineate the geological process of carbon sequestration and the effectivity of fixing carbon. The program also has goals to increase the potential of CO2 storage, to assess the technology risk and management mode, to analyze the economic transformation, the optimal pathway, climate control, international cooperation management and policy issues. Interdisciplinary integration research is needed to condense key basic science issues and solutions for serving the national carbon-neutral strategy.It is foreseeable that China will further increase investment in realizing a carbon emission peak and its carbon-neutral strategy in the future. This is also a great opportunity for the development of CCUS-related technologies. The contribution of CCUS technology in carbon emission mitigation is generally low today. For instance, even in Norway, which has the highest proportion of carbon emissions treated by CCUS, the value is less than 5% (Cai et al., 2020). However, as the guaranteed technology of carbon peak strategy, the contribution ratio of CCUS in carbon emission mitigation is expected to significantly increase in the future.Although the CCUS technology has been implemented for many years and many projects have been carried out, there are still many challenges to be solved, such as:(i) CCUS related technology development and cost control The CCUS technology includes capture, transportation, utilization and storage, all of which need to consume a lot of energy. At present, the cost of the CCUS projects is still high. It is estimated that the cost of the whole CCUS process will be 150-540 RMB per ton of CO2 by 2025, of which CO2 capture cost accounts for more than two thirds of the total cost, about 100-480 RMB/ton. In comparison, the cost of CO2 sequestration is 50-60 RMB/ton, while the cost of CO2 transportation is very low, less than 1 RMB/ton (Cai et al., 2021). Obviously, the wider promotion of CCUS projects in the future largely depends on the further development of CO2 capture technology and the rapid reduction of cost.(ii) Effect of long-term CO2-water-rock interaction on rock structure and mechanical properties In the process of CO2 geological storage and utilization, the injected CO2 will inevitably change the pH of formation water, breaking the original water-rock balance and inducing a new water-rock reaction. Thus, the rock structure and mechanical properties of the caprock are likely to be changed over time, which affects the safety of the storage reservoirs. The current studies mostly focus on the effect of CO2-water-rock interaction on the leakage channels (porosity and permeability) of the caprock (Credoz et al., 2009; Liu et al., 2020). However, the study on the change of rock mechanical properties caused by chemical reactions requires further research attention. A few previous studies only simply correlated the evolution of rock mechanical properties with porosity, but without considering the influence of changes in mineral composition induced by CO2-water-rock interaction on the rock mechanical properties (Agarwal, 2019). Therefore, it is necessary to further deepen the relevant investigation and build a comprehensive rock mechanical parameter evolution model considering the changes of porosity, mineral composition and content, and other factors (Tian et al., 2019).(iii) CO2 leakage monitoring and risk assessment methods The leakage risk of CO2 after injection has been one of the main concerns, which directly affects the safety and feasibility of CCUS technology (Bachu, 2008). At this point, the construction of a CO2 leakage monitoring system is particularly important. However, the CO2 leakage process is usually characterized by sudden occurrence and weak surface response. Therefore, a single monitoring method is difficult to ensure the reliability of monitoring. In the future, it is necessary to combine various monitoring methods with their respective advantages.For a long-term (more than 100 years) CO2 leakage risk assessment, the most commonly used method at present is to employ the reactive transport modelling. However, due to the large time scale, parameter uncertainty and the difficulty of validation, the predicted results have high uncertainty. Some natural CO2 gas reservoirs have existed for more than thousands of years (Jonathan et al., 2018). Taking natural CO2 gas reservoirs as a natural analogue of CO2 geological sequestration can solve the problem that long-term simulated results are difficult to verify, thereby improving the reliability of long-term risk assessment (Xu et al., 2019). AcknowledgementThis work was performed in support of the National Natural Science Foundation of China (Grant Nos. 42141013 and 41772247). Conflict of interest The authors declare no competing interest.Open Access This article is distributed under the terms and conditions of the Creative Commons Attribution (CC BY-NC-ND) license, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.Cited as: Xu, T., Tian, H., Zhu, H., Cai, J. China actively promotes CO2 capture, utilization and storage research to achieve carbon peak and carbon neutrality. Advances in Geo-Energy Research, 2022, 6(1): 1-3. https://doi.org/10.46690/ager.2022.01.0
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Multiphase fluid flow and subsequent geochemical transport invariably saturated fractured rocks: 1. Approaches
Reactive fluid flow and geochemical transport in unsaturated fractured rocks has received increasing attention for studies of contaminant transport, groundwater quality, waste disposal, acid mine drainage remediation, mineral deposits, sedimentary diagenesis, and fluid-rock interactions in hydrothermal systems. This paper presents methods for modeling geochemical systems that emphasize: (1) involvement of the gas phase in addition to liquid and solid phases in fluid flow, mass transport and chemical reactions, (2) treatment of physically and chemically heterogeneous and fractured rocks, (3) the effect of heat on fluid flow and reaction properties and processes, and (4) the kinetics of fluid-rock interaction. The physical and chemical process model is embodied in a system of partial differential equations for flow and transport, coupled to algebraic equations and ordinary differential equations for chemical interactions. For numerical solution, the continuum equations are discretized in space and time. Space discretization is based on a flexible integral finite difference approach that can use irregular gridding to model geologic structure; time is discretized fully implicitly as a first-order finite difference. Heterogeneous and fractured media are treated with a general multiple interacting continua method that includes double-porosity, dual-permeability, and multi-region models as special cases. A sequential iteration approach is used to treat the coupling between fluid flow and mass transport on the one hand, chemical reactions on the other. Applications of the methods developed here to variably saturated geochemical systems are presented in a companion paper (part 2, this issue)
Accurate Eye Tracking from Dense 3D Surface Reconstructions using Single-Shot Deflectometry
Eye-tracking plays a crucial role in the development of virtual reality
devices, neuroscience research, and psychology. Despite its significance in
numerous applications, achieving an accurate, robust, and fast eye-tracking
solution remains a considerable challenge for current state-of-the-art methods.
While existing reflection-based techniques (e.g., "glint tracking") are
considered the most accurate, their performance is limited by their reliance on
sparse 3D surface data acquired solely from the cornea surface. In this paper,
we rethink the way how specular reflections can be used for eye tracking: We
propose a novel method for accurate and fast evaluation of the gaze direction
that exploits teachings from single-shot phase-measuring-deflectometry (PMD).
In contrast to state-of-the-art reflection-based methods, our method acquires
dense 3D surface information of both cornea and sclera within only one single
camera frame (single-shot). Improvements in acquired reflection surface
points("glints") of factors are easily achievable. We show the
feasibility of our approach with experimentally evaluated gaze errors of only
demonstrating a significant improvement over the current
state-of-the-art
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