63 research outputs found

    Evolution of superconductivity by oxygen annealing in FeTe0.8S0.2

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    Oxygen annealing dramatically improved the superconducting properties of solid-state-reacted FeTe0.8S0.2, which showed only a broad onset of superconducting transition just after the synthesis. The zero resistivity appeared and reached 8.5 K by the oxygen annealing at 200\degree C. The superconducting volume fraction was also enhanced from 0 to almost 100%. The lattice constants were compressed by the oxygen annealing, indicating that the evolution of bulk superconductivity in FeTe0.8S0.2 was correlated to the shrinkage of lattice.Comment: 13 pages, 6 figure

    Spin Configuration and Scattering Rates on the Heavily Electron-doped Surface of Topological Insulator Bi2_2Se3_3

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    Heavily electron-doped surfaces of Bi2_2Se3_3 have been studied by spin and angle resolved photoemission spectroscopy. Upon doping, electrons occupy a series of {\bf k}-split pairs of states above the topological surface state. The {\bf k}-splitting originates from the large spin-orbit coupling and results in a Rashba-type behavior, unequivocally demonstrated here via the spin analysis. The spin helicities of the lowest laying Rashba doublet and the adjacent topological surface state alternate in a left-right-left sequence. This spin configuration sets constraints to inter-band scattering channels opened by electron doping. A detailed analysis of the scattering rates suggests that intra-band scattering dominates with the largest effect coming from warping of the Fermi surface

    Spin-Resolved Photoemission on Anti-Ferromagnets: Direct Observation of Zhang-Rice Singlets in CuO

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    We demonstrate that it is possible to obtain spin-resolved valence band spectra with a very high degree of spin polarization from antiferromagnetic transition metal materials if the excitation light is circularly polarized and has an energy close to the cation 2p3/2 (L3) white line. We are able to unravel the different spin states in the single-particle excitation spectrum of CuO and show that the top of the valence band is of pure singlet character, which provides strong support for the existence and stability of Zhang-Rice singlets in high-Tc superconductors

    Local Electronic and Magnetic Structure of Ni below and above TC: A Spin-Resolved Circularly Polarized Resonant Photoemission Study

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    We report the measurement of the local Ni 3d spin polarization, not only below but also above the Curie temperature (TC), using the newly developed spin-resolved circularly polarized 2p (L3) resonant photoemission technique. The experiment identifies the presence of 3d8 singlets at high energies and 3d8 triplets at low energies extending all the way to the Fermi energy, both below and above TC, showing that it is the orbital degeneracy of the 3d band and the Hund's rule splitting which is of utmost importance to understand Ni and other 3d ferromagnets

    A Spin-Resolved Photoemission Study of Photohole Lifetimes in Ferromagnetic Gadolinium

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    High resolution spin-resolved photoemission is used to probe the properties of a Gd(0001) surface state. The state shows both a spin-mixing behavior reflecting the exchange of magnons with the local moments and a reduction of the exchange splitting with increasing temperature. The surface state polarization at low T suggests that the surface layer has an enhanced Tc of 365K or greater. Measurements of the photoemission linewidths show that at low temperatures, the lifetime of a majority spin photohole is predominantly limited by electron-phonon scattering and that of a minority spin photohole by electron-magnon scattering. Since similar behavior may be expected for bulk states close to the Fermi level, the transport properties of this material will also be determined by different decay mechanisms in the two channels

    Combined cytogenetic and molecular methods for taxonomic verification and description of Brassica populations deriving from different origins

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    Agriculture faces great challenges to overcome global warming and improve system sustainability, requiring access to novel genetic diversity. So far, wild populations and local landraces remain poorly explored. This is notably the case for the two diploid species, Brassica oleracea L. (CC, 2n=2x=18) and B. rapa L. (AA, 2n=2x=20). In order to explore the genetic diversity in both species, we have collected populations in their centre of origin, the Mediterranean basin, on a large contrasting climatic and soil gradient from northern Europe to southern sub-Saharan regions. In these areas, we also collected 14 populations belonging to five B. oleracea closely related species. Our objective was to ensure the absence of species misidentification at the seedling stage among the populations collected and to describe thereafter their origins. We combined flow cytometry, sequencing of a species-specific chloroplast genomic region, as well as cytogenetic analyses in case of unexpected results for taxonomic verification. Out of the 112 B. oleracea and 154 B. rapa populations collected, 103 and 146, respectively, presented a good germination rate and eighteen populations were misidentified. The most frequent mistake was the confusion of these diploid species with B. napus. Additionally for B. rapa, two autotetraploid populations were observed. Habitats of the collected and confirmed wild populations and landraces are described in this study. The unique plant material described here will serve to investigate the genomic regions involved in adaptation to climate and microbiota within the framework of the H2020 Prima project ‘BrasExplor’

    Extrinsic Magnetotransport Phenomena in Ferromagnetic Oxides

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    This review is focused on extrinsic magnetotransport effects in ferromagnetic oxides. It consists of two parts; the second part is devoted to an overview of experimental data and theoretical models for extrinsic magnetotransport phenomena. Here a critical discussion of domain-wall scattering is given. Results on surfacial and interfacial magnetism in oxides are presented. Spin-polarized tunnelling in ferromagnetic junctions is reviewed and grain-boundary magnetoresistance is interpreted within a model of spin-polarized tunnelling through natural oxide barriers. The situation in ferromagnetic oxides is compared with data and models for conventional ferromagnets. The first part of the review summarizes basic material properties, especially data on the spin-polarization and evidence for half-metallicity. Furthermore, intrinsic conduction mechanisms are discussed. An outlook on the further development of oxide spin-electronics concludes this review.Comment: 133 pages, 47 figures, submitted to Rep. Prog. Phy
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