Dielectric confinement of excitons in type-I and type-II semiconductor nanorods

We theoretically study the effect of the dielectric environment on the exciton ground state of CdSe and CdTe/CdSe/CdTe nanorods. We show that insulating environments enhance the exciton recombination rate and blueshift the emission peak by tens of meV. These effects are particularly pronounced for type-II nanorods. In these structures, the dielectric confinement may even modify the spatial distribution of electron and hole charges. A critical electric field is required to separate electrons from holes, whose value increases with the insulating strength of the surroundings.Comment: Journal of Physics: Condensed Matter (in press

Study of moments of event shapes in e+e- annihilation using JADE data

Data from e+e- annihilation into hadrons collected by the JADE experiment at centre-of-mass energies between 14 GeV and 44 GeV were used to study moments of event shape distributions. The data were compared with Monte Carlo models and with predictions from QCD NLO order calculations. The strong coupling constant measured from the moments is alpha_S(M_Z) = 0.1286 +/- 0.0007 (stat) +/- 0.0011 (expt) +/- 0.0022 (had) +/- 0.0068 (theo), alpha_S(M_Z) = 0.1286 +/- 0.0072 (total error), consistent with the world average. However, systematic deficiencies in the QCD NLO order predictions are visible for some of the higher moments.Comment: JADE note 147 submitted as contributed paper to ICHEP 2004, corrected statistical error of 6 observable average and several typo

Measurement of the Strong Coupling Constant alpha_S from the Four-Jet Rate in e+e- Annihilation using JADE data

Data from e+e- annihilation into hadrons collected by the JADE experiment at centre-of-mass energies between 14 GeV and 44 GeV were used to study the four-jet rate as a function of the Durham algorithm's resolution parameter y_cut. The four-jet rate was compared to a QCD NLO order calculations including NLLA resummation of large logarithms. The strong coupling constant measured from the four-jet rate is alpha_S(M_Z) = 0.1169 +/- 0.0004 (stat) +/- 0.0012 (expt) +/- 0.0021 (had) +/- 0.0007 (theo), alpha_S(M_Z) = 0.1169 +/- 0.0026 (total error) in agreement with the world average.Comment: JADE note 146 submitted as contributed paper to ICHEP 200

Generalized method of image dyons for quasi-two dimensional slabs with ordinary-topological insulator interfaces

Electrostatic charges near the interface bewteen topological (TI) and ordinary (OI) insulators induce magnetic fields in the medium that can be described through the so-called method of image dyons (electric charge - magnetic monopole pairs), the magnetoelectric extension of the method of image charges in classical electrostatics. Here, we provide the expressions for the image dyons and ensuing magnetoelectric potentials in a system comprised by two planar-parallel OI-TI interfaces conforming a finite-width slab. The obtained formulae extend earlier work in that they account for all different combinations of materials forming the slab and its surroundings, including asymmetric systems, as well as all possible combinations of external magnetization orientations on the interfaces. The equations are susceptible of implementation in simple computational codes, to be solved recurrently, in order to model magnetoelectric fields in topological quantum wells, thin films, or layers of two-dimensional materials. We exemplify this by calculating the magnetic fields induced by a point charge in nanometer-thick quantum wells, by means of a Mathematica code made available in repositories.Comment: 9 pages, 7 figure

Configuration interaction approach to Fermi liquid-Wigner crystal mixed phases in semiconductor nanodumbbells

Full configuration interaction calculations demonstrate the existence of mixed correlation phases in truly three-dimensional elongated nanocrystals subject to inhomogeneous spatial confining potentials. In such phases, the electron density behaves like a Fermi liquid in some regions, while, simultaneously, other more dilute regions display the typical quasi-classical Wigner distribution. The present results confirm and strengthen previous local spin-density functional theory predictions [Ballester et al., Phys. Rev. B 82, 115405 (2010)]. Additionally, simulation of the in-plane and z-polarized modes of the absorption spectra reveals the different correlation regimes occurring in these system

Mixed correlation phases in elongated quantum dots

It is theoretically shown, within the local spin-density-functional theory framework, that inhomogeneous confining potentials in elongated, diluted N-electron quantum dots may lead to the formation of mixed phases in which some regions of the N-electron system behave like a Fermi liquid while, simultaneously, other, more dilute regions display quasiclassical Wigner crystallization. The characterization of the mixed phases in the addition energy spectrum and the infrared response is reported. An infrared sensor of electron filling is suggested

An intramolecular oxa-Michael reaction on α,β-unsaturated α-amino-δ-hydroxycarboxylic acid esters. Synthesis of functionalized 1,3-dioxanes

A highly diastereoselective intramolecular oxa-Michael reaction on α,β-unsaturated α-amino-δ-hydroxycarboxylic acid esters is presented; 1,3-dioxanes functionalized in positions 2,4 and 6 were obtained in good yields and with excellent selectivities; an experimental and computational study was carried out to understand the reaction course in terms of yields and selectivities. This reaction proceeds under mild reaction conditions using highly electrophilic aldehydes and ketones