245 research outputs found
Attosecond control of electrons emitted from a nanoscale metal tip
Attosecond science is based on steering of electrons with the electric field
of well-controlled femtosecond laser pulses. It has led to, for example, the
generation of XUV light pulses with a duration in the sub-100-attosecond
regime, to the measurement of intra-molecular dynamics by diffraction of an
electron taken from the molecule under scrutiny, and to novel ultrafast
electron holography. All these effects have been observed with atoms or
molecules in the gas phase. Although predicted to occur, a strong light-phase
sensitivity of electrons liberated by few-cycle laser pulses from solids has
hitherto been elusive. Here we show a carrier-envelope (C-E) phase-dependent
current modulation of up to 100% recorded in spectra of electrons laser-emitted
from a nanometric tungsten tip. Controlled by the C-E phase, electrons
originate from either one or two sub-500as long instances within the 6-fs laser
pulse, leading to the presence or absence of spectral interference. We also
show that coherent elastic re-scattering of liberated electrons takes place at
the metal surface. Due to field enhancement at the tip, a simple laser
oscillator suffices to reach the required peak electric field strengths,
allowing attosecond science experiments to be performed at the 100-Megahertz
repetition rate level and rendering complex amplified laser systems
dispensable. Practically, this work represents a simple, exquisitely sensitive
C-E phase sensor device, which can be shrunk in volume down to ~ 1cm3. The
results indicate that the above-mentioned novel attosecond science techniques
developed with and for atoms and molecules can also be employed with solids. In
particular, we foresee sub-femtosecond (sub-) nanometre probing of (collective)
electron dynamics, such as plasmon polaritons, in solid-state systems ranging
in size from mesoscopic solids via clusters to single protruding atoms.Comment: Final manuscript version submitted to Natur
Semimetallization of dielectrics in strong optical fields
At the heart of ever growing demands for faster signal processing is ultrafast charge transport and control by electromagnetic fields in semiconductors. Intense optical fields have opened fascinating avenues for new phenomena and applications in solids. Because the period of optical fields is on the order of a femtosecond, the current switching and its control by an optical field may pave a way to petahertz optoelectronic devices. Lately, a reversible semimetallization in fused silica on a femtosecond time scale by using a few-cycle strong field (similar to 1 V/angstrom) is manifested. The strong Wannier-Stark localization and Zener-type tunneling were expected to drive this ultrafast semimetallization. Wider spread of this technology demands better understanding of whether the strong field behavior is universally similar for different dielectrics. Here we employ a carrier-envelope-phase stabilized, few-cycle strong optical field to drive the semimetallization in sapphire, calcium fluoride and quartz and to compare this phenomenon and show its remarkable similarity between them. The similarity in response of these materials, despite the distinguishable differences in their physical properties, suggests the universality of the physical picture explained by the localization of Wannier-Stark states. Our results may blaze a trail to PHz-rate optoelectronics.open11178sciescopu
Carrier-envelope phase effects on the strong-field photoemission of electrons from metallic nanostructures
Sharp metallic nanotapers irradiated with few-cycle laser pulses are emerging
as a source of highly confined coherent electron wavepackets with attosecond
duration and strong directivity. The possibility to steer, control or switch
such electron wavepackets by light is expected to pave the way towards direct
visualization of nanoplasmonic field dynamics and real-time probing of electron
motion in solid state nanostructures. Such pulses can be generated by
strong-field induced tunneling and acceleration of electrons in the near-field
of sharp gold tapers within one half-cycle of the driving laser field. Here, we
show the effect of the carrier-envelope phase of the laser field on the
generation and motion of strong-field emitted electrons from such tips. This is
a step forward towards controlling the coherent electron motion in and around
metallic nanostructures on ultrashort length and time scales
Exploiting disorder for perfect focusing
We demonstrate experimentally that disordered scattering can be used to
improve, rather than deteriorate, the focusing resolution of a lens. By using
wavefront shaping to compensate for scattering, light was focused to a spot as
small as one tenth of the diffraction limit of the lens. We show both
experimentally and theoretically that it is the scattering medium, rather than
the lens, that determines the width of the focus. Despite the disordered
propagation of the light, the profile of the focus was always exactly equal to
the theoretical best focus that we derived.Comment: 4 pages, 4 figure
Focusing and Compression of Ultrashort Pulses through Scattering Media
Light scattering in inhomogeneous media induces wavefront distortions which
pose an inherent limitation in many optical applications. Examples range from
microscopy and nanosurgery to astronomy. In recent years, ongoing efforts have
made the correction of spatial distortions possible by wavefront shaping
techniques. However, when ultrashort pulses are employed scattering induces
temporal distortions which hinder their use in nonlinear processes such as in
multiphoton microscopy and quantum control experiments. Here we show that
correction of both spatial and temporal distortions can be attained by
manipulating only the spatial degrees of freedom of the incident wavefront.
Moreover, by optimizing a nonlinear signal the refocused pulse can be shorter
than the input pulse. We demonstrate focusing of 100fs pulses through a 1mm
thick brain tissue, and 1000-fold enhancement of a localized two-photon
fluorescence signal. Our results open up new possibilities for optical
manipulation and nonlinear imaging in scattering media
Attosecond nanoscale near-field sampling
The promise of ultrafast light-field-driven electronic nanocircuits has stimulated the development of the new research field of attosecond nanophysics. An essential prerequisite for advancing this new area is the ability to characterize optical near fields from light interaction with nanostructures, with sub-cycle resolution. Here we experimentally demonstrate attosecond near-field retrieval for a tapered gold nanowire. By comparison of the results to those obtained from noble gas experiments and trajectory simulations, the spectral response of the nanotaper near field arising from laser excitation can be extracted.113023Ysciescopu
Past Achievements and Future Challenges in 3D Photonic Metamaterials
Photonic metamaterials are man-made structures composed of tailored micro- or
nanostructured metallo-dielectric sub-wavelength building blocks that are
densely packed into an effective material. This deceptively simple, yet
powerful, truly revolutionary concept allows for achieving novel, unusual, and
sometimes even unheard-of optical properties, such as magnetism at optical
frequencies, negative refractive indices, large positive refractive indices,
zero reflection via impedance matching, perfect absorption, giant circular
dichroism, or enhanced nonlinear optical properties. Possible applications of
metamaterials comprise ultrahigh-resolution imaging systems, compact
polarization optics, and cloaking devices. This review describes the
experimental progress recently made fabricating three-dimensional metamaterial
structures and discusses some remaining future challenges
Plasmonic Luneburg and Eaton Lenses
Plasmonics is an interdisciplinary field focusing on the unique properties of
both localized and propagating surface plasmon polaritons (SPPs) -
quasiparticles in which photons are coupled to the quasi-free electrons of
metals. In particular, it allows for confining light in dimensions smaller than
the wavelength of photons in free space, and makes it possible to match the
different length scales associated with photonics and electronics in a single
nanoscale device. Broad applications of plasmonics have been realized including
biological sensing, sub-diffraction-limit imaging, focusing and lithography,
and nano optical circuitry. Plasmonics-based optical elements such as
waveguides, lenses, beam splitters and reflectors have been implemented by
structuring metal surfaces or placing dielectric structures on metals, aiming
to manipulate the two-dimensional surface plasmon waves. However, the abrupt
discontinuities in the material properties or geometries of these elements lead
to increased scattering of SPPs, which significantly reduces the efficiency of
these components. Transformation optics provides an unprecedented approach to
route light at will by spatially varying the optical properties of a material.
Here, motivated by this approach, we use grey-scale lithography to
adiabatically tailor the topology of a dielectric layer adjacent to a metal
surface to demonstrate a plasmonic Luneburg lens that can focus SPPs. We also
realize a plasmonic Eaton lens that can bend SPPs. Since the optical properties
are changed gradually rather than abruptly in these lenses, losses due to
scattering can be significantly reduced in comparison with previously reported
plasmonic elements.Comment: Accepted for publication in Nature Nanotechnolog
Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates
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Scalable, ultra-resistant structural colors based on network metamaterials
Structural colors have drawn wide attention for their potential as a future printing technology for various applications, ranging from biomimetic tissues to adaptive camouflage materials. However, an efficient approach to realize robust colors with a scalable fabrication technique is still lacking, hampering the realization of practical applications with this platform. Here, we develop a new approach based on large-scale network metamaterials that combine dealloyed subwavelength structures at the nanoscale with lossless, ultra-thin dielectric coatings. By using theory and experiments, we show how subwavelength dielectric coatings control a mechanism of resonant light coupling with epsilon-near-zero regions generated in the metallic network, generating the formation of saturated structural colors that cover a wide portion of the spectrum. Ellipsometry measurements support the efficient observation of these colors, even at angles of 70°. The network-like architecture of these nanomaterials allows for high mechanical resistance, which is quantified in a series of nano-scratch tests. With such remarkable properties, these metastructures represent a robust design technology for real-world, large-scale commercial applications
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