Radiation transport in cloudy and aerosol loaded atmospheres

Thesis (Ph.D.) University of Alaska Fairbanks, 1992The equation for radiation transport in vertical inhomogeneous absorbing, scattering, and emitting atmospheres is derived from first principles. It is cast in a form amenable to solution, and solved using the discrete ordinate method. Based on the discrete ordinate solution a new computationally efficient and stable two-stream algorithm which accounts for spherical geometry is developed. The absorption and scattering properties of atmospheric molecules and particulate matter is discussed. The absorption cross sections of the principal absorbers in the atmosphere, H\sb2O, CO\sb2 and O\sb3, vary erratically and rapidly with wavelength. To account for this variation, the correlated-k distribution method is employed to simplify the integration over wavelength necessary for calculation of warming/cooling rates. The radiation model, utilizing appropriate absorption and scattering cross sections, is compared with ultraviolet radiation measurements. The comparison suggests that further experiments are required. Ultraviolet (UV) and photosynthetically active radiation (PAR) is computed for high and low latitudes for clear and cloudy skies under different ozone concentrations. An ozone depletion increases UV-B radiation detrimental to life. Water clouds diminish UV-B, UV-A and PAR for low surface albedos and increase them for high albedos. The relative amount of harmful UV-B increases on overcast days. The daily radiation doses exhibit small monthly variations at low latitudes but vary by a factor of 3 at high latitudes. Photodissociation and warming/cooling rates are calculated for clear skies, aerosol loaded atmospheres, and atmospheres with cirrus and water clouds. After major volcanic explosions aerosols change O\sb3 and NO\sb2 photodissociation rates by 20%. Both aged aerosols and cirrus clouds have little effect on photodissociation rates. Water clouds increase $(\sim$100%) photodissociation rates that are sensitive to visible radiation above the cloud. Solar warming rates vary by 50% in the stratosphere due to changing surface albedo. Water clouds have a similar effect. The net effect of cirrus clouds is to warm the troposphere and the stratosphere. Only extreme volcanic aerosol loadings affect the terrestrial warming rate, causing warming below the aerosol layer and cooling above it. Aerosols give increased solar warming above the aerosol layer and cooling below it

Ground-based measurements of total ozone column amount with a multichannel moderate-bandwidth filter instrument at the Troll research station, Antarctica

Combining information from several channels of the Norwegian Institute for Air Research (NILU-UV) irradiance meter, one may determine the total ozone column (TOC) amount. A NILU-UV instrument has been deployed and operated on two locations at Troll research station in Jutulsessen, Queen Maud Land, Antarctica, for several years. The method used to determine the TOC amount is presented, and the derived TOC values are compared with those obtained from the Ozone Monitoring Instrument (OMI) located on NASA’s AURA satellite. The findings show that the NILU-UV TOC amounts correlate well with the results of the OMI and that the NILU-UV instruments are suitable for monitoring the long-term change and development of the ozone hole. Because of the large footprint of OMI, NILU-UV is a more suitable instrument for local measurements.publishedVersio

Ash and ice clouds during the Mt Kelud February 2014 eruption as interpreted from IASI and AVHRR/3 observations

During the Mt Kelud February 2014 eruption the ash cloud was detectable on 13–14 February in the infrared with the reverse absorption technique by, for example, the Advanced Very High Resolution Radiometer (AVHRR/3). The Infrared Atmospheric Sounding Interferometer (IASI) observed the ash cloud also on 15 February when AVHRR did not detect any ash signal. The differences between ash detection with AVHRR/3 and IASI are discussed along with the reasons for the differences, supported by radiative transfer modelling. The effect of concurrent ice clouds on the ash detection and the ash signal in the IASI measurements is demonstrated. Specifically, a radiative transfer model is used to simulate IASI spectra with ash-only, with ice cloud only and with both ash and ice clouds. It is shown that modelled IASI spectra with ash and ice clouds reproduce the measured IASI spectra better than ash-only- or ice-only-modelled spectra. The ash and ice modelled spectra that best reproduce the IASI spectra contain about a factor of 12 less ash than the ash-only spectra that come closest to reproducing the measured spectra

Tilt error in cryospheric surface radiation measurements at high latitudes: A model study

We have evaluated the magnitude and makeup of error in cryospheric radiation observations due to small sensor misalignment in in situ measurements of solar irradiance. This error is examined through simulation of diffuse and direct irradiance arriving at a detector with a cosine-response fore optic. Emphasis is placed on assessing total error over the solar shortwave spectrum from 250 to 4500 nm, as well as supporting investigation over other relevant shortwave spectral ranges. The total measurement error introduced by sensor tilt is dominated by the direct component. For a typical high-latitude albedo measurement with a solar zenith angle of 60°, a sensor tilted by 1, 3, and 5° can, respectively introduce up to 2.7, 8.1, and 13.5 % error into the measured irradiance and similar errors in the derived albedo. Depending on the daily range of solar azimuth and zenith angles, significant measurement error can persist also in integrated daily irradiance and albedo. Simulations including a cloud layer demonstrate decreasing tilt error with increasing cloud optical depth