Surface plasmon resonance imaging detection of silver nanoparticle-tagged immunoglobulin

This article is available open access through the publisher’s website at the link below. Copyright @ 2011 The Royal Society.The detection sensitivity of silver nanoparticle (AgNP)-tagged goat immunoglobulin G (gIgG) microarrays was investigated by studying surface plasmon resonance (SPR) images captured in the visible wavelength range with the help of a Kretchmann-configured optical coupling set-up. The functionalization of anti-gIgG molecules on the AgNP surface was studied using transmission electron microscopy, photon correlation measurements and UV–visible absorption spectroscopy. A value of 1.3 × 107 M−1 was obtained for the antibody–antigen binding constant by monitoring the binding events at a particular resonance wavelength. The detection limit of this SPR imaging instrument is 6.66 nM of gIgG achieved through signal enhancement by a factor of larger than 4 owing to nanoparticle tagging with the antibody.The European Commissio

Emission of light through thin silver films via near-field coupling to surface plasmon polaritons

Copyright © 2006 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in Applied Physics Letters 88 (2006) and may be found at http://link.aip.org/link/?APPLAB/88/051109/1We show that the emission of light from a dye layer through an adjacent thin silver film is maximal for a silver thickness of approximately 50 nm. This effect is explained as the result of competition between enhancement of the electric field at the metal surface due to the excitation of a surface plasmon-polariton mode, the amount of power coupled to the surface plasmon-polariton mode, and the attenuation of the field transmitted through the silver, all three of which vary with metal thickness. We indicate how these findings may be of relevance in the design of some surface plasmon-polariton-based fluorescence biosensing schemes

Reply to "Can gravitational dynamics be obtained by diffeomorphism invariance of action?"

In a previous work we showed that, in a suitable setting, one can use diffeomorphism invariance in order to derive gravitational field equations from boundary terms of the gravitational action. Standing by our results we reply here to a recent comment questioning their validity.Comment: Accepted for publication in PR

Sensing using differential surface plasmon ellipsometry

Copyright © 2004 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in Journal of Applied Physics 96 (2004) and may be found at http://link.aip.org/link/?JAPIAU/96/3004/1In this work a differential ellipsometric method utilizing surface plasmons (SPs) for monitoring refractive index changes, which could be used in chemical and biological sensors, is presented. The method is based upon determining the azimuth of elliptically polarized light reflected from a Kretschmann SP system, resulting from linearly polarized light containing both p and s components incident upon it. The sensitivity of this azimuth to the refractive index of a dielectric on the nonprism side of the metal film is demonstrated both experimentally and theoretically. The smallest refractive index change which is resolvable is of the order of 10–7 refractive index units, although it is believed that this could be improved upon were it not for experimental constraints due to atmospheric changes and vibrations. The method requires the Kretschmann configuration to be oriented at a fixed angle, and the SP to be excited at a fixed wavelength. With no moving parts this method would be particularly robust from an application point of view

Spontaneous emission of radiation by metallic electrons in the presence of electromagnetic fields of surface plasmon oscillations

The spontaneous emission of radiation of metallic electrons embedded in a high-intensity enhanced surface plasmon field is considered analytically. The electrons are described by exact dressed quantum states which contain the interaction with the plasmon field non-perturbatively. Considerable deviations from the pertubative behaviour have been found in the intensity dependence of the emitted fundamental and the second harmonic signals, even at moderate incoming laser intensities. The theoretical predictions deduced from the formalism are in good qualitative agreement with the experimental results.Comment: 23 pages, 6 figure

Performance analysis of higher mode spoof surface plasmon polariton for terahertz sensing

We investigated the spoof surface plasmon polaritons (SSPPs) on 1D grooved metal surface for terahertz sensing of refractive index of the filling analyte through a prism-coupling attenuated total reflection setup. From the dispersion relation analysis and the finite element method-based simulation, we revealed that the dispersion curve of SSPP got suppressed as the filling refractive index increased, which cause the coupling resonance frequency redshifting in the reflection spectrum. The simulated results for testing various refractive indexes demonstrated that the incident angle of terahertz radiation has a great effect on the performance of sensing. Smaller incident angle will result in a higher sensitive sensing with a narrower detection range. In the meanwhile, the higher order mode SSPP-based sensing has a higher sensitivity with a narrower detection range. The maximum sensitivity is 2.57 THz/RIU for the second-order mode sensing at 45° internal incident angle. The proposed SSPP-based method has great potential for high sensitive terahertz sensing

A Higgs Mechanism for Gravity

In this paper we elaborate on the idea of an emergent spacetime which arises due to the dynamical breaking of diffeomorphism invariance in the early universe. In preparation for an explicit symmetry breaking scenario, we consider nonlinear realizations of the group of analytical diffeomorphisms which provide a unified description of spacetime structures. We find that gravitational fields, such as the affine connection, metric and coordinates, can all be interpreted as Goldstone fields of the diffeomorphism group. We then construct a Higgs mechanism for gravity in which an affine spacetime evolves into a Riemannian one by the condensation of a metric. The symmetry breaking potential is identical to that of hybrid inflation but with the non-inflaton scalar extended to a symmetric second rank tensor. This tensor is required for the realization of the metric as a Higgs field. We finally comment on the role of Goldstone coordinates as a dynamical fluid of reference.Comment: 15 pages, 2 figures, 3 tables, appendix C on on-shell d.o.f. added, references adde

Otto-coupled surface plasmons in a liquid crystal cell

Copyright © 2009 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in Applied Physics Letters 95 (2009) and may be found at http://link.aip.org/link/?APPLAB/95/171102/1Surface plasmons on silver in the visible domain are excited using a several micron thick layer of liquid crystal as the optical tunnel barrier. This thickness is possible when the orientation of the director in the liquid crystal varies from homeotropic at the entrance surface (against the coupling prism) to homogeneous on the thick silver layer at the other side of the cell, with the director tilting in a plane normal to the plane of incidence. This geometry also allows the excitation of guided modes, which mixes with the surface plasmon resonance. Both types of mode are then explored as a function of applied voltage