Giant absorption of light by molecular vibrations on a chip

Vibrational overtone spectroscopy of molecules is a powerful tool for drawing information on molecular structure and dynamics. It relies on absorption of near infrared radiation (NIR) by molecular vibrations. Here we show the experimental evidence of giant enhancement of the absorption of light in solutions of organic molecules due to the switch from ballistic to diffusive propagation of light through a channel silicate glass waveguide. We also experimentally address a dynamics of absorption as a function of time of adsorption of the organic molecules on a waveguide. The observed enhancement in diffusion regime is by a factor of 300 in N-Methylaniline and by factor of 80 in Aniline compared to the expected values in the ballistic propagation of light in a waveguide. Our results underscore the importance of a guide surface modification and the disordered6 molecular nano-layer in enhancement of absorption by amines on engineered integrated system

Ultimate photo-induced Kerr rotation achieved in semiconductor microcavities

Photoinduced Kerr rotation by more than $\pi /2$ radians is demonstrated in planar quantum well microcavity in the strong coupling regime. This result is close to the predicted theoretical maximum of $\pi$. It is achieved by engineering microcavity parameters such that the optical impedance matching condition is reached at the smallest negative detuning between exciton resonance and the cavity mode. This ensures the optimum combination of the exciton induced optical non-linearity and the enhancement of the Kerr angle by the cavity. Comprehensive analysis of the polarization state of the light in this regime shows that both renormalization of the exciton energy and the saturation of the excitonic resonance contribute to the observed optical nonlinearities.Comment: Shortened version prepared to submit in Phys. Rev. Letter

Optically induced transparency in bosonic cascade lasers

Bosonic cascade lasers are terahertz (THz) lasers based on stimulated radiative transitions between bosonic condensates of excitons or exciton-polaritons confined in a trap. We study the interaction of an incoming THz pulse resonant in frequency with the transitions between neighboring energy levels of the cascade. We show that at certain optical pump conditions the cascade becomes transparent to the incident pulse: it neither absorbs nor amplifies it, in the mean field approximation. The populations of intermediate levels of the bosonic cascade change as the THz pulse passes, nevertheless. In comparison, a fermionic cascade laser does not reveal any of these properties.Comment: 4 pages, 5 figure

Quantization of entropy in a quasi-two-dimensional electron gas

We demonstrate that the partial entropy of a two-dimensional electron gas (2DEG) exhibits quantized peaks at resonances between the chemical potential and electron levels of size quantization. In the limit of no scattering, the peaks depend only on the subband quantization number and are independent on material parameters, shape of the confining potential, electron effective mass and temperature. The quantization of partial entropy is a signature of a topological phase transition in a 2DEG. In the presence of stationary disorder, the magnitude of peaks decreases. Its deviation from the quantized values is a direct measure of the disorder induced smearing of the electronic density of states.Comment: 4 pages, 2 figure